Ilya Alexeev

Remote atmospheric breakdown for standoff detection by using an intense short laser pulse

A remote atmospheric breakdown is a very rich source of UV and broadband visible light that could provide an early warning of the presence of chemical-biological warfare agents at extended standoff distances. A negatively chirped laser pulse propagating in air compresses in time and focuses transversely, which results in a rapid laser intensity increase and ionization near the focal region that can be located kilometers away from the laser system. Proof-of-principle laboratory experiments are performed on the generation of remote atmospheric breakdown and the spectroscopic detection of mock biological warfare agents. We have generated third harmonics at 267 nm and UV broadband radiation in air from the compression and focusing of femtosecond laser pulses. Fluorescence emission from albumin aerosols as they were illuminated by the femtosecond laser pulse has been observed.

Longitudinal compression of short laser pulses in air

We have performed laboratory experiments to study long distance propagation of large bandwidth ultrashort laser pulses in air. Initial pulse length, frequency chirping, and laser pulse energy were varied where the maximum propagation distance was up to 105 m. We have demonstrated the compression of initially negatively chirped low intensity laser pulses due to the linear group velocity dispersion of air. The characteristics of the compressed pulse such as pulse duration and spectral chirping were found to be significantly affected by the laser pulse intensity, with higher intensities corresponding to longer minimum compressed pulse duration.

Measurements of intense femtosecond laser pulse propagation in air

The nonlinear self-focusing of an intense femtosecond pulse propagating in air can be balanced by the plasma defocusing as the laser intensity is increased above the threshold for multiphoton ionization. The resultant laser∕plasma filament can extend many meters, suitable for many applications such as remote atmospheric breakdown, laser induced electrical discharge, and femtosecond laser material interactions. Direct (bore-sight) measurements of filament size and fluence over 4 m showed a preservation of the total energy in the filament during propagation. This indicates the energy lost in creating the central plasma column through multiphoton ionization was continuously being replenished from the surrounding radiation. Electrical measurement of the filament conductivity estimated the plasma density to be 1×1016cm−3 and electrical discharges triggered by a femtosecond laser filament were found to occur at substantially reduced breakdown fields.

Ultraviolet light generation by intense laser filaments propagating in air

Sub-millimeter diameter filaments can develop from laser self-focusing in air. These filaments produce ultraviolet radiations in form of third harmonics and frequency upshifting. Using high-power laser we observed generation of third harmonic radiation in air.

Characterization of the third-harmonic radiation generated by intense laser self-formed filaments propagating in air

We perform laboratory experiments to study ultraviolet radiation generated by intense self-formed laser filaments produced by propagating high-power femtosecond laser pulses in air. The laser used in the experiment is a 0.5 TW Ti:sapphire system with the center wavelength at 800 nm. The observed ultraviolet emission occurs in the form of the third harmonic and frequency-upshifted radiation from the fundamental. We present direct characterization of the generated harmonic and frequency-upshifted radiation, including transverse imaging and spatially resolved spectral measurements.

Exploring the depth range for three-dimensional laser machining with aberration correction

The spherical aberration generated when focusing from air into another medium limits the depth at which ultrafast laser machining can be accurately maintained. We investigate how the depth range may be extended using aberration correction via a liquid crystal spatial light modulator (SLM), in both single point and parallel multi-point fabrication in fused silica. At a moderate numerical aperture (NA = 0.5), high fidelity fabrication with a significant level of parallelisation is demonstrated at the working distance of the objective lens, corresponding to a depth in the glass of 2.4 mm. With a higher numerical aperture (NA = 0.75) objective lens, single point fabrication is demonstrated to a depth of 1 mm utilising the full NA, and deeper with reduced NA, while maintaining high repeatability. We present a complementary theoretical model that enables prediction of the effectiveness of SLM based correction for different aberration magnitudes.

Tunable, high peak power terahertz radiation from optical rectification of a short modulated laser pulse.

A new way of generating high peak power terahertz radiation using ultra-short pulse lasers is demonstrated. The optical pulse from a titanium:sapphire laser system is stretched and modulated using a spatial filtering technique to produce a several picosecond long pulse modulated at the terahertz frequency. A collinear type II phase matched interaction is realized via angle tuning in a gallium selenide crystal. Peak powers of at least 1.5 kW are produced in a 5 mm thick crystal, and tunability is demonstrated between 0.7 and 2.0 THz. Simulations predict that 150 kW of peak power can be produced in a 5 mm thick crystal. The technique also allows for control of the terahertz bandwidth.

Optical trap assisted laser nanostructuring in the near-field of microparticles

Particle based near-field nanostructuring is an excellent possibility to overcome the optical diffraction limit in laser based material processing. In the near-field of microspheres which are irradiated with pulsed laser radiation, it is possible to generate nanoholes with diameters below 100 nm using a laser wavelength of 800 nm. To improve this approach, it is possible to position the microparticles with an optical trap to generate arbitrary structure geometries. In this paper, the authors describe the basic principle of optical trap assisted nanostructuring and present simulational and experimental results demonstrating the potential of this innovative nanoscale optical material processing technology.

Determination of the effective refractive index of nanoparticulate ITO layers

Nanoparticles of transparent conducting oxides, such as indium tin oxide, can be used in printing techniques to generate functional layers for various optoelectronic devices. Since these deposition methods do not create fully consolidated films, the optical properties of such layers are expected to be notably different from those of the bulk material and should be characterized on their own. In this work we present a way to measure the effective refractive index of a particulate ITO layer by refraction of light. The obtained data points are used to identify an accurate layer model for spectroscopic ellipsometry. In this way the complex refractive index of the particle layer is determined in a wide spectral range from ultra violet to near infrared.

Direct measurements of the dynamics of self-guided femtosecond laser filaments in air

Imaging of femtosecond laser filaments is accomplished by utilizing a recently developed diagnostic which is not damaged by the filaments and which greatly reduces the nonlinearities in the detection system. This calibrated detection system allows quantities such as the filament energy and fluence distribution to be determined with greater detail, accuracy, and confidence than was previously possible. The diagnostic is placed on a rail so that filament images can be obtained at a large number of positions along the propagation path. It is found that filaments formed from 450-fs pulses carry higher fluence and propagate farther than filaments formed from 50-fs pulses.