Longqing Cong

Ultrasensitive terahertz sensing with high-Q Fano resonances in metasurfaces

High quality factor resonances are extremely promising for designing ultra-sensitive refractive index label-free sensors, since it allows intense interaction between electromagnetic waves and the analyte material. Metamaterial and plasmonic sensing have recently attracted a lot of attention due to subwavelength confinement of electromagnetic fields in the resonant structures. However, the excitation of high quality factor resonances in these systems has been a challenge. We excite an order of magnitude higher quality factor resonances in planar terahertz metamaterials that we exploit for ultrasensitive sensing. The low-loss quadrupole and Fano resonances with extremely narrow linewidths enable us to measure the minute spectral shift caused due to the smallest change in the refractive index of the surrounding media. We achieve sensitivity levels of 7.75 × 103 nm/refractive index unit (RIU) with quadrupole and 5.7 × 104 nm/RIU with the Fano resonances which could be further enhanced by using thinner substrates. These findings would facilitate the design of ultrasensitive real time chemical and biomolecular sensors in the fingerprint region of the terahertz regime.

Experimental demonstration of ultrasensitive sensing with terahertz metamaterial absorbers: A comparison with the metasurfaces

Planar metasurfaces and plasmonic resonators have shown great promise for sensing applications across the electromagnetic domain ranging from the microwaves to the optical frequencies. However, these sensors suffer from lower figure of merit and sensitivity due to the radiative and the non-radiative loss channels in the plasmonic metamaterial systems. We demonstrate a metamaterial absorber based ultrasensitive sensing scheme at the terahertz frequencies with significantly enhanced sensitivity and an order of magnitude higher figure of merit compared to planar metasurfaces. Magnetic and electric resonant field enhancement in the impedance matched absorber cavity enables stronger interaction with the dielectric analyte. This finding opens up opportunities for perfect metamaterial absorbers to be applied as efficient sensors in the finger print region of the electromagnetic spectrum with several organic, explosive, and bio-molecules that have unique spectral signature at the terahertz frequencies.

A perfect metamaterial polarization rotator

Polarization conveys valuable information for electromagnetic signal processing exhibiting tremendous potential in developing application driven photonic devices. Manipulation of polarization state of an electromagnetic wave has drawn a lot of research interests in many different fields, especially in the terahertz regime. Here, we propose a unique approach to efficiently rotate the linear polarization of terahertz wave in a broadband configuration with tri-layer metasurfaces. We experimentally observe a nearly perfect orthogonal polarization conversion with an ultrahigh efficiency, demonstrating a ultrathin terahetz rotator. The Fabry-Perot cavity effect in the tri-layer metasurfaces is attributed to the underlying mechanism of high transmittance and polarization rotation.

Manipulating polarization states of terahertz radiation using metamaterials

We present a double-ring-chain metamaterial that enables efficient polarization conversion of terahertz waves. The experimental results and numerical simulations reveal that the linear-to-linear polarization rotation and linear-to-elliptic polarization transformation are simply accomplished by altering the dimensional parameters of the metamaterial unit cells. The polarization state conversion is found to be critically related to the resonant properties of the long bars and the rings in the unit geometries and is well described by the Jones matrix. This approach promises both passive and active polarization conversion of terahertz radiation using planar metamaterials.

Multispectral terahertz sensing with highly flexible ultrathin metamaterial absorber

We report the simulation, fabrication, and experimental characterization of a multichannel metamaterial absorber with the aim to be used as a label-free sensing platform in the terahertz regime. The topology of the investigated resonators deposited on a thin flexible polymer by means of optical lithography is capable of supporting multiple resonances over a broad frequency range due to the individual contribution of each sub-element of the unit cell. In order to explore the performance of the chosen structure in terms of sensing phenomenon, the reflection feature is monitored upon variation of the refractive index and the thickness of the analyte. We achieve numerically maximum frequency sensitivity of about 139.2 GHz/refractive index unit. Measurements carried out using terahertz time-domain spectroscopy show good agreement with the numerical predictions. The results are very promising, suggesting a potential use of the metamaterial absorber in wide variety of multispectral terahertz sensing applications.

Tailoring the slow light behavior in terahertz metasurfaces

We experimentally study the effect of near field coupling on the transmission of light in terahertz metasurfaces. Our results show that tailoring the coupling between the resonators modulates the amplitude of resulting electromagnetically induced transmission, probed under different types of asymmetries in the coupled system. Observed change in the transmission amplitude is attributed to the change in the amount of destructive interference between the resonators in the vicinity of strong near field coupling. We employ a two-particle model to theoretically study the influence of the coupling between bright and quasi-dark modes on the transmission properties of the system and we find an excellent agreement with our observed results. Adding to the enhanced transmission characteristics, our results provide a deeper insight into the metamaterial analogues of atomic electromagnetically induced transparency and offer an approach to engineer slow light devices, broadband filters, and attenuators at terahertz frequencies.

A Tunable Dispersion-Free Terahertz Metadevice with Pancharatnam-Berry-Phase-Enabled Modulation and Polarization Control.

It is extremely challenging to control the phase of light at will in free space. Here, Pancharatnam-Berry-phase-enabled, tunable phase control of free-space light is experimentally demonstrated in an ultrathin flexible dispersion-free metadevice. This metadevice enables the broadband conversion of linearly polarized light into any desired output polarization.

Active Photoswitching of Sharp Fano Resonances in THz Metadevices

Fano resonances offer exciting features in enhancing the non-linearity and sensing capabilities in metamaterial systems. An active photoswitching of Fano resonances in a terahertz metadevice at low optical pump powers is demonstrated, which signifies the extreme sensitivity of the high-quality-factor resonant electric field to the external light illumination.

Probing the transition from an uncoupled to a strong near-field coupled regime between bright and dark mode resonators in metasurfaces

The coupling of multiple plasmonic resonators that sustain bright or dark modes provide intriguing spectral signatures. However, probing the onset of coupling effects while engaging the resonators with an increasing proximity has not yet been studied experimentally in detail. Nevertheless, this is of utmost importance to bridge the phenomenological understanding with the peculiarities of real-world-samples. Here, we take advantage of the ability to control spatial dimensions of THz metasurfaces deep in the sub-wavelength domain to study different regimes that occur while coupling split-ring-resonators that sustain a bright and a dark mode with increasing strength. We identify the length scales at which the resonators are uncoupled and then enter the regimes of weak, moderate, and strong coupling. It is shown that a strong coupling takes place only at distances smaller than one hundredth of the resonance wavelength. Understanding the features that emerge from such hybridization is important to take advantage of fundamental effects in metamaterials such as classical analogs of electromagnetically induced transparency, lasing spaser, near-field manipulation, and sensing with dark mode resonances.

Modulating the fundamental inductive-capacitive resonance in asymmetric double-split ring terahertz metamaterials

We investigate resonant transmission of planar asymmetric metamaterials made from double split-ring resonators. As the symmetry of the unit cell resonator is broken by displacing the two gaps away from the center in opposite directions, a giant amplitude modulation is observed at the fundamental inductive-capacitive resonance due to strong polarization conversion. The modulation is nearly absent when the gaps are moved together in the same direction. This effect persists in metamaterials with different structural designs. These asymmetric metamaterials may open up new avenues toward the control of terahertz waves and the development of modulator and polarizer based terahertz devices.