J. X. Shao

Charge exchange of keV O? ions transmitted through Al2O3 nano-capillaries

The transmission of 10–18 keV O− ions through Al2O3 nano-capillaries has been investigated experimentally. From the angular distribution of the transmitted particles, O0 and O− and O+ ions can be distinguished in the mixed scattered beams. The fractions of the scattered ions increase with both the tilt angle and the incident energy, which indicates strongly that there is dynamical charge exchange in the scattering of negative ions on the insulator surface. Moreover, it is found that the scattered neutrals (O0) are only more or less guided along the capillary axis, which is greatly different from the case of the guiding effect of highly charged ions.

L-shell x-ray yields and production cross-sections of molybdenum induced by low-energy highly charged argon ions*

L-shell x-ray yields of molybdenum bombarded by highly charged Arq+ ions (q = 11-16) are measured. The x-ray production cross-sections are extracted from the yields data. The energy of the incident Ar ions ranges from 200 to 350 keV. After the binding energy correction, experimental data are explained in the framework of binary-encounter-approximation (BEA). The direct ionization is treated in the united atom (UA) limit (Lapicki and Lichten 1985 Phys. Rev. A 31 1354), not in the separate atom (SA) limit. The calculation results of BEA (Gacia and Fortner 1973 Rev. Mod. Phys. 45 111) are much lower than the experimental results, while the results of binding energy modified BEA are basically in agreement with the experimental results.

Transmission of 18 keV negative ions Cl− through nanocapillariesin Al2O3 membrane

We investigate the angular distribution of the transmitted 18 keV negative ions Cl− through Al2O3 nanocapillaries of 50 nm in diameter and 10 μm in length. Elastic scattering ions and inelastic scattering ions are obtained simultaneously. The experimental result is partially consistent with the guiding effect. We can qualitatively explain our experimental result through a dynamic process.

THRESHOLD KINETIC ENERGY FOR GOLD X-RAY EMISSION INDUCED BY HIGHLY CHARGED IONS

The X-rays induced in the interaction of highly charged Argon ions with gold surface were investigated. We had altered the projectile kinetic energy from 150keV to about 400keV. The results show that, there is a threshold projectile kinetic energy for this excitation. Combining the colliding theory of classic electrodynamics with the concept of quantized orbits, we crudely give this threshold kinetic energy.

Dynamics of slow electrons transmitting through straight glass capillary and tapered glass capillary

It has been found that the transmission rate of the electrons through insulating capillaries as a function of time/incident charge is not the same as that of the ions. The question arises that by using the electrons, if the negative charge patches can be formed to facilitate the transmission of the following electrons, thereby substantiating that the so-called guiding effect works also for electrons. This study aims to observe the time evolutions of the transmission of electrons through a straight glass tube and a tapered glass capillary. This will reveal the details of how and (or) if the negative charge patches can be formed when the electrons transport through them. In this work, a set of MCP/phosphor two-dimensional detection system based on Labview platform is developed to obtain the time evolution of the angular distribution of the transmitted electrons. The pulsed electron beams are obtained to test our detection system. The time evolution of the angular profile of 1.5 keV electrons transmitting through the glass tube/capillary is observed. The transmitted electrons are observed on the detector for a very short time and disappear for a time and then appear again for both the glass tube and tapered glass capillary, leading to an oscillation. The positive charge patches are formed in the insulating glass tube and tapered glass capillary since the secondary electron emission coefficient for the incident energy is larger than 1. It is due to the fact that fast discharge of the deposited charge leads to the increase of the transmission rate, while the fast blocking of the incident electrons due to the deposited positive charge leads to the decrease of the transmission rate. The geometrical configuration of the taper glass capillary tends to make the secondary electrons deposited at the exit part to form the negative patches that facilitate the transmission of electrons. This suggests that if the stable transmission needs to be reached for producing the electron micro-beam by using tapered glass capillaries, the steps must be taken to have the proper grounding and shielding of the glass capillaries and tubes. Our results show a difference in transmission through the insulating capillary between electrons and highly charged ions.

Scaling law of single ion–atom impact ionization cross sections of noble gases from He to Xe at strong perturbative energies*

We extend our previous work of a classical over-barrier ionization (COBI) model to calculate the single ionization cross sections of noble gases ranging from He to Xe at strong perturbative energies. The calculation results are in good agreement with extensive experimental data. The scaling law of single ion-atom impact ionization cross sections of noble gases on projectile charge q and energy E, also on target ionization energy I is drawn from the model.

Multiple ionization of atoms and molecules impacted by very high-q fast projectiles in the strong coupling regime (q/v > 1)

In this paper, we present a simple theoretical approach to calculate the multiple ionization of big atoms and molecules induced by very high-q fast projectiles in a strong coupling regime (q/v > 1). The results obtained from this approach are in excellent agreement with the available experimental data. A probable scenario of molecular multiple ionization by fast and very high-q projectiles is discussed. The very small computational time required here and the good agreement with the existing experimental data make it a good candidate for studying the multiple ionization of complex molecules under high linear energy transfers.

Sequential over-barrier ionization of multi-electron atoms in the tens-to-hundreds keV/u energy range

Our previous work on the classical over-barrier ionization model for helium double ionization is extended to the complex multi-electron system of Ne. The total and q-fold ionization cross sections are calculated at energies ranging from a few tens to several hundred keV/u. The calculation results are in good agreement with the experimental data, and the energy dependence of the cross sections suggests that the multi-ionization of a strong perturbated complex atom is probably the sequential over-barrier ionization process.

Experimental study of cross-section ratios in the collisions of Cq+ and Oq+ (q=1-4) on atomic helium in strong-interaction region

We have measured the cross-section ratios of helium induced by Cq+ and Oq+ (q = 1?4) in an energy range from 20 keV/amu to 500 keV/amu, and obtained the two-dimensional spectra by employing the coincidence method combined with the MPA-3 data acquisition system. Hence, we obtain the ratios of total single-ionization cross-sections (SI, SC, SLSI, and DLSI), total double-ionization cross-sections (DI, DC, TI, SLDI, and DLDI) and cross-sections of every process (SI, SC, SLSI, DLSI, DI, DC, TI, SLDI, and DLDI), which induce the single-ionization and double-ionization, to the total cross sections respectively. The competitive relations between the reaction-channels and the experimental data law of each reaction-channel are revealed explicitly, and the qualitative explanations involved in those results are also presented accordingly.

X-RAY EMISSION FROM THE METASTABLE COMPONENTS OF SLOW Ar16+ BEAM ON METALLIC SURFACES

K-shell X-ray emission was observed in the neutralization process of Ar16+ interacting with beryllium and molybdenum at slow speed (less than Bohr velocity). The K-shell X-ray emission came from the metastable component of Ar16+ beam with the configuration (1s2s) produced from electron cyclotron resonance ion source. The intensity ratio of Kβ X-ray emission to Kα X-ray emission (IKβ/IKα) in the neutralization process decreased when the kinetic energy of the projectile increased. This is closely related to the flight time the projectiles spend above the surface, which is dominated by both the work function of the metal and the normal velocity component of the incident ions to the surface according to the classical over-barrier model. As the relation between IKβ/IKα and the above-flight time shows, the longer time above the surface the larger ratio due to the above-surface contribution. Furthermore, the smaller work function leads to the smaller contribution from the above surface.