Jan Hansman

Airborne radioiodine in northern Serbia from Fukushima

The results obtained with the monitoring system set up to assess the impact of the Fukushima accident on the environment of Vojvodina (Northern Province of Serbia) are presented and discussed. Aerosol, rain, fresh milk and spinach samples were collected daily in the weeks following the accident. In the aerosol samples, (131)I activity concentrations of several mBq m(-3) were measured, while in rain, milk and spinach samples, (131)I levels had values in a range of (0.3-1.7) Bq kg(-1). These are the first results on the impact of the Fukushima accident on the Pannonian basin region. Our results are compared with the reported values from other parts of the world.

NATURAL RADIOACTIVITY IN RAW MATERIALS USED IN BUILDING INDUSTRY IN SERBIA

Natural radioactivity is responsible for most of the total radiation dose received by human population. Geological materials used in building industry usually become contaminated with naturally occurring radioactive materials. They are used as mixtures in building industry (kaolin, zircon, frit, feldspar) or mechanically processed and used for covering floors and walls of the rooms (granite). In this paper, activity concentrations of 226Ra, 232Th and 40K in 6 kaolin, 11 zircon, 18 granite, 3 marble, 6 sand, 4 perlite, 4 feldspar, 5 korund and 1 frit samples imported in Serbia were determined by gamma-ray spectrometry. Activity concentration index, dose rate and annual effective dose were calculated for each of the investigated samples. Measurement of an external gamma dose rate by using a commonly available radiation survey meter can give some indication of the need for further investigations. The absorbed dose rate and annual effective doses for workers in the ceramic industry “Keramika Kanjiza Plus” in Serbia working with granite are determined.

Efficiency study of a big volume well type NaI(Tl) detector by point and voluminous sources and Monte-Carlo simulation.

The activity of environmental samples is usually measured by high resolution HPGe gamma spectrometers. In this work a set-up with a 9in.x9in. NaI well-detector with 3in. thickness and a 3in.×3in. plug detector in a 15-cm-thick lead shielding is considered as an alternative (Hansman, 2014). In spite of its much poorer resolution, it requires shorter measurement times and may possibly give better detection limits. In order to determine the U-238, Th-232, and K-40 content in the samples by this NaI(Tl) detector, the corresponding photopeak efficiencies must be known. These efficiencies can be found for certain source matrix and geometry by Geant4 simulation. We found discrepancy between simulated and experimental efficiencies of 5-50%, which can be mainly due to effects of light collection within the detector volume, an effect which was not taken into account by simulations. The influence of random coincidence summing on detection efficiency for radionuclide activities in the range 130-4000Bq, was negligible. This paper describes also, how the efficiency in the detector depends on the position of the radioactive point source. To avoid large dead time, relatively weak Mn-54, Co-60 and Na-22 point sources of a few kBq were used. Results for single gamma lines and also for coincidence summing gamma lines are presented.

Correlation of unsupported 210Pb activity in soil and moss

The activities of unsupported (210)Pb, a naturally occurring radionuclide, were measured in samples of soil and terrestrial mosses collected in Serbia. Considering that clay particles in soil have a high affinity for Pb adsorption, and that mosses usually capture aerosol particles to obtain necessary nutrients, measurable amounts of airborne (210)Pb, the daughter of (222)Rn, can be registered in both soil and mosses. The objective of the present study was to determine if it is possible to compare the activity of unsupported (210)Pb in soil and moss collected at the same sampling site, and to establish if a correlation exists between these measured values.

Radioactivity in the indoor building environment in Serbia

Measurement of activity concentrations of radionuclides in building materials and radon in indoor space is important in the assessment of population exposures, as most individuals spend 80 % of their time indoors. This paper presents the results of activity concentration measurements of: radon emanated from the soil, radionuclides (226)Ra, (232)Th and (40)K in the soil, indoor radon in the city of Novi Sad (the capital city of Vojvodina) using charcoal canisters and indoor radon in the Vojvodina region using alpha-track detectors and the radioactivity of some building materials. Influences of floor level, space under the rooms, boarding, and the heating system on indoor radon accumulation in the Vojvodina province, situated in the northern part of Serbia, are also presented in this paper. The total effective dose and the activity concentration index are calculated applying the dose criteria recommended by the European Union for building materials.

Establishment of a method for 222Rn determination in water by low-level liquid scintillation counter

A procedure for the determination of (222)Rn in environmental water samples using liquid scintillation counting (LSC) was performed. The (226)Ra content in the water was determined by gamma-ray spectroscopy. An application of this procedure to drinking water collected from a public drinking fountain in Vojvodina (Serbia) is presented, including calculations of the annual effective dose for ingestion and inhalation for adults.

Isotope analyses of the lake sediments in the Plitvice Lakes, Croatia

The analyses of radioactive isotopes 14C, 137Cs and 210Pb, and stable isotope 13C were performed in the sediment cores, top 40 cm, taken in 2011 from karst lakes Prošće and Kozjak in the Plitvice Lakes National Park, central Croatia. Frozen sediment cores were cut into 1 cm thick layers and dried. 14C activity in both carbonate and organic fractions was measured using accelerator mass spectrometry technique with graphite synthesis. 137Cs, 210Pb, 214Pb and 214Bi were measured by low level gamma spectrometry method on ORTECHPGe detector with the efficiency of 32%.Distribution of 14C activity from both lakes showed increase of the 14C activity in the top 10–12 cm in both carbonate and organic fractions as a response to thermonuclear bomb-produced 14C in the atmosphere in the sixties of the 20th century. Anthropogenically produced 137Cs was also observed in sediment profiles. Sedimentation rates for both lake sediments were estimated based on the unsupported 210Pb activity.Different 14C activity of the carbonate fraction (63–80 pMC, percent of modern carbon) and organic fraction (82–93 pMC) is the result of geochemical and biological processes of the sediment precipitation in the lake waters. This is also confirmed by the δ13C values of both fractions. Carbon isotope composition, a14C and δ13C, was compared with the lake sediments from the same lakes collected in 1989 and 2003.

Influence of broadleaf forest vegetation on atmospheric deposition of airborne radionuclides

The activities of airborne radionuclides 7Be and unsupported 210Pb (210Pbus) were measured in moss samples taken from 17 different locations. The objective was to estimate the influence of the broadleaf forest vegetation on atmospheric deposition of airborne radionuclides attached to aerosols. Two moss samples were collected at each location: within the forest stand (inside the area of the tree canopy projection) and within forest openings (outside the area of the tree canopy projection). Samples were taken in the spring season, before the leaves of trees came forth and in the autumn season, right before fall defoliation. A measurement indicates an absence of variation in 210Pbus concentration, however spring/autumn ratios of 7Be concentrations in mosses showed the expected seasonal difference in 7Be deposition. It was also noted that atmospheric deposition of 7Be at the forest openings was about two times higher than deposition in the forest. Using very simplified models, these measurements can be used to get estimation at how long 7Be and aerosols can reside on the leaves before precipitation eventually wash it to the ground mosses. It was estimated that the mean residence time of aerosols in the leaves was up to 50 days.

Radioactivity in fertilizers and radiological impact

The contents of natural radionuclides (226Ra, 232Th and 40K) in 33 fertilizers and 50 soil samples from Vojvodina region, Serbia, were measured by low level gamma spectrometry. The obtained results showed that the averages of radiation hazard parameters for the fertilizers are higher than acceptable level for radium equivalent activity (Raeq), representative level index (Iγ), external hazard index (Hex) and absorbed dose rate (D) [1]. Based on the measured values of the activity concentration of radionuclides in soils, the activity concentrations of radionuclides for most commonly grown crops in Vojvodina were calculated.

RADIOLOGICAL IMPACTS ASSESSMENT FOR WORKERS IN CERAMIC INDUSTRY IN SERBIA

Studies have been carried out to determine the natural radioactivity in some materials used in ceramic industry (zircon, zirkosil, Zircobit MO/S, zircon silicate, zirklonil frit, hematite, bentonite, wollastonite, raw kaolin, kaolinized granite, sileks ball, feldspar, pigment, white base serigraphic, engobe) and their associated radiation hazard. The external hazard index, Hex, values, radium equivalent activity, Raeq, total absorbed dose rates, D and annual effective dose, De were derived for all measured materials and compared with the recommended values to assess the external radiation hazards to workers who worked in ceramic industries in Serbia.