Hisaki Kofuji

134Cs and 137Cs activities in coastal seawater along Northern Sanriku and Tsugaru Strait, northeastern Japan, after Fukushima Dai-ichi Nuclear Power Plant accident

A total of 37 seawater samples were collected at 10 sites along the coastline of the Northern Sanriku and Tsugaru Strait, 250-450 km north of the Fukushima Dai-ichi Nuclear Power Plant in April-December 2009 and May-June 2011, and analyzed for (134)Cs and (137)Cs activities using low-background γ-spectrometry. The (134)Cs and (137)Cs activities measured in these samples in May 2011 were found to be 2-3 mBq/L and 2.5-4 mBq/L, respectively. By June, these values had decreased by 25-45%/month and 5-30%/month, respectively. These results can be plausibly explained by surface infusion of these isotopes into the sea by atmospheric transport from Fukushima and their subsequent reduction by water migration to off-shore and deeper regions.

Lateral variation of 134Cs and 137Cs concentrations in surface seawater in and around the Japan Sea after the Fukushima Dai-ichi Nuclear Power Plant accident.

A total of 82 surface seawater samples was collected in the Japan Sea and the southwestern Okhotsk Sea before and after the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident. Analysis of (134)Cs and (137)Cs concentrations using low-background γ-spectrometry revealed that the (137)Cs concentration of the samples collected in June 2011 was 1.5-2.8mBq/L, which is approximately 1-2 times higher than the pre-accident (137)Cs level, while the (134)Cs concentration was less than detectable to 1mBq/L. In addition to (134)Cs being clearly detected (∼1mBq/L), (137)Cs concentration in water samples from the northeastern Japan Sea (2-2.8mBq/L) was also higher than that from the coast in the southwestern Japan Sea (∼1.5mBq/L). These higher concentrations in the northeastern Japan Sea could be ascribed to the atmospheric transport of nuclides from the FDNPP as aerosols and subsequent transport and dilution after delivery to the sea surface.

Residence times of global weapons testing fallout 237Np in a grassland soil compared to 239 + 240Pu, 241Am, and 137Cs.

The vertical distribution of weapons testing fallout 237Np has been determined in an undisturbed grassland soil (Alfisol). By using a compartmental model for multi-layered soils, the mean residence half-times of 237Np in each soil layer were calculated and compared with results on weapons fallout 239 + 240Pu, 241Am and 137Cs in the same soil. The results show that the mobility of 237Np was in most soil horizons either equal or slightly enhanced as compared to that of Pu, Am, and radiocesium.

Spatial variations of low levels of 134Cs and 137Cs in seawaters within the Sea of Japan after the Fukushima Dai-ichi Nuclear Power Plant accident

Our method based on low background γ-spectrometry enabled the measurement of low radiocesium concentrations in only 20 L of seawater. In May 2011 after deposition of radiocesium, (134)Cs concentration in surface water within the Sea of Japan was confirmed to be significantly small (<0.1-1 mBq/L) by the method. The concentration was not detected (<0.1 mBq/L) below 50 m depth. The Fukushima-derived radiocesium migrated from the surface water of the Sea of Japan without advection to below the thermocline.

228Ra/226Ra ratio and 7Be concentration in the Sea of Japan as indicators for water transport: comparison with migration pattern of Fukushima Dai-ichi NPP-derived 134Cs and 137Cs

To assess the migration patterns of radiocesium emitted from the Fukushima Dai-ichi Nuclear Power Plant (FDNPP), we analyzed (228)Ra/(226)Ra ratios and (7)Be concentrations and compared them with (134)Cs and (137)Cs concentrations in seawater samples collected within the Sea of Japan before and after the FDNPP accident (i.e., during the period 2007-2012) using low-background γ-spectrometry. The (228)Ra/(226)Ra ratios in surface waters exhibited lateral and seasonal variations, reflecting the flow patterns of surface water. This indicates the transport patterns of the FDNPP-derived radiocesium by surface water. Cosmogenic (7)Be (half-life: 53.3 d) exhibited markedly high concentrations (5-10 mBq/L) at depths shallower than 50 m, with concentrations decreasing steeply (0.2-2 mBq/L) at depths of 50-250 m. The distribution of (7)Be concentrations suggests that the downward delivery of the FDNPP-derived radiocesium to below 50 m depth was negligible for a few months prior to its removal from the Sea of Japan.

The geochemistry of uranium in pore waters from lake sediments

The concentration of pore water uranium in six sediments from oligotrophic, mesotrophic, acidotrophic and dystrophic lakes was measured by inductively coupled plasma-mass spectrometry. Profiles of pore water U can be divided into two groups such as low (17±7 ng/l) and high concentration (69±30 ng/l). These values were 1–2 orders of magnitude higher than that of lake waters (6±4 ng/l) due to the release of U from the sediments by decomposition of organic materials. Variations in pore water U concentrations seem to relate to the differences in pore water pH, the association forms, and their contents of U in the lake sediments.

Spatial variations of 226Ra, 228Ra, 137Cs, and 228Th activities in the southwestern Okhotsk Sea

We collected 14 water column seawater samples in the southwestern Okhotsk Sea and 7 surface samples around the northern area of Hokkaido Island, Northern Japan, and employed low-background γ-spectrometry with convenient minimal radiochemical processing to determine the activities of (226)Ra (half-life t(1/2)=1600 y), (228)Ra (5.75 y), (137)Cs (30.2 y), and (228)Th (1.91 y) in the samples. Activities of (226)Ra (~2.3 mBq/L), (228)Ra (~0.7 mBq/L), and (137)Cs (~1 mBq/L) of surface waters on the Okhotsk Sea side show notable differences from those on the Japan Sea side (Soya Warm Current Water; SWCW) (~1.5 mBq/L; 1.5-2 mBq/L; 1.4-1.6 mBq/L), indicating their different origins and lateral mixing patterns. All of these nuclides exhibit unique vertical profiles; activities of soluble (226)Ra, (228)Ra, (137)Cs, and reactive (228)Th exhibit small variations from 50 to 500 m depth ((226)Ra, ~2.2 mBq/L; (228)Ra, ~0.4 mBq/L; (137)Cs, ~1 mBq/L; (228)Th, ~0.13 mBq/L). These profiles can be explained by the convective mixing of surface water such as the East Sakhalin Current Water (ESCW) to this layer.

Neutron activation of chemical reagents exposed to the neutrons released by the JCO criticality accident

Induced radionuclides in the chemical reagents collected in the JCOs Wet Chemistry Testing Laboratory were measured using HPGe detectors in the Low Level Radioactivity Laboratory (LLRL) and in Ogoya underground laboratory. Radioactive nuclei produced by neutron capture reactions were detected in most of the reagents. Products of the (n, p) reaction were detected only in Raney-Nickel and metallic powder of stainless steel. Preliminary estimation of the neutron fluence was made on the basis of determinations of radionuclide concentrations.

Residual neutron-induced radionuclides in a soil sample collected in the vicinity of the criticality accident site in Tokai-mura, Japan: A Progress Report

Abstract Residual neutron-induced radionuclides were measured in a soil sample collected in the vicinity of the location where a criticality accident occurred (in Tokai-mura, from 30 September to 1 October, 1999). Concentrations of 24 Na , 140 La , 122 Sb , 59 Fe , 124 Sb , 46 Sc , 65 Zn , 134 Cs and 60 Co in the soil sample were determined by γ-ray spectrometry, and neutron activation analysis was carried out for selected target elements in the sample. Tentative estimates of the apparent thermal and epithermal neutron fluences which reached the sample were obtained through combined analyses of 59 Fe / 58 Fe , 124 Sb / 123 Sb , 46 Sc / 45 Sc , 65 Zn / 64 Zn , 134 Cs / 133 Cs and 60 Co / 59 Co .

Opening of the closed water area and consequent changes of 228Ra/226Ra activity ratios in coastal lagoon Nakaumi, southwest Japan

In Lake Nakaumi, the second largest coastal lagoon in Japan, artificially closed (Honjyo) area, which was left untouched for 28 years, was partly opened in May, 2009. (228)Ra/(226)Ra ratio of waters in Honjyo area and Lake Nakaumi showed a well-tuned seasonal variation exhibiting high value in summer. After the opening event, however, the (228)Ra/(226)Ra ratios in the Honjyo water showed an unclear seasonal variation in both surface and deep water. This opening event caused the change of active movement of lake and marine water.