Isak Silander

Fiber-laser-based noise-immune cavity-enhanced optical heterodyne molecular spectrometry instrumentation for Doppler-broadened detection in the 10 12 cm 1 Hz 1∕2 region

A fiber-laser-based noise-immune cavity-enhanced optical heterodyne molecular spectrometry (FL-NICE-OHMS) system for white-noise-limited Doppler-broadened detection down to 5.6 x 10(-12) cm(-1) Hz( ...

Dicke narrowing in the dispersion mode of detection and in noise-immune cavity-enhanced optical heterodyne molecular spectroscopy—theory and experimental verification

Dicke narrowing in both the absorption and dispersion modes of detection have been scrutinized by noise-immune cavity-enhanced optical heterodyne molecular spectroscopy (NICE-OHMS) using an isolate ...

Frequency modulation background signals from fiber-based electro optic modulators are caused by crosstalk

Frequency modulated spectroscopy (FMS) performed by the use of fiber-coupled electro optic modulators (FC-EOMs) is often plagued by background signals that bring in noise and, by their temperature ...

Doppler broadened noise-immune cavity-enhanced optical heterodyne molecular spectrometry: optimum modulation and demodulation conditions, cavity length, and modulation order

Doppler broadened noise-immune cavity-enhanced optical heterodyne molecular spectrometry (Db-NICE-OHMS) has been scrutinized with respect to modulation and demodulation conditions (encompassing the ...

Speed-dependent effects in dispersion mode of detection and in noise-immune cavity-enhanced optical heterodyne molecular spectrometry: experimental demonstration and validation of predicted line shape

Speed-dependent effects (SDEs) in both the absorption and dispersion modes of detection have been detected and scrutinized by the noise-immune cavity-enhanced optical heterodyne molecular spectrome ...

Speed-dependent Voigt dispersion line-shape function: applicable to techniques measuring dispersion signals

An analytical expression for a Voigt dispersion line-shape function that incorporates speed-dependent effects (SDEs) on the collision broadening, applicable to spectroscopic techniques that measure ...

Doppler-broadened mid-infrared noise-immune cavity-enhanced optical heterodyne molecular spectrometry based on an optical parametric oscillator for trace gas detection.

An optical parametric oscillator based Doppler-broadened (Db) noise-immune cavity-enhanced optical heterodyne molecular spectrometry (NICE-OHMS) system suitable for addressing fundamental vibrational transitions in the 3.2-3.9 μm mid-infrared (MIR) region has been realized. An Allan-Werle analysis provides a detection sensitivity of methane of 1.5×10(-9)  cm(-1) with a 20 s integration time, which corresponds to 90 ppt of CH4 if detected at the strongest transition addressed at 40 Torr. This supersedes that of previous Db MIR NICE-OHMS demonstrations and suggests that the technique can be suitable for detection of both the environmentally important (13)CH(4) and CH3D isotopologues. It also opens up for detection of many other molecular species at ppt and sub-ppt concentration levels.

Use of etalon-immune distances to reduce the influence of background signals in frequency-modulation spectroscopy and noise-immune cavity-enhanced optical heterodyne molecular spectroscopy

The detection sensitivity of phase-modulated techniques such as frequency-modulation spectroscopy (FMS) and noise-immune cavity-enhanced optical heterodyne molecular spectroscopy (NICE-OHMS) is oft ...

Fiber-laser-based noise-immune cavity-enhanced optical heterodyne molecular spectrometry incorporating an optical circulator

To reduce the complexity of fiber-laser-based noise-immune cavity-enhanced optical heterodyne molecular spectrometry, a system incorporating a fiber-coupled optical circulator to deflect the cavity-reflected light for laser stabilization has been realized. Detection near the shot-noise limit has been demonstrated for both Doppler-broadened and sub-Doppler signals, yielding a lowest detectable absorption and optical phase shift of 2.2×10(-12)  cm(-1) and 4.0×10(-12)  cm(-1), respectively, both for a 10 s integration time, where the former corresponds to a detection limit of C2H2 of 5 ppt.

Doppler broadened NICE-OHMS beyond the triplet formalism: assessment of optimum modulation index

The dependence of Doppler broadened noise-immune cavity-enhanced optical heterodyne molecular spectrometry (NICE-OHMS) on the modulation index, beta, has been investigated experimentally on C2H2 an ...