K. C. Lee

Entangling macroscopic diamonds at room temperature.

Optical pulses are used to quantum mechanically entangle two diamonds several centimeters apart. Quantum entanglement in the motion of macroscopic solid bodies has implications both for quantum technologies and foundational studies of the boundary between the quantum and classical worlds. Entanglement is usually fragile in room-temperature solids, owing to strong interactions both internally and with the noisy environment. We generated motional entanglement between vibrational states of two spatially separated, millimeter-sized diamonds at room temperature. By measuring strong nonclassical correlations between Raman-scattered photons, we showed that the quantum state of the diamonds has positive concurrence with 98% probability. Our results show that entanglement can persist in the classical context of moving macroscopic solids in ambient conditions.

Single-Photon-Level Quantum Memory at Room Temperature

Room-temperature, easy-to-operate quantum memories are essential building blocks for future long distance quantum information networks operating on an intercontinental scale, because devices like quantum repeaters, based on quantum memories, will have to be deployed in potentially remote, inaccessible locations. Here we demonstrate controllable, broadband and efficient storage and retrieval of weak coherent light pulses at the single-photon level in warm atomic cesium vapor using the robust far off-resonant Raman memory scheme. We show that the unconditional noise floor of this technically simple quantum memory is low enough to operate in the quantum regime, even in a room-temperature environment.

Multimode memories in atomic ensembles

The ability to store multiple optical modes in a quantum memory allows for increased efficiency of quantum communication and computation. Here we compute the multimode capacity of a variety of quantum memory protocols based on light storage in ensembles of atoms. We find that adding a controlled inhomogeneous broadening improves this capacity significantly.

Multi-pulse addressing of a Raman quantum memory: Configurable beam splitting and efficient readout

We address an optical quantum memory with multiple pulses, enabling unit efficiency readout and programmable beam splitting. The resulting coherent processor with built-in storage is universal for scalable photonic quantum information processing.

High-fidelity polarization storage in a gigahertz bandwidth quantum memory

We demonstrate a dual-rail optical Raman memory inside a polarization interferometer; this enables us to store polarization-encoded information at GHz bandwidths in a room-temperature atomic ensemble. By performing full process tomography on the system, we measure up to 97 ± 1% process fidelity for the storage and retrieval process. At longer storage times, the process fidelity remains high, despite a loss of efficiency. The fidelity is 86 ± 4% for 1.5 μs storage time, which is 5000 times the pulse duration. Hence, high fidelity is combined with a large time-bandwidth product. This high performance, with an experimentally simple setup, demonstrates the suitability of the Raman memory for integration into large-scale quantum networks.

Efficient spatially resolved multimode quantum memory

Light storage in atomic ensembles has been implemented successfully, but the retrieval efficiency can be low. We propose to improve this efficiency with appropriately phase-matched backward propagating retrieval. This method allows for easy spatial filtering of the retrieved light; in addition, multiple optical modes can be stored in the transverse momentum of the ensemble. We model walk-off effects with a full numerical simulation, and confirm the applicability of the scheme.

Quantum memory in an optical lattice

Arrays of atoms trapped in optical lattices are appealing as storage media for photons, since motional dephasing of the atoms is eliminated. The regular lattice is also associated with band structure in the dispersion experienced by incident photons. Here we study the influence of this band structure on the efficiency of quantum memories based on electromagnetically induced transparency (EIT) and on Raman absorption. We observe a number of interesting effects, such as both reduced and superluminal group velocities, enhanced atom-photon coupling, and anomalous transmission. These effects are ultimately deleterious to the memory efficiency, but they are easily avoided by tuning the optical fields away from the band edges.

Applications of Raman Scattering in Quantum Technologies

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Entang-bling: Observing quantum correlations in room-temperature solids

Quantum entanglement in the motion of macroscopic solid bodies has implications both for quantum technologies and foundational studies of the boundary between the quantum and classical worlds. Entanglement is usually fragile in room-temperature solids, owing to strong interactions both internally and with the noisy environment. We generated motional entanglement between vibrational states of two spatially separated, millimeter-sized diamonds at room temperature. By measuring strong nonclassical correlations between Raman-scattered photons, we showed that the quantum state of the diamonds has positive concurrence with 98% probability. Our results show that entanglement can persist in the classical context of moving macroscopic solids in ambient conditions.

Synchronizing single photons with quantum memories

Without deterministic single photon sources, multiphoton rates fall exponentially with the number of photons required, making practical photonics unfeasible. We show how quantum memories improve multiphoton rates by many orders of magnitude.