Jacques Dubeau

A neutron spectrometer using nested moderators

The design, simulation results and measurements of a new neutron energy spectrometer are presented. The device, which may be called NNS, for Nested Neutron Spectrometer, works under the same principles as a Bonner Sphere Spectrometer (BSS) System, i.e. whereby a thermal neutron detector is surrounded by a polyethylene moderator. However, the moderator is cylindrical in shape. The different thicknesses of moderator are created by inserting one cylinder into another, much like nested Russian dolls. This design results in a much lighter instrument that is also easier to use in the field. Simulations and measurements show that, despite its shape, the device can be made to offer a near angular isotropic response to neutrons and that unfolded neutron spectra are in agreement with those obtained with a more traditional BSS.

Characterization of neutron fields from bare and heavy water moderated 252Cf spontaneous fission source using Bonner Sphere Spectrometer

In this work a calibrated Bonner Sphere Spectrometer (BSS), together with ISO shadow cones, was used to quantify the total and scattered components of bare and heavy water moderated (252)Cf neutron fields. All measurements were performed with a BSS that was calibrated at the National Physical Laboratory (NPL), Teddington, UK, which is a global primary standard laboratory and world-leading facility for neutron metrology and neutron instruments calibration. The fields were characterized for source-spectrometer distances of 80, 100, 150 and 200cm; and at heights of 103 and 200cm from the facility floor. As expected, the scattered contribution was greatest at the farthest distance from the source and closer to the floor. Hence, at a distance of 200cm and a height of 103cm, the scatter added to the direct field up to 162% of the total neutron fluence and up to 61% of the ambient dose equivalent, while at the same distance and height of 200cm above the floor, these values were up to 146% and 52%, respectively. In the case of heavy water moderated (252)Cf neutron fields, a shadow cone subtraction technique could not be implemented, however Monte Carlo simulations were utilized in order to differentiate between the direct and scatter components of the neutron fields. In this case, at a source-detector distance of 200cm and a height of 103cm, the scatter added to the direct field up to 148% of the total neutron fluence and up to 45% of the ambient dose equivalent, while at the same distance and a height of 200cm above the floor, these values were up to 134% and 42%, respectively.

Correction and verification of AECL Bonner Sphere response matrix based on mono-energetic neutron calibration performed at NPL

The AECL Bonner Sphere Spectrometer (BSS) was taken to National Physical Laboratory (NPL) for calibration in mono-energetic neutron fields and bare (252)Cf neutron fields. The mono-energetic radiations were performed using ISO-8529 prescribed neutron energies: 0.071, 0.144, 0.565, 1.2, 5 and 17 MeV. A central SP9 proportional counter was also evaluated at the NPL thermal neutron calibration facility in order to assess an effective pressure of (3)He inside the counter, i.e. number density of (3)He atoms. Based on these measurements and methods outlined by Thomas and Soochak, a new BSS response matrix was generated. The response matrix is then verified by unfolding spectra corresponding to various neutron fields. Those are NPL bare (252)Cf source, National Institute of Standards and Technology bare and heavy water moderated (252)Cf source and (241)AmBe calibration source located at National Research Council. A good agreement was observed with expected neutron fluence rates, as well as derived dosimetric quantities, such as International Commission on Radiological Protection-74 ambient dose equivalent.

Neutron spectrometry and dosimetry study at two research nuclear reactors using Bonner sphere spectrometer (BSS), rotational spectrometer (ROSPEC) and cylindrical nested neutron spectrometer (NNS)

Neutron spectrometry and subsequent dosimetry measurements were undertaken at the McMaster Nuclear Reactor (MNR) and AECL Chalk River National Research Universal (NRU) Reactor. The instruments used were a Bonner sphere spectrometer (BSS), a cylindrical nested neutron spectrometer (NNS) and a commercially available rotational proton recoil spectrometer. The purposes of these measurements were to: (1) compare the results obtained by three different neutron measuring instruments and (2) quantify neutron fields of interest. The results showed vastly different neutron spectral shapes for the two different reactors. This is not surprising, considering the type of the reactors and the locations where the measurements were performed. MNR is a heavily shielded light water moderated reactor, while NRU is a heavy water moderated reactor. The measurements at MNR were taken at the base of the reactor pool, where a large amount of water and concrete shielding is present, while measurements at NRU were taken at the top of the reactor (TOR) plate, where there is only heavy water and steel between the reactor core and the measuring instrument. As a result, a large component of the thermal neutron fluence was measured at MNR, while a negligible amount of thermal neutrons was measured at NRU. The neutron ambient dose rates at NRU TOR were measured to be between 0.03 and 0.06 mSv h⁻¹, while at MNR, these values were between 0.07 and 2.8 mSv h⁻¹ inside the beam port and <0.2 mSv h⁻¹ between two operating beam ports. The conservative uncertainty of these values is 15 %. The conservative uncertainty of the measured integral neutron fluence is 5 %. It was also found that BSS over-responded slightly due to a non-calibrated response matrix.

Detection of bremsstrahlung radiation of 90Sr–90Y for emergency lung counting

This study explores the possibility of developing a field-deployable (90)Sr detector for rapid lung counting in emergency situations. The detection of beta-emitters (90)Sr and its daughter (90)Y inside the human lung via bremsstrahlung radiation was performed using a 3″ × 3″ NaI(Tl) crystal detector and a polyethylene-encapsulated source to emulate human lung tissue. The simulation results show that this method is a viable technique for detecting (90)Sr with a minimum detectable activity (MDA) of 1.07 × 10(4) Bq, using a realistic dual-shielded detector system in a 0.25-µGy h(-1) background field for a 100-s scan. The MDA is sufficiently sensitive to meet the requirement for emergency lung counting of Type S (90)Sr intake. The experimental data were verified using Monte Carlo calculations, including an estimate for internal bremsstrahlung, and an optimisation of the detector geometry was performed. Optimisations in background reduction techniques and in the electronic acquisition systems are suggested.

Measurements of neutron energy spectra from 7Li(p,n)7Be reaction with Bonner sphere spectrometer, Nested Neutron Spectrometer and ROSPEC

Neutron spectrometry measurements were carried out at the McMaster Accelerator Laboratory (MAL), which is equipped with a 3-MV Van de Graaff-type accelerator. Protons were accelerated onto a thick natural lithium target inducing the (7)Li(p,n)(7)Be threshold reaction. Depending on the proton energy, slightly different poly-energetic neutron fields were produced. Neutron spectra were measured at two incident proton energies: 2.15 and 2.24 MeV, which produced poly-energetic neutrons with maximum kinetic energies of 401 and 511 keV, respectively. Measurements were performed at a distance of 1.5 m from the target in the forward direction with three different instruments: Bonner sphere spectrometer, Nested Neutron Spectrometer and ROtational proton recoil SPECtrometer.

A COMPARISON OF BETA SKIN DOSES CALCULATED WITH VARSKIN 5.35.3 AND MCNP5

The computer code VARSKIN, version 5.3, is widely used to calculate superficial dose caused by the routine handling of radioactive substances or in skin contamination incidents. It allows a variety of source configurations, points, volume, surface and syringe-like (cylindrical) and a variety of exposure situations such as direct skin contact or exposure through clothing. However, there is a need for more benchmarking data of VARSKIN, especially for beta particles, with complex irradiation geometries. Dose calculations using MCNP5 and VARSKIN 5.3 for a variety of mass-less point beta-emitting sources were performed. Both programs gave comparable results that are in good agreement with published dose rate conversion factors for sources on contact with the skin or with fabric. However, important differences appear, with VARSKIN 5.3 values as much as 40% below the Monte Carlo results, when an air gap of a few mm is introduced between the fabric and skin.

Measurement of the neutron field characteristics inside and outside the vault of a 70 MeV cyclotron

Neutron fields are created inside and outside the vault as byproducts of radioisotope production of the 70 MeV cyclotron at Zevacor Molecular Inc. Neutron energy distribution measurements were obtained for a 10 μΑ accelerator proton beam incident on a Rb/Ga target using the Nested Neutron Spectrometer. The neutron fluence rate at a 30 cm diameter conduit outside of the vault reached 3.95×10⁴ cm⁻² s⁻¹ and was measured to be 7.68×10⁷ cm⁻² s⁻¹ inside the vault at a distance of 1 m from the target. Neutron output is expected to be approximately 20 times greater during routine operational conditions (200 μΑ). Inside the vault, the spectrum showed features similar to theoretical models and may provide a useful environment to test space-bound electronics.

Poster - 25: Neutron Spectral Measurements around a Scanning Proton Beam

We describe the measurements of neutron spectra that we undertook around a scanning proton beam at the Skandion proton therapy clinic in Uppsala, Sweden. Measurements were undertaken using an extended energy range Nested Neutron Spectrometer (NNS, Detec Inc., Gatineau, QC) operated in pulsed and current mode. Spectra were measured as a function of location in the treatment room and for various Bragg peak depths. Our preliminary unfolded data clearly show the direct, evaporation and thermal neutron peaks and we can show the effect on the neutron spectrum of a water phantom in the primary proton beam.

A field portable neutron spectrometer based on the Bonner Sphere Principles

The Bonner Sphere Spectrometer (BSS) has been used since 1960 for the determination of neutron energy spectra ranging from 25 meV to 20 MeV. Although some researchers have taken fun sets of Bonner spheres inside nuclear power plants for field measurements, the volume and mass of the whole device have usually limited its use to laboratories and to calibration and reference facilities. The instrument presented here operates under the same principles of the Bonner spheres, except that different amounts of moderator around a thermal neutron detector are configured by adding or removing cylindrical shells. For this reason it is called the Nested Neutron Spectrometer (NNS). Thus, only the mass and volume equivalent to a single Bonner sphere need to be carried in the field. The reconfiguration of the moderator is very quick, leading to a reduced setup time. The instrument can then easily be used in the workplace and the measured spectra allow the calculation of the ambient dose equivalent rate, without the inherent inaccuracies of REM meters. The focus of this paper is the design principles of the NNS, laboratory test results and field measurements. Measurements were obtained using radionuclide neutron sources, mono-energetic neutrons from accelerators and from neutrons around the containment of a nuclear power reactor. Results are very similar for the NNS and BSS, with the former being much easier to use in the field.