Hidenori Yonehara

Spatial distribution of thoron and radon concentrations in the indoor air of a traditional Japanese wooden house.

A radon-thoron discriminative passive dosimeter has been developed that can estimate both radon (222Rn) and thoron (220Rn) concentrations at the same time. Two polycarbonate films are installed as solid-state nuclear track detectors in the dosimeter housing. One film registers alpha tracks originating from predominantly thoron and its progeny together with a small contribution from radon, and the other film registers alpha tracks originating from radon and its progeny together with a negligible contribution from thoron. The lower detection limit is estimated to be 2.9 Bq m-3 for the radon concentration and 9.0 Bq m-3 for the thoron concentration for 2 mo exposure. Preliminary measurements from 1991-1992, in a traditional Japanese wooden house located in Kyoto, indicated that the indoor thoron concentration increases exponentially as the interior mud (or plaster-coated) wall is approached. A soil-based plaster commonly used in Japanese wooden houses to fill walls (or as a surface coating on the walls) is the probable source of the indoor thoron. Since thoron is not measured by the usual radon measurements, and the majority of Japanese houses are made of wood, attention should be paid to indoor thoron and its decay products, which may give a significant fraction of the total natural radiation exposure to the general public.

Radon and thoron exposures for cave residents in Shanxi and Shaanxi provinces.

Abstract Tokonami, S., Sun, Q., Akiba, S., Zhuo, W., Furukawa, M., Ishikawa, T., Hou, C., Zhang, S., Narazaki, Y., Ohji, B., Yonehara, H. and Yamada, Y. Radon and Thoron Exposures for Cave Residents in Shanxi and Shaanxi Provinces. Radiat. Res. 162, 390–396 (2004). Measurements of natural radiation were carried out in cave dwellings distributed in the Chinese loess plateau. Those dwellings are located in Shanxi and Shaanxi provinces. Radon and thoron gas concentrations were measured using a passive integrating radon-thoron discriminative detector. Concentrations of thoron decay products were estimated from measurements of their deposition rates. A detector was placed at the center of each dwelling for 6 months and replaced with a fresh one for another 6 months. Measurements were conducted in 202 dwellings from August 2001 through August 2002. A short-term measurement was conducted during the observation period. In addition, γ-ray dose rates were measured both indoors and outdoors with an electronic pocket dosimeter. Radioactivities in soil were determined by γ-ray spectrometry with a pure germanium detector. Among 193 dwellings, indoor radon concentrations ranged from 19 to 195 Bq m−3 with a geometric mean (GM) of 57 Bq m−3, indoor thoron concentrations ranged from 10 to 865 Bq m−3 with a GM of 153 Bq m−3, and indoor equilibrium equivalent thoron concentrations ranged from 0.3 to 4.9 Bq m−3 with a GM of 1.6 Bq m−3. Arithmetic means of the γ-ray dose rates were estimated to be 140 nGy h−1 indoors and 110 nGy h−1 outdoors. The present study revealed that the presence of thoron is not negligible for accurate radon measurements and thus that special attention should be paid to thoron and its decay products for dose assessment in such an environment. More systematic studies are necessary for a better understanding of thoron and its decay products.

A simple passive monitor for integrating measurements of indoor thoron concentrations

A simple passive monitor was developed for integrating measurements of indoor thoron concentrations. The monitor was remodeled from a commercially available radon monitor with allyl diglycol carbonate (CR-39) detector. By adding four holes (φ=12 mm) and covering them with high permeability of filter paper, the air exchange rate of the monitor was largely enhanced. The technical characteristics of both the radon and thoron monitors were examined through calibration experiments. A high conversion factor of 1.32±0.14 tracks cm−2⋅(kBq m−3 h−1)−1 and the low lower detection limit for thoron measurements provide the essential conditions for measuring thoron more precisely and sensitively. Furthermore, the main physical advantages of the monitor are its simple construction, light weight, and compactness as well as its low cost, which are preferable for large-scale and long-term indoor surveys. Simultaneous measurements of both indoor thoron and radon are indispensable for accurate assessments of public exposure ...

Radon–Thoron Discriminative Measurements in Gansu Province, China, and Their Implication for Dose Estimates

Indoor radon measurements were carried out in cave dwellings of the Chinese loess plateau in Gansu province, where previously the Laboratory of Industrial Hygiene (LIH), China, and the U.S. National Cancer Institute (NCI) had conducted an international collaborative epidemiological study. The LIH–NCI study showed an increased lung cancer risk due to high residential radon levels, and estimated the excess odds ratio at 100 Bq/m3 to be 0.19 (Wang et al., 2002). The present study used two types of newly developed passive monitors: One is a discriminative monitor for radon and thoron; the other is a selective monitor for thoron decay products. The arithmetic mean concentrations of indoor radon and thoron were 91 and 351 Bq/m3, respectively. As reported by our previous study in Shanxi and Shaanxi provinces (Tokonami et al., 2004), the presence of high thoron concentration was confirmed and thoron was predominant over radon in the cave dwellings. However, the mean equilibrium equivalent thoron concentration (EETC) was found to be much lower than expected when assuming the equilibrium factor of 0.1 provided by the UNSCEAR (2000) report. The effective dose by radon and thoron decay products was estimated to be 3.08 mSv/yr. It was significantly lower than the dose of 8.22 mSv/yr estimated from the measurements that did not take into consideration any discrimination between radon and thoron. Excess relative risk of lung cancer per sievert may be much higher than the risk estimated from the LIH–NCI study, considering that discriminative measurements were not used in their study.

Simple discriminative measurement technique for radon and thoron concentrations with a single scintillation cell

A simple, discriminative measurement technique for radon and thoron concentrations is discussed. In this technique, a single scintillation cell is used for both radon and thoron measurements. It consists of two measurements that use the difference of the half life between the two isotopes. Alpha counting efficiencies for their associated radionuclides were estimated by a Monte Carlo calculation. When evaluating the conversion factor for concentration on two types of scintillation cells, both agreed well with experimental values. Optimum measurement conditions on the timetable are also discussed. This technique can provide two concentrations promptly. Although it is not highly sensitive, it is applicable to performance tests for radon/thoron monitors and simultaneous exhalation rate measurements for both radon and thoron.

Influence of air flow on the behavior of thoron and its progeny in a traditional Japanese house.

Air flow influence on the spatial distribution of thoron (220Rn) concentration in a typical Japanese traditional house was investigated at various indoor air flow levels. The effect of air flow on the behavior of both thoron and radon progeny were examined simultaneously. Measurements were carried out by using two types of passive monitors, the radon-thoron discriminative monitor and the Radtrak monitor. Thoron and radon progeny were measured by filter grab sampling with ZnS scintillation counting. Under static condition, a horizontal distribution with greatly varied thoron concentrations was found as reported by previous studies. Under turbulent conditions, thoron concentrations in the middle of the room increased and the concentration gradient of thoron gas became lower. An obvious vertical distribution of thoron was also observed. Prominent diurnal variation of radon progeny concentrations was observed whereas that of thoron progeny concentrations was not. Concentration of thoron progeny changed little at different air flow levels, although the thoron gas level at the middle of the room varied significantly. The influence of air flows on detection efficiencies of the two types of thoron monitors were also checked. The mechanism of behavioral change of thoron and its progeny in turbulent atmosphere is discussed.

Radon and thoron doses in kindergartens and elementary schools

Exposing the Raduet Rn-Tn solid-state nuclear track detectors, radon (Rn: (222)Rn) and thoron (Tn: (220)Rn) activity concentrations have been measured in 7 kindergartens and 18 elementary schools in Slovenia. Diurnal variations of both gases were monitored using a Rad7 device. The Rn concentration was in the range from 145 to 794 Bq m(-3) in kindergartens and from 70 to 770 Bq m(-3) in schools, and the Tn concentration was in the range from 21 to 73 Bq m(-3) in kindergartens and from 4 to 91 Bq m(-3) in schools. The Tn versus Rn concentration ratio varied from 0.02 to 0.83. Monthly effective doses due to radon and its decay products ranged from 109 to 600 μSv month(-1) in kindergartens and from 21 to 232 μSv month(-1) in schools, and those due to thoron and its decay products ranged from 3.8 to 13.3 μSv month(-1) in kindergartens and from 0.29 to 6.62 μSv month(-1) in schools. The contribution of thoron to the total effective dose was from 1.3 to 11 % in kindergartens and from 0.4 to 17 % in schools.

Perceived risk of nuclear power and other risks during the last 25 years in Japan.

Abstract The present study described the results of three “fixed-point” surveys on perceived risk related to a list of social and individual risk events during 25 years in Japan. Female clerical staff and researchers were asked to rank 30 items related to various types of technologies and human activities according to their subjective judgments on the order of perceived magnitude of risk in 1983, 1992, and 2007. A similar survey was undertaken for Japanese citizens using web-based questionnaires in 2007. In general, the risk perceptions of the Japanese people, irrespective of gender, age, and occupation, have been uniform during the last 25 years. The female clerical staffs have consistently judged nuclear power as most risky during the last 25 years, whereas researchers’ judgment fluctuated with events such as the Chernobyl accident. The ranking of the risk of motor vehicles fell during the 25-y period, whereas those of health risks with food preservatives, x-rays, and antibiotics rose transiently in the 1992 survey. During the 15 years from 1992 to 2007, people tended to learn how to accommodate themselves to these technologies with low risks in exchange for high benefits, except in the case of nuclear power. Nuclear power was regarded as a high-risk item by the Japanese even before the Fukushima nuclear power plant accident in March 2011. This partly explains that the crisis inevitably provokes further high risk perception in Japan, although the overall health threat to the human population in Japan is estimated to be relatively limited so far.

Meta-analysis of second cancer risk after radiotherapy among childhood cancer survivors.

Cancer risks among childhood cancer survivors following radiotherapy have not yet been well characterised in terms of radiation dose. A meta-analysis of studies on the excess relative risk per gray (ERR) of second cancer was conducted previously; unfortunately, the small number of eligible studies restricted quantitative evaluations. To solve this problem, a statistical method to calculate ERR estimates from other estimates was developed, and a meta-analysis was conducted again. The PubMed database was searched and 26 relevant studies were identified. ERR estimates were available in 15 studies, and for the other 11 studies, the regression-based model was used to calculate ERR estimates from other estimates. The overall ERR estimate was 0.40, which was much lower than that of atomic bomb survivors exposed as young children. Heterogeneity of the risk among studies was suggested, and a further study is needed to explore the heterogeneity among studies.

Determination of rare earth elements, thorium and uranium by inductively coupled plasma mass spectrometry and strontium isotopes by thermal ionization mass spectrometry in soil samples of Bryansk region contaminated due to Chernobyl accident

The present paper describes the inductively coupled plasma mass spectrometric (ICP-MS) determination of rare earth elements (REEs), thorium and uranium in forest, pasture, field and kitchen garden soils from a Russian territory and in certified reference materials (JLK-1, JSD-2 and BCR-1). In addition to concentration data, strontium isotopic composition of the soil samples were measured by thermal ionization mass spectrometry. The measurements contributed to the understanding of the background levels of these elements in an area contaminated due to Chernobyl accident. There was not a significant variation in the concentration of REEs at different depth levels in forest soil samples, however, the ratio of Th/U varied from 3.32 to 3.60. Though concentration of U and Th varied to some extent, the ratio did not show much variation. The value of 87Sr/86Sr ratio, was in the top layer soil sample relatively higher than in the lower layers.