J. Amaré

Cosmogenic radionuclide production in NaI(Tl) crystals

The production of long-lived radioactive isotopes in materials due to the exposure to cosmic rays on Earth surface can be an hazard for experiments demanding ultra-low background conditions, typically performed deep underground. Production rates of cosmogenic isotopes in all the materials present in the experimental set-up, as well as the corresponding cosmic rays exposure history, must be both well known in order to assess the relevance of this effect in the achievable sensitivity of a given experiment. Although NaI(Tl) scintillators are being used in experiments aiming at the direct detection of dark matter since the first nineties of the last century, very few data about cosmogenic isotopes production rates have been published up to date. In this work we present data from two 12.5 kg NaI(Tl) detectors, developed in the frame of the ANAIS project, which were installed inside a convenient shielding at the Canfranc Underground Laboratory just after finishing surface exposure to cosmic rays. The very fast start of data taking allowed to identify and quantify isotopes with half-lives of the order of tens of days. Initial activities underground have been measured and then production rates at sea level have been estimated following the history of detectors; values of about a few tens of nuclei per kg and day for Te isotopes and 22Na and of a few hundreds for I isotopes have been found. These are the first direct estimates of production rates of cosmogenic nuclides in NaI crystals. A comparison of the so deduced rates with calculations using typical cosmic neutron flux at sea level and a carefully selected description of excitation functions will be also presented together with an estimate of the corresponding contribution to the background at low and high energies, which can be relevant for experiments aiming at rare events searches.

Status of the ANAIS experiment at Canfranc

Abstract The present status of the ANAIS experiment (Annual Modulation with NaIs) is shown. ANAIS is intended to use more than 100 kg of NaI(Tl) in the Canfranc Underground Laboratory (Spain) searching for seasonal modulation effects in the WIMP signal; in a first stage, a prototype (one single 10.7 kg crystal) has been developed in order to obtain the best conditions regarding the energy threshold and the radioactive background in the low energy region as well as to check the stability of the environmental conditions. The first results corresponding to an exposure of 2069.85 kg day show an average background level of 1.2 counts/(keV kg day) from threshold ( E thr ∼ 4 keV, even using one single photomultiplier) up to 10 keV.

Light yield of undoped sapphire at low temperature under particle excitation

In this letter, we report on the performance of scintillating sapphire bolometers developed in the framework of the ROSEBUD (Rare Objects Search with Bolometers UnDerground) Collaboration devoted to dark matter searches. The simultaneous measurement of heat and light allows the discrimination of the type of particle increasing the sensitivity for these searches. A heat versus light negative correlation for gamma events has been observed. Its interpretation, in a simple framework, allows the estimation of the light yield of undoped sapphire at a temperature of about 20 mK under gamma, alpha, and neutron excitation.

Analysis of the 40K contamination in NaI(Tl) crystals from different providers in the frame of the ANAIS project

NaI(Tl) large crystals are applied in the search for galactic dark matter particles through their elastic scattering off the target nuclei in the detector by measuring the scintillation signal produced. However, energies deposited in the form of nuclear recoils are small, which added to the low efficiency to convert that energy into scintillation, makes that events at or very near the energy threshold, attributed either to radioactive backgrounds or to spurious noise (nonbulk NaI(Tl) scintillation events), can compromise the sensitivity goals of such an experiment. DAMA/LIBRA experiment, using 250 kg NaI(Tl) target, reported first evidence of the presence of an annual modulation in the detection rate compatible with that expected for a dark matter signal just in the region below 6 keVee (electron equivalent energy). In the frame of the ANAIS (Annual modulation with NaI Scintillators) dark matter search project a large and long effort has been carried out in order to understand the origin of events at very low energy in large sodium iodide detectors and develop convenient filters to reject those nonattributable to scintillation in the bulk NaI(Tl) crystal. 40K is probably the most relevant radioactive contaminant in the bulk for NaI(Tl) detectors because of its important contribution to the background at very low energy. ANAIS goal is to achieve levels at or below 20 ppb natural potassium. In this paper we will report on our effort to determine the 40K contamination in several NaI(Tl) crystals, by measuring in coincidence between two (or more) of them. Results obtained for the 40K content of crystals from different providers will be compared and prospects of the ANAIS dark matter search experiment will be briefly reviewed.

Update on the ANAIS experiment. ANAIS-0 prototype results at the new Canfranc Underground Laboratory

ANAIS experiment will look for dark matter annual modulation using NaI(Tl) scintillators at the Canfranc Underground Laboratory (LSC). Highly purified NaI(Tl) crystals are being developed to reach the required sensitivity. In a parallel way, the ANAIS-0 module (made with a low background St Gobain NaI(Tl) crystal) has been taking data at the LSC, testing different configurations: various photomultiplier tubes (PMTs) models with/without light guides. Low background PMTs with light guides and ultra low background PMTs without light guides have shown a similar contribution to the background. A complete simulation of the ANAIS-0 module with shielding in the different configurations tested has been carried out and compared with the experimental data, considering contributions to the background from NaI bulk contaminants, PMTs, light guides, quartz windows and shielding materials. A good understanding of the background above 500 keV can be reported.

Status of the ANAIS Dark Matter Project at the Canfranc Underground Laboratory

The ANAIS experiment aims at the confirmation of the DAMA/LIBRA signal. A detailed analysis of two NaI(Tl) crystals of 12.5 kg each grown by Alpha Spectra will be shown: effective threshold at 1 keVee is at reach thanks to outstanding light collection and robust PMT noise filtering protocols and the measured background is well understood down to 3 keVee, having quantified K, U and Th content and cosmogenic activation in the crystals. A new detector was installed in Canfranc in March 2015 together with the two previous modules and preliminary characterization results will be presented. Finally, the status and expected sensitivity of the full experiment with 112 kg will be reviewed.

Background analysis and status of the ANAIS dark matter project

ANAIS (Annual modulation with NaI Scintillators) is a project aiming to set up at the new facilities of the Canfranc Underground Laboratory (LSC), a large scale NaI(Tl) experiment in order to explore the DAMA/LIBRA annual modulation positive result using the same target and technique. Two 12.5 kg each NaI(Tl) crystals provided by Alpha Spectra took data at the LSC in the ANAIS-25 set-up. The comparison of the background model for the ANAIS-25 prototypes with the experimental results is presented. ANAIS crystal radiopurity goals have been achieved for 232Th and 238U chains, but a 210Pb contamination out-of-equilibrium was identified, whose origin has been studied. The high light collection efficiency obtained with these prototypes allows to anticipate an energy threshold of the order of 1 keVee. A new detector, with improved performances, was received in March 2015 and very preliminary results are shown.

Study of scintillation in natural and synthetic quartz and methacrylate

Abstract Samples from different materials typically used as optical windows or light guides in scintillation detectors were studied in a very low background environment, at the Canfranc Underground Laboratory, searching for scintillation. A positive result can be confirmed for natural quartz: two distinct scintillation components have been identified, not being excited by an external gamma source. Although similar effect has not been observed neither for synthetic quartz nor for methacrylate, a fast light emission excited by intense gamma flux is evidenced for all the samples in our measurements. These results could affect the use of these materials in low energy applications of scintillation detectors requiring low radioactive background conditions, as they entail a source of background.

Cosmogenic production of tritium in dark matter detectors

Abstract The direct detection of dark matter particles requires ultra-low background conditions at energies below a few tens of keV. Radioactive isotopes are produced via cosmogenic activation in detectors and other materials and those isotopes constitute a background source which has to be under control. In particular, tritium is specially relevant due to its decay properties (very low endpoint energy and long half-life) when induced in the detector medium, and because it can be generated in any material as a spallation product. Quantification of cosmogenic production of tritium is not straightforward, neither experimentally nor by calculations. In this work, a method for the calculation of production rates at sea level has been developed and applied to some of the materials typically used as targets in dark matter detectors (germanium, sodium iodide, argon and neon); it is based on a selected description of tritium production cross sections over the entire energy range of cosmic nucleons. Results have been compared to available data in the literature, either based on other calculations or from measurements. The obtained tritium production rates, ranging from a few tens to a few hundreds of nuclei per kg and per day at sea level, point to a significant contribution to the background in dark matter experiments, requiring the application of specific protocols for target material purification, material storing underground and limiting the time the detector is on surface during the building process in order to minimize the exposure to the most dangerous cosmic ray components.

Production and relevance of cosmogenic radionuclides in NaI(Tl) crystals

The cosmogenic production of long-lived radioactive isotopes in materials is an hazard for experiments demanding ultra-low background conditions. Although NaI(Tl) scintillators have been used in this context for a long time, very few activation data were available. We present results from two 12.5 kg NaI(Tl) detectors, developed within the ANAIS project and installed at the Canfranc Underground Laboratory. The prompt data taking starting made possible a reliable quantification of production of some I, Te and Na isotopes with half-lives larger than ten days. Tnitial activities underground were measured and then production rates at sea level were estimated following the history of detectors; a comparison of these rates with calculations using typical cosmic neutron flux at sea level and a selected description of excitation functions was also carried out. After including the contribution from the identified cosmogenic products in the detector background model, we found that the presence of 3H in the crystal ...