Jiro Itatani

5-fs, multi-mJ, CEP-locked parametric chirped-pulse amplifier pumped by a 450-nm source at 1 kHz

We report on the development of an optical parametric chirpedpulse amplifier at a 1-kHz repetition rate with a 5.5-fs pulse duration, a 2.7-mJ pulse energy and carrier-envelope phase-control. The amplifier is pumped by a 450-nm pulse from a frequency-doubled Ti:sapphire laser.

Carrier-envelope phase-dependent high harmonic generation in the water window using few-cycle infrared pulses

High harmonic generation (HHG) using waveform-controlled, few-cycle pulses from Ti:sapphire lasers has opened emerging researches in strong-field and attosecond physics. However, the maximum photon energy of attosecond pulses via HHG remains limited to the extreme ultraviolet region. Long-wavelength light sources with carrier-envelope phase stabilization are promising to extend the photon energy of attosecond pulses into the soft X-ray region. Here we demonstrate carrier-envelope phase-dependent HHG in the water window using sub-two-cycle optical pulses at 1,600 nm. Experimental and simulated results indicate the confinement of soft X-ray emission in a single recombination event with a bandwidth of 75 eV around the carbon K edge. Control of high harmonics by the waveform of few-cycle infrared pulses is a key milestone to generate soft X-ray attosecond pulses. We measure a dependence of half-cycle bursts on the gas pressure, which indicates subcycle deformation of the waveform of the infrared drive pulses in the HHG process.

Observing hot carrier distribution in an n-type epitaxial graphene on a SiC substrate

Hot carrier dynamics in the Dirac band of n-type epitaxial graphene on a SiC substrate were traced in real time using femtosecond-time-resolved photoemission spectroscopy. The spectral evolution directly reflects the energetically linear density of states superimposed with a Fermi–Dirac distribution. The relaxation time is governed by the internal energy dissipation of electron–electron scattering, and the observed electronic temperature indicates cascade carrier multiplication.

Quantum path selection in high-harmonic generation by a phase-locked two-color field

We report the results of our studies on the selection of the quantum path in high-harmonic generation (HHG) with a relative-phase-locked two-color laser field. It is shown that by tuning the relative phase between fundamental and second-harmonic fields, The timing of tunnel ionization and subsequent electron trajectories on the sub-cycle time scale can be controlled. We have clearly observed a phase-dependent two-step feature in the harmonic spectra that can be attributed to the selection of two major trajectories in the two-color field HHG.

Generation of carrier-envelope phase-stable mid-infrared pulses via dual-wavelength optical parametric amplification

Carrier-envelope phase-stable mid-infrared pulses spanning from 5 μm to 11 μm with a pulse energy of 5 μJ were produced by difference frequency generation of two-color near-infrared pulses that were produced in a novel inline optical parametric amplifier. The mid-infrared electric waveform was characterized by electro-optic sampling using 6.5-fs pulses at 620 nm.

Generation of soft x-ray and water window harmonics using a few-cycle, phase-locked, optical parametric chirped-pulse amplifier.

Multimillijoule, few-cycle, carrier-envelope-phase (CEP)-locked, near-IR pulses at 750 nm from an optical parametric chirped-pulse amplifier are applied to the generation of CEP-dependent, soft x-ray high harmonics around the boron K-edge at 188 eV. The dependence on the CEP manifests the phase coherence of high harmonics preserved in the highest-photon energy ever reported. Multimillijoule optical pulses also allow the extension of the cutoff energy up to 325 eV, exceeding the carbon K-edge of the water window. However, in this spectral range, the CEP dependence of harmonic spectra is not observed, suggesting the degradation of temporal coherence due to the heavy ionization of helium atoms.

Large-Scale, High-Efficiency Transmission Grating for Terawatt-Class Ti:Sapphire Lasers at 1 kHz

A novel transmission grating with a large scale (170 mm long, 40 mm high, and 1 mm thick) has been developed. The diffraction efficiency is over 93% and is almost flat from 750 to 850 nm. We developed a 1-kHz, 10-mJ, 0.5-TW Ti:sapphire laser system by using transmission gratings in a compressor. The throughput of the compressor was about 70%. The large-scale grating is capable of increasing the peak power up to multi-terawatts at 1 kHz.

Generation of ultrashort intense optical pulses at 1.6 μm from a bismuth triborate-based optical parametric chirped pulse amplifier with carrier-envelope phase stabilization

We describe a few-cycle intense optical parametric chirped pulse amplifier (OPCPA) in the IR that is based on bismuth triborate (BiB3O6, BIBO) crystals. Two Ti:sapphire chirped pulse amplification systems are used to generate seed and pump pulses for the OPCPA. Carrier-envelope phase (CEP)-stabilized seed pulses in the IR are produced by difference frequency mixing of white light spanning from the visible to near IR range. The seed pulses, which have a nearly one octave-spanning spectrum around 1.6 μm, are temporally stretched in an acousto-optic programmable dispersive filter and amplified up to 550 μJ in two BIBO-based parametric amplifiers without losing their bandwidth. After compression in a fused silica block, we obtained 9.2 fs optical pulses with a repetition rate of 1 kHz, which comprise less than two optical cycles at 1.6 μm. These optical pulses were used to generate extreme ultraviolet (XUV) high harmonics in krypton. We succeeded in measuring the CEP dependence of the XUV radiation near the silicon L edge around 100 eV, verifying the passive stabilization of the CEP of the sub-two cycle IR pulses. The XUV spectra consist of two half-cycle cutoffs and show a clear transition from a modulated structure to a continuum near the cutoff. The continuum-like spectra as well as their CEP dependence indicate that they originate in a single recombination burst, showing that few-cycle IR OPCPA light sources are capable of generating attosecond pulses in the XUV region.

Wavefront analysis of high-efficiency, large-scale, thin transmission gratings

Large-scale (180 × 60 × 1 mm(3)) transmission gratings with groove densities of 1250 and 1740 lines/mm have been developed, resulting in diffraction efficiencies above 95%. The throughput of a folded pulse compressor with two large-scale transmission gratings was approximately 80% in a 20-fs Ti:sapphire chirped-pulse amplification (CPA) laser. The parabolic bending of the transmission grating due to anti-reflection (AR) coating was minimized to 2.9 λ at 633 nm by improving the evaporation process. By a simple analysis, we explain why this level of bending does not induce a wavefront distortion through the transmission grating near the Littrow condition while the wavefront from a reflection grating is distorted to nearly twice the bending of the grating. The calculation based on the measured bending shows that both the group delay difference relative to the ideally flat grating from 750 to 850 nm and the spatial pulse front distortion over a 60-mm-diameter input beam are negligible, even when the dispersive beam covers ~140 mm on the grating. The spatial pulse front distortion measured after the compressor was less than the measurement limit (1.5 fs) for a 20-mm-diameter beam, where the beam size in the dispersive direction on the grating was 85 mm.

1.2 mJ sub-4-fs source at 1 kHz from an ionizing gas

We demonstrate a 1.2 mJ, 3.8 fs, carrier-envelope phase-controlled laser source by novel energy-scalable spectral broadening in an ionizing gas medium, which is widely applicable to sub-10-fs multimillijoule laser systems to obtain sub-2-cycle (<4 fs) multi-millijoule pulses.