Joshua Folk

Electron Transport through SingleMn12Molecular Magnets

We report transport measurements through a single-molecule magnet, the Mn12 derivative [Mn12O12(O2C-C6H4-SAc)16(H2O)4], in a single-molecule transistor geometry. Thiol groups connect the molecule to gold electrodes that are fabricated by electromigration. Striking observations are regions of complete current suppression and excitations of negative differential conductance on the energy scale of the anisotropy barrier of the molecule. Transport calculations, taking into account the high-spin ground state and magnetic excitations of the molecule, reveal a blocking mechanism of the current involving nondegenerate spin multiplets.

Kondo Effect in the Presence of Magnetic Impurities

We measure transport through gold grain quantum dots fabricated using electromigration, with magnetic impurities in the leads. A Kondo interaction is observed between dot and leads, but the presence of magnetic impurities results in a gate-dependent zero-bias conductance peak that is split due to a RKKY interaction between the spin of the dot and the static spins of the impurities. A magnetic field restores the single Kondo peak in the case of an antiferromagnetic RKKY interaction. This system provides a new platform to study Kondo and RKKY interactions in metals at the level of a single spin.

Detecting spin-polarized currents in ballistic nanostructures.

We demonstrate a mesoscopic spin polarizer/analyzer system that allows the spin polarization of current from a quantum point contact in a large in-plane magnetic field to be measured. A transverse electron focusing geometry is used to couple current from an emitter point contact into a collector point contact. At large in-plane fields, with the point contacts biased to transmit only a single spin (g<e(2)/h), the voltage across the collector depends on the spin polarization of the current incident on it. Spin polarizations of >70% are found for both emitter and collector at 300 mK and 7 T in-plane field.

Low-Temperature Saturation of the Dephasing Time and Effects of Microwave Radiation on Open Quantum Dots

The dephasing time

Spin Degeneracy and Conductance Fluctuations in Open Quantum Dots

{\ensuremath{\tau}}_{\ensuremath{\phi}}

Ground state spin and coulomb blockade peak motion in chaotic quantum dots

of electrons in open semiconductor quantum dots, measured using ballistic weak localization, is found to saturate below

Decoherence in Nearly Isolated Quantum Dots

\ensuremath{\sim}100\mathrm{mK}

Origins of nonlocality near the neutrality point in graphene.

, roughly twice the electron base temperature, independent of dot size. Microwave radiation deliberately coupled to the dots affects quantum interference indistinguishably from elevated temperatures, suggesting that direct dephasing due to radiation is not the cause of the observed saturation. Coulomb blockade measurements show that the applied microwaves create sufficient source-drain voltages to account for dephasing due to Joule heating.

Quantum chaos in open versus closed quantum dots: Signatures of interacting particles

The dependence of conductance fluctuations on parallel magnetic field is used as a probe of spin degeneracy in open GaAs quantum dots. The variance of fluctuations at high parallel field is reduced from the low-field variance (with broken time-reversal symmetry) by factors ranging from roughly 2 in a 1 microm (2) dot to greater than 4 in 8 microm (2) dots. The factor of 2 is expected for Zeeman splitting of spin-degenerate channels. A possible explanation for the larger suppression based on field-dependent spin-orbit scattering is proposed.

Electron-Hole Asymmetric Chiral Breakdown of Reentrant Quantum Hall States.

We investigate experimentally and theoretically the behavior of Coulomb blockade (CB) peaks in a magnetic field that couples principally to the ground-state spin (rather than the orbital moment) of a chaotic quantum dot. In the first part, we discuss numerically observed features in the magnetic field dependence of CB peak and spacings that unambiguously identify changes in spin S of each ground state for successive numbers of electrons on the dot, N. We next evaluate the probability that the ground state of the dot has a particular spin S, as a function of the exchange strength, J, and external magnetic field strength, B. In the second part, we describe recent experiments on gate-defined GaAs quantum dots in which Coulomb peak motion and spacing are measured as a function of in-plane magnetic field, allowing changes in spin between N and N + 1 electron ground states to be inferred.