Krzysztof T. Kaczmarek

Interfacing GHz-bandwidth heralded single photons with a warm vapour Raman memory

Broadband quantum memories, used as temporal multiplexers, are a key component in photonic quantum information processing, as they make repeat-until-success strategies scalable. We demonstrate a prototype system, operating on-demand, by interfacing a warm vapour, high time-bandwidth-product Raman memory with a travelling wave spontaneous parametric down-conversion source. We store single photons and observe a clear influence of the input photon statistics on the retrieved light, which we find currently to be limited by noise. We develop a theoretical model that identifies four-wave mixing as the sole important noise source and point towards practical solutions for noise-free operation.

A cavity-enhanced room-temperature broadband Raman memory

Quantum memories enable the synchronisation of photonic operations. Raman memories are a promising platform, but are susceptible to four-wave mixing noise. We present a demonstration of a cavity-enhanced Raman memory, showing suppression of four-wave mixing.

Broadband noise-free optical quantum memory with neutral nitrogen-vacancy centers in diamond

It is proposed that the ground-state manifold of the neutral nitrogen-vacancy center in diamond could be used as a quantum two-level system in a solid-state-based implementation of a broadband noise-free quantum optical memory. The proposal is based on the same-spin Λ-type three-level system created between the two E orbital ground states and the A1 orbital excited state of the center, and the cross-linear polarization selection rules obtained with the application of a transverse electric field or uniaxial stress. Possible decay and decoherence mechanisms of this system are discussed, and it is shown that high-efficiency, noise-free storage of photons as short as a few tens of picoseconds for at least a few nanoseconds could be possible at low temperature.

Theory of noise suppression in Λ -type quantum memories by means of a cavity

Quantum memories, capable of storing single photons or other quantum states of light, to be retrieved on demand, offer a route to large-scale quantum information processing with light. A promising class of memories is based on far-off-resonant Raman absorption in ensembles of Λ-type atoms. However, at room temperature these systems exhibit unwanted four-wave mixing, which is prohibitive for applications at the single-photon level. Here, we show how this noise can be suppressed by placing the storage medium inside a moderate-finesse optical cavity, thereby removing the main roadblock hindering this approach to quantum memory.

Two-way interconversion of millimeter-wave and optical fields in Rydberg gases

We show that cold Rydberg gases enable an efficient six-wave mixing process where terahertz or microwave fields are coherently converted into optical fields and vice versa. This process is made possible by the long lifetime of Rydberg states, the strong coupling of millimeter waves to Rydberg transitions and by a quantum interference effect related to electromagnetically induced transparency (EIT). Our frequency conversion scheme applies to a broad spectrum of millimeter waves due to the abundance of transitions within the Rydberg manifold, and we discuss two possible implementations based on focussed terahertz beams and millimeter wave fields confined by a waveguide, respectively. We analyse a realistic example for the interconversion of terahertz and optical fields in rubidium atoms and find that the conversion efficiency can in principle exceed 90\%.

High efficiency Raman memory by suppressing radiation trapping

Raman interactions in alkali vapours are used in applications such as atomic clocks, optical signal processing, generation of squeezed light and Raman quantum memories for temporal multiplexing. To achieve a strong interaction the alkali ensemble needs both a large optical depth and a high level of spin-polarisation. We implement a technique known as quenching using a molecular buffer gas which allows near-perfect spin-polarisation of over in caesium vapour at high optical depths of up to a factor of 4 higher than can be achieved without quenching. We use this system to explore efficient light storage with high gain in a GHz bandwidth Raman memory.

A noise-free quantum memory for broadband light at room temperature

We implement a low-noise, broadband quantum memory for light via off-resonant two-photon absorption in warm atomic vapour. We store heralded single photons and verify that the retrieved fields are anti-bunched.

A noiseless quantum optical memory at room temperature

A quantum optical memory (QM) is a device that can store and release quantum states of light on demand. Such a device is capable of synchronising probabilistic events, for example, locally synchronising non-deterministic photon sources for the generation of multi-photon states, or successful quantum gate operations within a quantum computational architecture [1], as well as for globally synchronising the generation of entanglement over long distances within the context of a quantum repeater [2]. Desirable attributes for a QM to be useful for these computational and communicational tasks include high end-to-end transmission (including storage and retrieval efficiency), large storage-time-bandwidth product, room temperature operation for scalability and, of utmost importance, noise free performance for true quantum operation.