Laurent Talon

Autocatalytic reaction fronts inside a porous medium of glass spheres.

We analyze experimentally chemical waves propagation in the disordered flow field of a porous medium. The reaction fronts travel at a constant velocity which drastically depends on the mean flow direction and rate. The fronts may propagate either downstream and upstream but, surprisingly, they remain static over a range of flow rate values. Resulting from the competition between the chemical reaction and the disordered flow field, these frozen fronts display a particular sawtooth shape. The frozen regime is likely to be associated with front pinning in low velocity zones, the number of which varies with the ratio of the mean flow and the chemical front velocities.

Experimental Evidence for Three Universality Classes for Reaction Fronts in Disordered Flows.

Self-sustained reaction fronts in a disordered medium subject to an external flow display self-affine roughening, pinning, and depinning transitions. We measure spatial and temporal fluctuations of the front in 1+1 dimensions, controlled by a single parameter, the mean flow velocity. Three distinct universality classes are observed, consistent with the Kardar-Parisi-Zhang (KPZ) class for fast advancing or receding fronts, the quenched KPZ class (positive-qKPZ) when the mean flow approximately cancels the reaction rate, and the negative-qKPZ class for slowly receding fronts. Both qKPZ classes exhibit distinct depinning transitions, in agreement with the theory.

Stabilizing viscosity contrast effect on miscible displacement in heterogeneous porous media, using lattice Bhatnagar–Gross–Krook simulations

We analyze the displacement of a viscous fluid by a miscible more viscous one in heterogeneous porous media. We performed lattice Bhatnagar–Gross–Krook simulations, which were previously successfully applied to the study of the dispersion of a passive tracer in a stochastic heterogeneous porous medium. In the present situation, the flow is stable (no viscous fingering) and leads to an overall Gaussian dispersion, the coefficient of which decreases as the viscosity ratio increases. The results are in reasonable agreement with the stochastic approach of Welty and Gelhar.

Strong pinning of propagation fronts in adverse flow.

Reaction fronts evolving in a porous medium exhibit a rich dynamical behavior. In the presence of an adverse flow, experiments show that the front slows down and eventually gets pinned, displaying a particular sawtooth shape. Extensive numerical simulations of the hydrodynamic equations confirm the experimental observations. Here we propose a stylized model, predicting two possible outcomes of the experiments for large adverse flow: either the front develops a sawtooth shape or it acquires a complicated structure with islands and overhangs. A simple criterion allows one to distinguish between the two scenarios and its validity is reproduced by direct hydrodynamical simulations. Our model gives a better understanding of the transition and is relevant in a variety of domains, when the pinning regime is strong and only relies on a small number of sites.