Humayun Khan

Determination of uranium contents in rock samples from Kakul phosphate deposit, Abbotabad (Pakistan), using fission-track technique

Abstract Some times high uranium contents are present in the phosphate rocks used for the manufacturing of fertilizer. In view of the harmful effects on human health due to the processing and use of such fertilizers in agriculture, it is important to analyse phosphate rocks for uranium content determination. Ten representative rock samples from Kakul phosphate deposit exposed near Abbotabad, Pakistan which are used for the manufacturing of fertilizers were studied for uranium content determination with the help of fission track and neutron activation analysis techniques. Each sample was split into three parts. The first and second parts (solid slabs and pellets) were subjected to fission track analysis, while the third part was analysed using neutron activation analysis technique for comparison. On the average a uranium content of 37 ppm was found in the phosphate rocks. The results of uranium content determinations with the help of fission track and neutron activation analysis techniques show a remarked resemblance up to ±0.1%. This indicates that the fission track analysis technique of uranium content determination is a reliable method inspite of its simplicity. The uranium content in the Kakul deposits is within the permissible limit allowed for the mining and processing of the phosphate rocks for the manufacturing of fertilizers.

Interactions of Relativistic Heavy Ions in Thick Heavy Element Targets and Some Unresolved Problems

Interactions of relativistic heavy ions with total energies above 30 GeV in thick Cu and Pb targets (≥ 2 cm) have been studied with various techniques. Radiochemical irradiation experiments using thick Cu targets, both in a compact form or as diluted “2π-Cu targets” have been carried out with several relativistic heavy ions, such as 44 GeV 12C (JINR, Dubna, Russia) and 72 GeV 40Ar (LBL, Berkeley, USA). Neutron measuring experiments using thick targets irradiated with various relativistic heavy ions up to 44 GeV 12C have been performed at the JINR. In addition, the number of “black prongs” in nuclear interactions (due to protons with energies less than 30 MeV and emitted from the target-like interaction partner at rest) produced with 72 GeV 22Ne ions in nuclear emulsion plates has been measured in the first nuclear interaction of the primary 22Ne ion and in the following second nuclear interaction of the secondary heavy (Z > 1) ion. Some essential results have been obtained. (1) Spallation products produced by relativistic secondary fragments in interactions ([44 GeV 12C or 72 GeV 40Ar] + Cu) within thick copper yield fewer products close to the target and many more products far away from the target as compared to primary beam interactions. This applies also to secondary particles emitted into large angles (Θ > 10°). (2) The neutron production of 44 GeV 12C within thick Cu and Pb targets is beyond the estimated yield as based on experiments with 12 GeV 12C. These rather independent experimental results cannot be understood within well-accepted nuclear reaction models. They appear to present unresolved problems.

Unroofing history of the Sillai Patti granite gneiss, Pakistan: constraints from zircon fission-track dating

Abstract A group of alkaline igneous rocks is exposed in the north of the Peshawar Plain, extending from Tarbela in the east up to Loe–Shilman near the Pakistan–Afghanistan border in the west. The alkaline rocks consist mainly of granites, syenites, gabbros, ijolites and carbonatites. Granitic gneisses of Paleozoic age are exposed at the Malakand and further westward at Sillai Patti. However, the fission-track dating studies on zircon, based on the present work, indicate that the age of the Sillai Patti granite gneiss is less than the absolute age of granite gneisses. Therefore, the zircon fission-track age of 24.28±2.97 Ma of the Sillai Patti granite gneiss, represents a time of post-metamorphic denudation history of the area, when these rocks passed through the 210°C isotherm, corresponding to a depth of about 6.7 km inside the earths crust from their present position if a paleogeothermal gradient of 30°C/km is assumed to have prevailed. Our average fission-track zircon age of 24.28±2.97 Ma is very similar to the average fission-track zircon age of 25.4±0.7 Ma of Mansehra granites. Average cooling rates of the Mansehra and Sillai Patti granite gneisses have been computed to be (8.00±0.22)°C/Ma and (8.00±0.98)°C/Ma, while the average denudation rates of the Mansehra and Sillai Patti granite gneisses have been computed to be (0.262±0.007) and (0.274±0.034) mm / yr , respectively, on the basis of zircon fission-track ages for the period between 25 Ma and the present time. This indicates that the two complexes have experienced similar average cooling/uplift-induced denudation histories during the last 25 Ma or so.