Jens Hänisch

Formation of nanosized BaIrO3 precipitates and their contribution to flux pinning in Ir-doped YBa2Cu3O7−δ quasi-multilayers

Structural and transport measurements for quasimultilayers of Ir-doped YBa2Cu3O7−δ prepared by pulsed-laser deposition are presented. Due to metallic Ir doping, BaIrO3 particles form during film growth. These nanosized particles, having a perovskite structure, grow epitaxially in cube-on-cube relationship inside the film. A strong increase in pinning force density and, hence, Jc was found.

Strong Tc dependence for strained epitaxial Ba(Fe1−xCox)2As2 thin films

Ba(Fe1−xCox)2As2 superconducting thin films have been grown on SrTiO3, (La,Sr)(Al,Ta)O3, LaAlO3, and YAlO3 (YAO) single crystal substrates by pulsed laser deposition. All the films, except on YAO, have been grown epitaxially without buffer layers. The films deposited on YAO contained 45° in-plane rotated grains and showed a broad superconducting transition. The onset Tc of the films is observed to increase from 16.2 to 24.5 K with increasing c/a, mainly due to a slight distortion of the AsFe4 tetrahedron. From this correlation, we expect that higher superconducting transition temperatures than 24.5 K in a strained epitaxial film may be possible.

High critical current density and its field dependence in mixed rare earth (Nd,Eu,Gd)Ba2Cu3O7−δ thin films

Compared with mono-rare earth 123 films, ternary rare earth (Nd,Eu,Gd)Ba2Cu3O7−δ (NEG123) films show higher critical current density (Jc) and improved irreversibility field (Hirr), but no increase in the characteristic field corresponding to a crossover from a low-field plateau to a linear region in a log Jc–log H plot. At intermediate fields, Jc vs H scales as H(−0.5±0.05) for NEG123, in contrast to H(−0.73±0.05) for mono-rare earth samples such as Gd123. The slow power decay of Jc vs H together with the improved Jc and Hirr strongly implies that extra flux pinning centers exist in NEG123, which are thought to be noncorrelated stress fields induced by lattice mismatch.

Scaling behavior of the critical current in clean epitaxial Ba(Fe1-xCox)2As2 thin films

The angular-dependent critical current density, Jc(theta), and the upper critical field, Hc2(theta), of epitaxial Ba(Fe1-xCox)2As2 thin films have been investigated. No Jc(theta) peaks for H || c were observed regardless of temperatures and magnetic fields. In contrast, Jc(theta) showed a broad maximum at theta=90 degree, which arises from intrinsic pinning. All data except at theta=90 degree can be scaled by the Blatter plot. Hc2(theta) near Tc follows the anisotropic Ginzburg-Landau expression. The mass anisotropy increased from 1.5 to 2 with increasing temperature, which is an evidence for multi-band superconductivity.

Coherent interfacial bonding on the FeAs tetrahedron in Fe/Ba(Fe1-xCox)2As2 bilayers

We demonstrate the growth of epitaxial Fe/Ba(Fe1−xCox)2As2 bilayers on MgO(001) and (La,Sr)(Al,Ta)O3(001) single crystal substrates using pulsed laser deposition (PLD). This architecture produces a coherent interfacial bond between body-centered cubic iron and Ba(Fe1−xCox)2As2 (Ba–122). The superconducting transition temperatures for both bilayers remain close to that of the PLD target. Direct observation of interfacial bonding between Fe and the Ba–122 FeAs sublattice by atomic resolution transmission electron microscopy implies that this bilayer architecture may work for other iron pnictide systems and pave the way for their fabrication into superconducting/ferromagnetic heterostructures.

Critical current scaling and anisotropy in oxypnictide superconductors.

Having succeeded in the fabrication of epitaxial superconducting LaFeAsO(1-x)F(x) thin films we performed an extensive study of electrical transport properties. In the face of multiband superconductivity we can demonstrate that an anisotropic Ginzburg-Landau scaling of the angular dependent critical current densities can be adopted, although being originally developed for single band superconductors. In contrast with single band superconductors the mass anisotropy of LaFeAsO(1-x)F(x) is temperature dependent. A very steep increase of the upper critical field and the irreversibility field can be observed at temperatures below 6 K, indicating that the band with the smaller gap is in the dirty limit. This temperature dependence can be theoretically described by two dominating bands responsible for superconductivity. A pinning force scaling provides insight into the prevalent pinning mechanism and can be specified in terms of the Kramer model.

Formation and pinning properties of growth-controlled nanoscale precipitates in YBa2Cu3O7-δ/transition metal quasi-multilayers

To study the possibility of enhancing the pinning forces in YBa2Cu3O7?? films through the introduction of nanosized precipitates, quasi-multilayers of YBa2Cu3O7?? and a transition metal (TM = Ti,Zr,Hf) were deposited on single-crystal SrTiO3 substrates using pulsed laser deposition. The transition metal layer thickness was chosen to be less than one unit cell, resulting in separated nanoscale islands that form inclusions with perovskite structure BaTM O3 during film growth. These inclusions grow biaxially textured within the film. Whereas the Ti-doped films show a very strong decrease in the critical temperature Tc and, hence, a strong decrease in the critical current density Jc with increasing TM amount for all temperatures, Hf and Zr doping show an increase in Jc for the smallest amounts of doping. An irreversibility field as high as 10.3?T at 77?K was observed in the case of low Hf content.

Epitaxial Growth of Superconducting Ba(Fe1-xCox)2As2 Thin Films on Technical Ion Beam Assisted Deposition MgO Substrates

The biaxially textured growth of superconducting Co-doped BaFe2As2 (Ba-122) thin films has been realized on ion beam assisted deposition (IBAD) MgO coated conductor templates by employing an iron buffer architecture. The iron pnictide coated conductor showed a superconducting transition temperature of 21.5 K, which is slightly lower than that of Co-doped Ba-122 films on single crystalline MgO substrates. A self-field critical current density of over 105 Acm-2 has already been achieved even at 8 K. The current experiment highlights the potential of possible coated conductor applications of the iron-based superconductors.

Influence of Fe buffer thickness on the crystalline quality and the transport properties of Fe/Ba(Fe1−xCox)2As2 bilayers

The implementation of an Fe buffer layer is a promising way to obtain epitaxial growth of Co-doped BaFe2As2 (Ba-122). However, the crystalline quality and the superconducting properties of Co-doped Ba-122 are influenced by the Fe buffer layer thickness, dFe. The well-textured growth of the Fe/Ba-122 bilayer with dFe = 15 nm results in a high Jc of 0.45 MAcm

Epitaxial LaFeAsO1−xFx thin films grown by pulsed laser deposition

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