Lasse Høgstedt

Low-noise mid-IR upconversion detector for improved IR-degenerate four-wave mixing gas sensing.

We compare a nonlinear upconversion detector with a conventional cryogenic InSb detector for the detection of coherent infrared light showing near-shot-noise-limited performance in the upconversion system. The InSb detector is limited by dark noise, which results in a 500 times lower signal-to-noise ratio. The two detectors are compared for the detection of a coherent degenerate four-wave mixing (DFWM) signal in the mid-infrared, and applied to measure trace-level acetylene in a gas flow at atmospheric pressure, probing its fundamental rovibrational transitions. In addition to lower noise, the upconversion system provides image information of the signal, thus adding new functionality compared to standard point detection methods. We further show that the upconversion detector system can be implemented as a simple replacement of the cryogenic detector.

Mid-infrared upconversion spectroscopy

Mid-infrared (MIR) spectroscopy is emerging as an attractive alternative to near-infrared or visible spectroscopy. MIR spectroscopy offers a unique possibility to probe the fundamental absorption bands of a large number of gases as well as the vibrational spectra of complex molecules. In this paper we discuss non-collinear upconversion as a means for obtaining MIR spectra in the 5–10 μm range with a resolution better than 20  cm−1 over the full interval using four discrete phase-match settings. A theoretical treatment of non-collinear upconversion is given and two different experimental implementations are tested.

Upconversion-based lidar measurements of atmospheric CO2

For the first time an upconversion based detection scheme is demonstrated for lidar measurements of atmospheric CO2-concentrations, with a hard target at a range of 3 km and atmospheric backscatter from a range of ~450 m. The pulsed signals at 1572 nm are upconverted to 635 nm, and detected by a photomultiplier tube, to test how the upconversion technology performs in a long range detection system. The upconversion approach is compared to an existing direct detection scheme using a near-IR detector with respect to signal-to-noise ratio and quantum efficiency. It is for the first time analyzed how the field-of-view of a receiver system, for long range detection, depends critically on the parameters for the nonlinear up-conversion process, and how to optimize these parameters in future systems.

Non-collinear upconversion of infrared light

Two dimensional mid-infrared upconversion imaging provides unique spectral and spatial information showing good potential for mid-infrared spectroscopy and hyperspectral imaging. However, to extract spectral or spatial information from the upconverted images an elaborate model is needed, which includes non-collinear interaction. We derive here a general theory providing the far field of the upconverted light when two arbitrary fields interact inside a nonlinear crystal. Theoretical predictions are experimentally verified for incoherent radiation and subsequently applied to previously published data with good agreement.

500 nm continuous wave tunable single-frequency mid-IR light source for C-H spectroscopy

A computer controlled tunable mid-IR light source, based on single resonant difference frequency generation (DFG), is experimentally investigated. The DFG process is pumped by an external cavity tapered diode laser, tunable over a spectral range of 30 nm. Grating feedback to the single mode channel of the tapered diode narrows the spectrum and allows for tuning of the emitted spectrum in the range from 780 to 810 nm. The DFG process takes place intra-cavity in a high finesse diode pumped 1064 nm solid state Nd:YVO4 laser cavity, using periodically poled LiNbO3 as the nonlinear material. Based on this new approach, a tunable single-frequency output power exceeding 3 mW was obtained in the mid-IR tuning range from 2.9 to 3.4 μm.

Upconversion detector for range-resolved DIAL measurement of atmospheric CH4

We demonstrate a robust, compact, portable and efficient upconversion detector (UCD) for a differential absorption lidar (DIAL) system designed for range-resolved methane (CH4) atmospheric sensing. The UCD is built on an intracavity pump system that mixes a 1064 nm pump laser with the lidar backscatter signal at 1646 nm in a 25-mm long periodically poled lithium niobate crystal. The upconverted signal at 646 nm is detected by a photomultiplier tube (PMT). The UCD with a noise equivalent power around 127 fW/Hz1/2 outperforms a conventional InGaAs based avalanche photodetector when both are used for DIAL measurements. Using the UCD, CH4 DIAL measurements have been performed yielding differential absorption optical depths with relative errors of less than 11% at ranges between 3 km and 9 km.

Upconversion enhanced degenerate four-wave mixing in the mid-infrared for sensitive detection of acetylene in gas flows

We present a new background free method for in situ gas detection that combines degenerate four-wave mixing with an infra-red light detector based on parametric frequency upconversion of infra-red light. The system is demonstrated at mid infrared wavelengths for low concentration measurements of acetylene diluted in a N2 gas flow at ambient conditions. It is demonstrated that the system is able to cover more than 100 nm in scanning range and detect concentrations as low as 3 ppm based on the R9e line. A major issue in small signal measurements is scattered light and it is showed how a spatial analysis can be used to reduce this level.

A mul ti-element THz imaging system

We report on a broadband multi-element THz imaging system based on fiber-coupled, integrated photoconductive emitters and detectors. 32 detectors and 32 emitters are arranged in a planar array. Advanced image reconstruction algorithms are employed to reconstruct an object in the imaging plane.

Identification of black plastics using an upconversion based mid-infrared imaging spectrograph

With upconversion based mid-infrared reflection spectroscopy we have proved it possible to differentiate between several common types of black plastics. This allow for the possibility of efficient sorting of black plastics in clean fractions, paving the road for both economically viable and ecologically sustainable recycling.

Intracavity upconversion for IR absorption lidar: Comparison of linear and ring cavity designs

Upconversion detection is a promising technology for measurement of IR signals in the 1.5 μm–2 μm region used for lidar remote sensing [1-2]. In comparison to conventional InGaAs detector, the upconversion detector can achieve IR detection with better signal-to-noise ratio (SNR), not only due to lower dark noise directly, but also because of its limited field-of-view and acceptance bandwidth that results in a much lower background noise.