J. W. Taylor

Spin waves and revised crystal structure of honeycomb iridate Na2IrO3.

We report inelastic neutron scattering measurements on Na2IrO3, a candidate for the Kitaev spin model on the honeycomb lattice. We observe spin-wave excitations below 5 meV with a dispersion that can be accounted for by including substantial further-neighbor exchanges that stabilize zigzag magnetic order. The onset of long-range magnetic order below T(N)=15.3  K is confirmed via the observation of oscillations in zero-field muon-spin rotation experiments. Combining single-crystal diffraction and density functional calculations we propose a revised crystal structure model with significant departures from the ideal 90° Ir-O-Ir bonds required for dominant Kitaev exchange.

Spin and orbital Ti magnetism at LaMnO3/SrTiO3 interfaces

In systems with strong electron-lattice coupling, such as manganites, orbital degeneracy is lifted, causing a null expectation value of the orbital magnetic moment. Magnetic structure is thus determined by spin-spin superexchange. In titanates, however, with much smaller Jahn-Teller distortions, orbital degeneracy might allow non-zero values of the orbital magnetic moment, and novel forms of ferromagnetic superexchange interaction unique to t(2g) electron systems have been theoretically predicted, although their experimental observation has remained elusive. In this paper, we report a new kind of Ti(3+) ferromagnetism at LaMnO(3)/SrTiO(3) epitaxial interfaces. It results from charge transfer to the empty conduction band of the titanate and has spin and orbital contributions evidencing the role of orbital degeneracy. The possibility of tuning magnetic alignment (ferromagnetic or antiferromagnetic) of Ti and Mn moments by structural parameters is demonstrated. This result will provide important clues for understanding the effects of orbital degeneracy in superexchange coupling.

One-Dimensional Magnetic Fluctuations in the Spin-2 Triangular Lattice α-NaMnO2

The S=2 anisotropic triangular lattice alpha-NaMnO2 is studied by neutron inelastic scattering. Antiferromagnetic order occurs at T< or =45 K with opening of a spin gap. The spectral weight of the magnetic dynamics above the gap (Delta approximately equal to 7.5 meV) has been analyzed by the single-mode approximation. Excellent agreement with the experiment is achieved when a dominant exchange interaction (|J|/k(B) approximately 73 K), along the monoclinic b axis and a sizable easy-axis magnetic anisotropy (|D|/k(B) approximately 3 K) are considered. Despite earlier suggestions for two-dimensional spin interactions, the dynamics illustrate strongly coupled antiferromagnetic S=2 chains and cancellation of the interchain exchange due to the lattice topology. alpha-NaMnO2 therefore represents a model system where the geometric frustration is resolved through the lowering of the dimensionality of the spin interactions.

Positron annihilation study of the Fermi surface of Ni2MnGa

The Fermi surface of the ferromagnetic shape-memory alloy Ni2MnGa has been determined experimentally with two-dimensional angular correlation of electron–positron annihilation radiation. Our results are supported by first principles electronic structure calculations. The measured electron occupancy within the Brillouin zone is consistent with the existence of two nesting features present in the Fermi surfaces calculated in previous studies. The nesting vectors of the calculated Fermi surface match the modulation of the pre-martensitic intermediate structure and that of the martensitic structure.

Temperature dependence of the spin and orbital magnetization density in Sm 0.982 Gd 0.018 Al 2 around the spin-orbital compensation point

Nonresonant ferromagnetic x-ray diffraction has been used to separate the spin and orbital contribution to the magnetization density of the proposed zero-moment ferromagnet

Neutron scattering and muon spin relaxation measurements of the noncentrosymmetric antiferromagnet CeCoGe3

{\mathrm{Sm}}_{0.982}{\mathrm{Gd}}_{0.018}{\mathrm{Al}}_{2}.

Effect of the pseudogap on suppressing high energy inelastic neutron scattering in superconducting YBa2Cu3O6.5

The alignment of the spin and orbital moments relative to the net magnetization shows a sign reversal at 84 K, the compensation temperature. Below this temperature the orbital moment is larger than the spin moment, and vice versa above it. This result implies that the compensation mechanism is driven by the different temperature dependencies of the

Quantized antiferromagnetic spin waves in the molecular Heisenberg ring CsFe8

4f

Bulk electronic structure of optimally doped Ba(Fe1-xCox)2As2

spin and orbital moments. Specific heat data indicate that the system remains ferromagnetically ordered throughout.

Measurement of Magnetic Exchange in Ferromagnet-Superconductor La2/3Ca1/3MnO3/YBa2Cu3O7 Bilayers

The magnetic states of the noncentrosymmetric pressure-induced superconductor CeCoGe3 have been studied with magnetic susceptibility, muon spin relaxation (?SR), single-crystal neutron diffraction, and inelastic neutron scattering (INS). CeCoGe3 exhibits three magnetic phase transitions at TN1=21,TN2=12, and TN3=8K. The presence of long-range magnetic order below TN1 is revealed by the observation of oscillations of the asymmetry in the ?SR spectra between 13 and 20 K and a sharp increase in the muon depolarization rate. Single-crystal neutron-diffraction measurements reveal magnetic Bragg peaks consistent with propagation vectors of k=(0,0,23) between TN1 and TN2,k=(0,0,58) between TN2 and TN3 and k=(0,0,12) below TN3. An increase in intensity of the (110) reflection between TN1 and TN3 also indicates a ferromagnetic component in these phases. These measurements are consistent with an equal moment two-up two-down magnetic structure below TN3 with a magnetic moment of 0.405(5)?B/Ce. Above TN2, the results are consistent with an equal moment two-up one-down structure with a moment of 0.360(6)?B/Ce. INS studies reveal two crystal-electric-field (CEF) excitations at ?19 and ?27meV. From an analysis with a CEF model, the wave functions of the J=52 multiplet are evaluated along with a prediction for the magnitude and direction of the ground-state magnetic moment. Our model correctly predicts that the moments order along the c axis, but the observed magnetic moment of 0.405(5)?B is reduced compared to the predicted moment of 1.0?B. This is ascribed to hybridization between the localized Ce3+ f electrons and the conduction band. This suggests that CeCoGe3 has a degree of hybridization between that of CeRhGe3 and the noncentrosymmetric superconductor CeRhSi3