Jon D. Swaim

Detection limits in whispering gallery biosensors with plasmonic enhancement

We perform numerical modeling of a gold nanorod bound to the surface of a microtoroid-based biosensor. Localized surface plasmon resonances in the nanorod give rise to strong enhancements in the electric field when excited near resonance, increasing the frequency shift for a single bovine serum albumin molecule by a factor of 870, with even larger enhancements predicted for smaller proteins. On resonance, the frequency shift is predicted to be on the order of MHz, more than an order of magnitude larger than measurement noise arising from time-averaged frequency and thermal fluctuations.

Detection of nanoparticles with a frequency locked whispering gallery mode microresonator

We detect 39 nm × 10 nm gold nanorods using a microtoroid stabilized via the Pound-Drever-Hall method. Real-time detection is achieved with signal-to-noise ratios up to 12.2. These nanoparticles are a factor of three smaller in volume than any other nanoparticle detected using whispering gallery mode sensing to date. We show through repeated experiments that the measurements are reliable and verify the presence of single nanorods on the microtoroid surface using electron microscopy. At our current noise level, the plasmonic enhancement of these nanorods could enable detection of proteins with radii as small as a = 2 nm.

Back-scatter based whispering gallery mode sensing

Whispering gallery mode biosensors allow selective unlabelled detection of single proteins and, combined with quantum limited sensitivity, the possibility for noninvasive real-time observation of motor molecule motion. However, to date technical noise sources, most particularly low frequency laser noise, have constrained such applications. Here we introduce a new technique for whispering gallery mode sensing based on direct detection of back-scattered light. This experimentally straightforward technique is immune to frequency noise in principle, and further, acts to suppress thermorefractive noise. We demonstrate 27 dB of frequency noise suppression, eliminating frequency noise as a source of sensitivity degradation and allowing an absolute frequency shift sensitivity of 76 kHz. Our results open a new pathway towards single molecule biophysics experiments and ultrasensitive biosensors.

Tapered nanofiber trapping of high-refractive-index nanoparticles

A nanofiber-based optical tweezer is demonstrated. Trapping is achieved by combining attractive near-field optical gradient forces with repulsive electrostatic forces. Silica-coated Fe2O3 nanospheres of 300 diameter are trapped as close as 50 nm away from the surface with 810 μW of optical power, with a maximum trap stiffness of 2.7 pN μm−1. Electrostatic trapping forces up to 0.5 pN are achieved, a factor of 50 larger than those achievable for the same optical power in conventional optical tweezers. Efficient collection of the optical field directly into the nanofiber enables ultra-sensitive tracking of nanoparticle motion and extraction of its characteristic Brownian motion spectrum, with a minimum position sensitivity of 3.4 A/Hz.

Atomic vapor as a source of tunable, non-Gaussian self-reconstructing optical modes

In this manuscript, we demonstrate the ability of nonlinear light-atom interactions to produce tunably non-Gaussian, partially self-healing optical modes. Gaussian spatial-mode light tuned near to the atomic resonances in hot rubidium vapor is shown to result in non-Gaussian output mode structures that may be controlled by varying either the input beam power or the temperature of the atomic vapor. We show that the output modes exhibit a degree of self-reconstruction after encountering an obstruction in the beam path. The resultant modes are similar to truncated Bessel-Gauss modes that exhibit the ability to self-reconstruct earlier upon propagation than Gaussian modes. The ability to generate tunable, self-reconstructing beams has potential applications to a variety of imaging and communication scenarios.

Sensitivity of cavity optomechanical field sensors

This article presents a technique for modeling cavity optomechanical field sensors. A magnetic or electric field induces a spatially varying strain across the sensor. The effect of this strain is accounted for by separating the mechanical motion of the sensor into eigenmodes, each modeled by a simple harmonic oscillator. The force induced on each oscillator can then be determined from an overlap integral between strain and the corresponding eigenmode, with the optomechanical coupling strength determining the ultimate resolution with which this force can be detected.

Squeezed-twin-beam generation in strongly absorbing media

We experimentally demonstrate the generation of squeezed, bright twin beams that arise due to competing gain and absorption, in a medium that is overall transparent. To accomplish this, we make use of a nondegenerate four-wave-mixing process in warm potassium vapor such that one of the twin beams experiences strong absorption. At room temperature and above, due to Doppler broadening and smaller frequency detunings compared to other schemes, the ground-state hyperfine splittings used in the present double-

Faster light with competing absorption and gain.

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Causality and information transfer in simultaneously slow- and fast-light media

setup are completely overlapped. We show that despite the resulting significant asymmetric absorption of the twin beams, quantum correlations may still be generated. Our results in this regime demonstrate that the simplified model of gain, followed by loss, is insufficient to describe the amount of quantum correlation resulting from the process.

Whispering gallery mode biosensors with plasmonic enhancement

We experimentally investigate the propagation of optical pulses through a fast-light medium with competing absorption and gain. The combination of strong absorption and optical amplification in a potassium-based four-wave mixing process results in pulse peak advancements up to 88% of the input pulse width, more than 35× that which is achievable without competing absorption. We show that the enhancement occurs even when the total gain of the four-wave mixer is unity, thereby rendering the medium transparent. By varying the pulse width, we observe a transition between fast and slow light, and show that fast light is optimized for large pulse widths.