Jeffrey K. Eliason

Non-Contact Measurement of Thermal Diffusivity in Ion-Implanted Nuclear Materials

Knowledge of mechanical and physical property evolution due to irradiation damage is essential for the development of future fission and fusion reactors. Ion-irradiation provides an excellent proxy for studying irradiation damage, allowing high damage doses without sample activation. Limited ion-penetration-depth means that only few-micron-thick damaged layers are produced. Substantial effort has been devoted to probing the mechanical properties of these thin implanted layers. Yet, whilst key to reactor design, their thermal transport properties remain largely unexplored due to a lack of suitable measurement techniques. Here we demonstrate non-contact thermal diffusivity measurements in ion-implanted tungsten for nuclear fusion armour. Alloying with transmutation elements and the interaction of retained gas with implantation-induced defects both lead to dramatic reductions in thermal diffusivity. These changes are well captured by our modelling approaches. Our observations have important implications for the design of future fusion power plants.

Thermal transport in suspended silicon membranes measured by laser-induced transient gratings

Studying thermal transport at the nanoscale poses formidable experimental challenges due both to the physics of the measurement process and to the issues of accuracy and reproducibility. The laser-induced transient thermal grating (TTG) technique permits non-contact measurements on nanostructured samples without a need for metal heaters or any other extraneous structures, offering the advantage of inherently high absolute accuracy. We present a review of recent studies of thermal transport in nanoscale silicon membranes using the TTG technique. An overview of the methodology, including an analysis of measurements errors, is followed by a discussion of new findings obtained from measurements on both “solid” and nanopatterned membranes. The most important results have been a direct observation of non-diffusive phonon-mediated transport at room temperature and measurements of thickness-dependent thermal conductivity of suspended membranes across a wide thickness range, showing good agreement with first-princ...

Non-diffusive thermal transport in GaAs at micron length scales

We use a transient thermal grating technique in reflection geometry to measure the effective thermal diffusivity in GaAs as a function of heat transfer distance at three temperatures. Utilizing heterodyne detection, we isolate the “amplitude” grating contribution of the transient grating signal, which encodes the thermal transport dynamics. As the thermal grating period decreases, and thus the heat-transfer distance, we observe a reduction in the effective thermal diffusivity, indicating a departure from diffusive behavior. Non-diffusive behavior is observed at room temperature, as well as low temperature (180 K) and high temperature (425 K). At the shortest thermal grating period measured corresponding to a heat transfer distance of approximately 1 μm, the effective diffusivity drops to a value roughly 50% of the bulk thermal diffusivity. These measurements show the utility of the reflection transient thermal grating technique to measure thermal transport properties of opaque materials.

Increase in elastic anisotropy of single crystal tungsten upon He-ion implantation measured with laser-generated surface acoustic waves

We report the experimental observation of an increase in the elastic anisotropy of tungsten upon He-ion implantation, probed optically using transient grating spectroscopy. Surface acoustic wave (SAW) velocity measurements were performed on a (110) oriented tungsten single crystal as a function of in-plane propagation direction for unimplanted and implanted samples. Our measurements allow us to finely resolve the remarkably small elastic anisotropy of the samples investigated. SAW velocity calculations are used to interpret the experimental data and to extract the Zener anisotropy parameter η and the elastic constant C44. Upon ion implantation, we observe an increase in the quantity (η−1) by a factor of 2.6. The surprising increase in elastic anisotropy agrees with previous theoretical predictions based on ab initio calculations of the effect of self-interstitial atoms and He-filled vacancy defects on the elastic properties of tungsten.

Lifetime of high-order thickness resonances of thin silicon membranes

Femtosecond laser pulses are used to excite and probe high-order longitudinal thickness resonances at a frequency of ∼270 GHz in suspended Si membranes with thickness ranging from 0.4 to 15 μm. The measured acoustic lifetime scales linearly with the membrane thickness and is shown to be controlled by the surface specularity which correlates with roughness characterized by atomic force microscopy. Observed Q-factor values up to 2400 at room temperature result from the existence of a local maximum of the material Q in the sub-THz range. However, surface specularity would need to be improved over measured values of ∼0.5 in order to achieve high Q values in nanoscale devices. The results support the validity of the diffuse boundary scattering model in analyzing thermal transport in thin Si membranes.

Laser-induced transient grating setup with continuously tunable period.

We present a modification of the laser-induced transient grating setup enabling continuous tuning of the transient grating period. The fine control of the period is accomplished by varying the angle of the diffraction grating used to split excitation and probe beams. The setup has been tested by measuring dispersion of bulk and surface acoustic waves in both transmission and reflection geometries. The presented modification is fully compatible with optical heterodyne detection and can be easily implemented in any transient grating setup.

Resonant attenuation of surface acoustic waves by a disordered monolayer of microspheres

Attenuation of surface acoustic waves (SAWs) by a disordered monolayer of polystyrene microspheres is investigated. Surface acoustic wave packets are generated by a pair of crossed laser pulses in a glass substrate coated with a thin aluminum film and detected via the diffraction of a probe laser beam. When a 170 μm-wide strip of micron-sized spheres is placed on the substrate between the excitation and detection spots, strong resonant attenuation of SAWs near 240 MHz is observed. The attenuation is caused by the interaction of SAWs with a contact resonance of the microspheres, as confirmed by acoustic dispersion measurements on the microsphere-coated area. Frequency-selective attenuation of SAWs by such a locally resonant metamaterial may lead to reconfigurable SAW devices and sensors, which can be easily manufactured via self-assembly techniques.