Jean-Luc Pelouard

Shaping the spatial and spectral emissivity at the diffraction limit

Metasurfaces have attracted a growing interest for their ability to artificially tailor an electromagnetic response on various spectral ranges. In particular, thermal sources with unprecedented abilities, such as directionality or monochromaticity, have been achieved. However, these metasurfaces exhibit homogeneous optical properties whereas the spatial modulation of the emissivity up to the wavelength scale is at the crux of the design of original emitters. In this letter, we study an inhomogeneous metasurface made of a nonperiodic set of optical nano-antennas that spatially and spectrally control the emitted light up to the diffraction limit. Each antenna acts as an independent deep subwavelength emitter for given polarization and wavelength. Their juxtaposition at the subwavelength scale encodes far field multispectral and polarized images. This opens up promising breakthroughs for applications such as optical storage, anti-counterfeit devices, and multispectral emitters for biochemical sensing.

Guided-mode resonator for thin InGaAs P-i-N short-wave infrared photo-diode

We investigate a resonant photodiode transferred onto a gold mirror. This comprises a backside dielectric subwavelength periodic structure and an absorbing region as thin as 90 nm. Electro-optical characterizations of individual pixels featuring focal-plane array-compatible geometries are fully explained by electro-magnetic simulations. In particular, we observe a near perfect collection of the photo-carriers and external quantum efficiency of up to 71% around 1.55 μm.

Water-Dispersed Hydrophobic Au Nanocrystal Assemblies with a Plasmon Fingerprint

Hydrophobic Au nanocrystal assemblies (both ordered and amorphous) were dispersed in aqueous solution via the assistance of lipid vesicles. The intertwine between vesicles and Au assemblies was made possible through a careful selection of the length of alkyl chains on Au nanocrystals. Extinction spectra of Au assemblies showed two peaks that were assigned to a scattering mode that red-shifted with increasing the assembly size and an absorption mode associated with localized surface plasmon that was independent of their size. This plasmon fingerprint could be used as a probe for investigating the optical properties of such assemblies. Our water-soluble assemblies enable exploring a variety of potential applications including solar energy and biomedicine.

Integration of nanostructured planar diffractive lenses dedicated to near infrared detection for CMOS image sensors.

This paper deals with the integration of metallic and dielectric nanostructured planar lenses into a pixel from a silicon based CMOS image sensor, for a monochromatic application at 1.064 μm. The first is a Plasmonic Lens, based on the phase delay through nanoslits, which has been found to be hardly compatible with current CMOS technology and exhibits a notable metallic absorption. The second is a dielectric Phase-Fresnel Lens integrated at the top of a pixel, it exhibits an Optical Efficiency (OE) improved by a few percent and an angle of view of 50°. The third one is a metallic diffractive lens integrated inside a pixel, which shows a better OE and an angle of view of 24°. The last two lenses exhibit a compatibility with a spectral band close to 1.064 μm.

Investigating the optical properties of nanogap optical antennas

We investigate the optical properties of nanogap MIM nanoantennas with a 2.1 nm thick gap. These plasmonic nanoantennas consist of a gold film, an insulating layer deposited by Atomic Layer Deposition, and a periodically structured gold layer. MIM nanoantennas are characterized by a tunable spectral response and a high field confinement within the nanogap. Nanometric gaps enable high coupling between the plasmons of the top and bottom metal surfaces. We demonstrated an excellent agreement between optical measurements and classical electromagnetic simulations. In particular, we observed a fluctuation in the gap thickness of 0.2 nm.

Nanostructured diode for infrared photodetection through non degenerate two-photon absorption

Two-photon absorption (TPA) is a third order non-linear process that relies on the quasi-simultaneous absorption of two photons. Therefore, it has been proved to be an interesting tool to measure ultra-fast correlations1 or to design all-optical switches.2 Yet, due to the intrinsically low efficiency of the non-linear processes, these applications rest upon high peak power light sources such as femtosecond and picosecond pulsed laser. However TPA has also been noticed as an appealing new scheme for quantum infrared detection.3, 4 Indeed, typical quantum detection of IR radiation is based on small gap semiconductors that need to be cooled down to cryogenic temperature to achieve sufficient detectivity. TPA enables the absorption of IR photons by wide gap semiconductors when pump photons are provided to complete optical transitions across the gap. Still, the low efficiency of TPA represents a difficulty to detect usual infrared photon fluxes. To tackle this issue, we combined three strategies to improve the detection efficiency. First, it has been proved theoretically and experimentally that using different pump and signal photon energies which is known as non degenerate TPA (NDTPA) help increasing the TPA efficiency by several orders of magnitude.5 Thus we decided to work with different pump and signal wavelength. Secondly, since TPA is a local quasi-instantaneous process, both pump and signal photons must be temporarily and spatially co-localized inside the active medium. We made sure to maximize the overlap of the fields inside our device. Finally, it is well known that TPA has a quadratic dependence with the signal electric fields modulus, so we designed a specific nanostructure to enhance the signal field inside the active medium of the detector.

Limited-size guided-mode resonance filters under focused beams

We investigate the impact of focused beams on metal-dielectric guided-mode-resonance filters. Under a planewave illumination, these filters show a resonant transmission at an easily tunable wavelength and a good angular acceptance. Although guided-mode resonance is involved, calculations show that under a focused beam the lateral extension of the electromagnetic field inside the waveguide is limited to the width of the beam. We investigate evolution of this lateral extension and the resonant transmission with the size of the beam, as well as the impact of a tilted beam. Guided-mode-resonance filtering under a focused beam is illustrated through the example of a Cassegrain microscope lens. A process for the fabrication of simple metal-dielectric filters is also presented.

Nanostructured diode for infrared photodetection through nondegenerate two-photon absorption

We investigate infrared detection at room temperature using non-degenerate two-photon absorption in a nanostructured indium phosphide photodiode. We designed the detector structure to achieve a good nonlinear absorption by combining three major ideas: first, we use the non-degenerate two-photon absorption process, which is known to be more efficient than the previously used degenerate two-photon absorption. Second, we ensured a correct spatial overlap of our pump field with our signal field. Third, we optimized the nanostructuration to increase the signal field amplitude locally within the active medium of the device. The resulting device consists of a PIN junction embedded between a back-reflecting gold mirror and a top grating. We experimentally characterized our diode with regard to reflectivity and two-photon absorption generated photocurrent for a continuous-wave pump and a nanosecond pulsed signal of around 3.39 μm. Owing to the nanostructuration, the generated photocurrent shows a gain of 24 with respect to the bulk response of InP.We investigate infrared detection at room temperature using non-degenerate two-photon absorption in a nanostructured indium phosphide photodiode. We designed the detector structure to achieve a good nonlinear absorption by combining three major ideas: first, we use the non-degenerate two-photon absorption process, which is known to be more efficient than the previously used degenerate two-photon absorption. Second, we ensured a correct spatial overlap of our pump field with our signal field. Third, we optimized the nanostructuration to increase the signal field amplitude locally within the active medium of the device. The resulting device consists of a PIN junction embedded between a back-reflecting gold mirror and a top grating. We experimentally characterized our diode with regard to reflectivity and two-photon absorption generated photocurrent for a continuous-wave pump and a nanosecond pulsed signal of around 3.39 μm. Owing to the nanostructuration, the generated photocurrent shows a gain of 24 with r...

Two-mode model for metal-dielectric guided-mode resonance filters

Symmetric metal-dielectric guided-mode resonators (GMR) can operate as infrared band-pass filters, thanks to high-transmission resonant peaks and good rejection ratio. Starting from matrix formalism, we show that the behavior of the system can be described by a two-mode model. This model reduces to a scalar formula and the GMR is described as the combination of two independent Fabry-Perot resonators. The formalism has then been applied to the case of asymmetric GMR, in order to restore the properties of the symmetric system. This result allows designing GMR-on-substrate as efficient as free-standing systems, the same high transmission maximum value and high quality factor being conserved.

Optical Nanoantennas For High-Efficient Ultra-Thin Solar Cells

We propose new concepts for light trapping in ultra-thin solar cells. It is shown that optical nanoantennas can lead to broadband absorption in 30nnm-thick GaAs solar cells, with 14.5% energy conversion efficiency.