Lorraine A. Remer

Aerosols from Overseas Rival Domestic Emissions over North America

Particles Without Borders Aerosols have important and often adverse impacts on atmospheric composition, air quality, and climate. However, aerosols can be transported long distances, limiting the efficacy of local regulations. Yu et al. (p. 566) used satellite data to estimate how much of the aerosol load in the atmosphere above North America originates overseas. Approximately half of the dust and pollution over North America comes from Asia, Europe, Africa, and the Middle East. Asian dust is the largest fraction of this total. Furthermore, potential increases in dust emissions in response to climate change might overwhelm any reductions in pollution from emerging Asian economies. Roughly half of all particulate matter found in the air above North America originates from sources overseas. Many types of aerosols have lifetimes long enough for their transcontinental transport, making them potentially important contributors to air quality and climate change in remote locations. We estimate that the mass of aerosols arriving at North American shores from overseas is comparable with the total mass of particulates emitted domestically. Curbing domestic emissions of particulates and precursor gases, therefore, is not sufficient to mitigate aerosol impacts in North America. The imported contribution is dominated by dust leaving Asia, not by combustion-generated particles. Thus, even a reduction of industrial emissions of the emerging economies of Asia could be overwhelmed by an increase of dust emissions due to changes in meteorological conditions and potential desertification.

Suomi‐NPP VIIRS aerosol algorithms and data products

[1]xa0The Visible Infrared Imaging Radiometer Suite (VIIRS) instrument on board the Suomi National Polar-orbiting Partnership (S-NPP) spacecraft was launched in October 2011. The instrument has 22 spectral channels with band centers from 412u2009nm to 12,050u2009nm. The VIIRS aerosol data products are derived primarily from the radiometric channels covering the visible through the short-wave infrared spectral regions (412u2009nm to 2250u2009nm). The major components of the VIIRS aerosol retrieval process are data screening, land inversion, ocean inversion, suspended matter typing, and aggregation. The primary data product produced is the aerosol optical thickness (AOT) environmental data record. A higher resolution AOT intermediate product is also produced. These AOT products and their corresponding retrieval algorithms are described in detail, including theoretical basis, retrieval limitations, and data quality flagging. Preliminary evaluation of the data products has been undertaken by the VIIRS aerosol calibration/validation team using Aerosol Robotic Network ground-based observations to show that the performance of AOT retrievals meets the requirements specified in the Joint Polar Satellite System Level 1 requirements.

The fertilizing role of African dust in the Amazon rainforest: A first multiyear assessment based on data from Cloud‐Aerosol Lidar and Infrared Pathfinder Satellite Observations

The productivity of the Amazon rainforest is constrained by the availability of nutrients, in particular phosphorus (P). Deposition of long-range transported African dust is recognized as a potentially important but poorly quantified source of phosphorus. This study provides a first multiyear satellite-based estimate of dust deposition into the Amazon Basin using three-dimensional (3-D) aerosol measurements over 2007–2013 from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). The 7u2009year average of dust deposition into the Amazon Basin is estimated to be 28 (8–48)u2009Tgu2009a−1 or 29 (8–50)u2009kgu2009ha−1u2009a−1. The dust deposition shows significant interannual variation that is negatively correlated with the prior-year rainfall in the Sahel. The CALIOP-based multiyear mean estimate of dust deposition matches better with estimates from in situ measurements and model simulations than a previous satellite-based estimate does. The closer agreement benefits from a more realistic geographic definition of the Amazon Basin and inclusion of meridional dust transport calculation in addition to the 3-D nature of CALIOP aerosol measurements. The imported dust could provide about 0.022u2009(0.006–0.037)u2009Tgu2009P of phosphorus per year, equivalent to 23 (7–39)u2009gu2009Pu2009ha−1u2009a−1 to fertilize the Amazon rainforest. This out-of-basin phosphorus input is comparable to the hydrological loss of phosphorus from the basin, suggesting an important role of African dust in preventing phosphorus depletion on timescales of decades to centuries.

Measurement of atmospheric optical parameters on U.S. Atlantic coast sites, ships, and Bermuda during TARFOX

The Aerosol Robotic Network (AERONET) of automatic Sun/sky radiometers collected data on U.S. Atlantic coast sites, ships, and Bermuda in 1996 during the Tropospheric Aerosol Radiative Forcing Observational Experiment (TARFOX). Spatial and temporal analysis of Sun photometry data was supported by synoptic analysis of air mass evolution. The spatial distribution of aerosol optical depth is presented. In several cases the aerosol size distributions deduced from sky almucantar measurements and solar disk attenuation measurements at the various coastal sites yielded similar results within the same air masses. Ship-based measurements in the Atlantic Ocean showed significant maritime aerosol optical property variations which for the most part could be attributed to the influence of continental sources and Saharan dust events. The Bermuda data (optical depths and Angstrom parameter values) illustrated changes in atmospheric optical properties for various air masses and trajectories. Almost no correlation was observed between aerosol optical depth and water vapor content when the data from all stations and ship measurements were considered together. In the case of individual stations or ship transects, different degrees of correlation could be observed. In continental conditions on the east coast, optical depth and water vapor are well correlated, while in a maritime environment, optical depth can be relatively small despite high water vapor contents.

Preliminary evaluation of S‐NPP VIIRS aerosol optical thickness

The Visible Infrared Imaging Radiometer Suite (VIIRS) is the next-generation polar-orbiting operational environmental sensor with a capability for global aerosol observations. The VIIRS aerosol Environmental Data Record (EDR) is expected to continue the decade-long successful multispectral aerosol retrieval from the NASAs Earth Observing System Moderate Resolution Imaging Spectroradiometer (MODIS) for scientific research and applications. Since the launch of the Suomi National Polar-orbiting Partnership (S-NPP), the VIIRS aerosol calibration/validation team has been continuously monitoring, evaluating, and improving the performance of VIIRS aerosol retrievals. In this study, the VIIRS aerosol optical thickness (AOT) at 550u2009nm EDR at current Provisional maturity level is evaluated by comparing it with MODIS retrievals and measurements from the Aerosol Robotic Network (AERONET) and the Maritime Aerosol Network (MAN). The VIIRS global mean AOT at 550u2009nm differs from that of MODIS by approximately −0.01 over ocean and 0.03 over land (0.00 and −0.01 for the collocated retrievals) but shows larger regional biases. Global validation with AERONET and with MAN measurements shows biases of 0.01 over ocean and −0.01 over land, with about 64% and 71% of retrievals falling within the expected uncertainty range established by MODIS over ocean (±(0.03u2009+u20090.05AOT)) and over land (±(0.05u2009+u20090.15AOT)), respectively. The VIIRS retrievals over land exhibit slight overestimation over vegetated surfaces and underestimation over soil-dominated surfaces. These results show that the VIIRS AOT at 550u2009nm product provides a solid global data set for quantitative scientific investigations and environmental monitoring.

Aerosol indirect effect on tropospheric ozone via lightning

[1]xa0Tropospheric ozone (O3) is a pollutant and major greenhouse gas and its radiative forcing is still uncertain. Inadequate understanding of processes related to O3 production, in particular those natural ones such as lightning, contributes to this uncertainty. Here we demonstrate a new effect of aerosol particles on O3production by affecting lightning activity and lightning-generated NOx (LNOx). We find that lightning flash rate increases at a remarkable rate of 30 times or more per unit of aerosol optical depth. We provide observational evidence that indicates the observed increase in lightning activity is caused by the influx of aerosols from a volcano. Satellite data analyses show O3is increased as a result of aerosol-induced increase in lightning and LNOx, which is supported by modle simulations with prescribed lightning change. O3production increase from this aerosol-lightning-ozone link is concentrated in the upper troposphere, where O3 is most efficient as a greenhouse gas. In the face of anthropogenic aerosol increase our findings suggest that lightning activity, LNOx and O3, especially in the upper troposphere, have all increased substantially since preindustrial time due to the proposed aerosol-lightning-ozone link, which implies a stronger O3 historical radiative forcing. Aerosol forcing therefore has a warming component via its effect on O3 production and this component has mostly been ignored in previous studies of climate forcing related to O3and aerosols. Sensitivity simulations suggest that 4–8% increase of column tropospheric ozone, mainly in the tropics, is expected if aerosol-lighting-ozone link is parameterized, depending on the background emission scenario. We note, however, substantial uncertainties remain on the exact magnitude of aerosol effect on tropospheric O3 via lightning. The challenges for obtaining a quantitative global estimate of this effect are also discussed. Our results have significant implications for understanding past and projecting future tropospheric O3forcing as well as wildfire changes and call for integrated investigations of the coupled aerosol-cloud-chemistry system.

An enhanced VIIRS aerosol optical thickness (AOT) retrieval algorithm over land using a global surface reflectance ratio database

The Visible/Infrared Imager Radiometer Suite (VIIRS) on board the Suomi National Polar-orbiting Partnership (S-NPP) satellite has been retrieving aerosol optical thickness (AOT), operationally and globally, over ocean and land since shortly after S-NPP launch in 2011. However, the current operational VIIRS AOT retrieval algorithm over land has two limitations in its assumptions for land surfaces: (1) it only retrieves AOT over the dark surfaces and (2) it assumes that the global surface reflectance ratios between VIIRS bands are constants. In this work, we develop a surface reflectance ratio database over land with a spatial resolution 0.1°u2009×u20090.1° using 2u2009years of VIIRS top of atmosphere reflectances. We enhance the current operational VIIRS AOT retrieval algorithm by applying the surface reflectance ratio database in the algorithm. The enhanced algorithm is able to retrieve AOT over both dark and bright surfaces. Over bright surfaces, the VIIRS AOT retrievals from the enhanced algorithm have a correlation of 0.79, mean bias of −0.008, and standard deviation (STD) of error of 0.139 when compared against the ground-based observations at the global AERONET (Aerosol Robotic Network) sites. Over dark surfaces, the VIIRS AOT retrievals using the surface reflectance ratio database improve the root-mean-square error from 0.150 to 0.123. The use of the surface reflectance ratio database also increases the data coverage of more than 20% over dark surfaces. The AOT retrievals over bright surfaces are comparable to MODIS Deep Blue AOT retrievals.

On the signature of the cirrus twilight zone

Cirrus clouds are known to play a key role in the climate system, but their overall effect on Earth?s radiation budget is not yet fully quantified. The uncertainties are, in part, due to ambiguities in cirrus extent or coverage. Here we show that despite careful filtering of cloudy pixels, cirrus clouds have a clear statistical signature. This signature can be estimated by the proximity to detectable cirrus clouds. Such a residual signature can affect retrievals that rely on a cloud-free atmosphere, such as aerosol optical depth (AOD) or sea surface temperature. Analyzing MODIS raw-data and products, we show a clear increase in the reflectance when approaching detectable cirrus clouds. We estimated a mean increase in AOD of 0.03???0.01 and a decrease in the Angstrom-exponent of ?0.22???0.20 in the first kilometer around detectable cirrus. The effect decays tenfold at a typical distance of 5.5???1.8 km. Such trends confirm the contribution of large particles that are likely to be ice crystals to the so-called cloud-free atmosphere near detectable cirrus clouds.

Just add aerosols

Data from clean regions of the atmosphere show how little aerosol is needed to change clouds. [Also see Report by Koren et al.] The more carbon dioxide and other greenhouse gases in the atmosphere, the stronger the climate warming that results. Likewise, the more aerosol particles suspended in the atmosphere, the greater the ability of these particles either to scatter sunlight back to space and cool the planet or to absorb sunlight in the atmosphere, thereby warming the atmosphere while cooling Earths surface. However, not all such climate forcing processes depend linearly on the concentrations of their forcing agent. The climatic effects of aerosols are complicated by their interactions with clouds (1). On page 1143 of this issue, Koren et al. (2) show that even small additions of aerosol particles to clouds in the cleanest regions of Earths atmosphere will have a large effect on those clouds and their contribution to climate forcing.

Dust, fertilization and sources

Aerosols, tiny suspended particles in the atmosphere, play an important role in modifying the Earths energy balance and are essential for the formation of cloud droplets. Suspended dust particles lifted from the worlds arid regions by strong winds contain essential minerals that can be transported great distances and deposited into the ocean or on other continents where productivity is limited by lack of usable minerals [1]. Dust can transport pathogens as well as minerals great distance, contributing to the spread of human and agricultural diseases, and a portion of dust can be attributed to human activity suggesting that dust radiative effects should be included in estimates of anthropogenic climate forcing. The greenish and brownish tints in figure 1 show the wide extent of monthly mean mineral dust transport, as viewed by the MODerate resolution Imaging Spectroradiometer (MODIS) satellite sensor. Figure 1. The monthly mean global aerosol system for February 2006 from the MODIS aboard the Terra satellite. The brighter the color, the greater the aerosol loading. Red and reddish tints indicate aerosol dominated by small particles created primarily from combustion processes. Green and brownish tints indicate larger particles created from wind-driven processes, usually transported desert dust. Note the bright green band at the southern edge of the Saharan desert, the reddish band it must cross if transported to the southwest and the long brownish transport path as it crosses the Atlantic to South America. Image courtesy of the NASA Earth Observatory (http://earthobservatory.nasa.gov). Even though qualitatively we recognize the extent and importance of dust transport and the role that it plays in fertilizing nutrient-limited regions, there is much that is still unknown. We are just now beginning to quantify the amount of dust that exits one continental region and the fraction that arrives at another continent [2]. At the deposition end of the chain, it is still unclear how the limited minerals in the dust such as iron are released for uptake by organisms either on land or in the ocean. Not all dust deposited into oceans results in a phytoplankton bloom. The process requires a chemical pathway that mobilizes a fraction of the iron into soluble form. Meskhidze et al [3] show that phytoplankton blooms following dust transport from the Gobi desert in Asia into the Pacific ocean result in a phytoplankton bloom only if the dust is accompanied by high initial SO2-to-dust ratios, suggesting that sulfuric acid coatings on the dust particle mobilize the embedded iron in the dust for phytoplankton uptake. Quantifying transport, deposition and nutrient availability are the latter ends of a puzzle that must begin by identifying and quantifying dust emission at the sources. The emission process is complex at the microscale requiring the right conditions for saltation and bombardment, which makes identification and inclusion of sources in global transport models very difficult. The result is that estimates of annual global dust emissions range from 1000 to 3000 Tg per year [4]. Even as global estimates of dust emissions are uncertain, localizing the sources brings even greater uncertainty. It has been recognized for several years that dust sources are not uniformly distributed over the arid regions of the Earth, but are regulated to topographic lows associated with dried lake deposits [5]. Using aerosol information from satellites, a comprehensive map of the worlds source regions shows sources localized to specific areas of the Earths arid regions [6]. Still these maps suggest broad emission sources covering several degrees of latitude and longitude. In the paper by Koren and co-authors [7] appearing in this issue, one particular dust source, the Bod?l? depression in Chad, is analyzed in detail. They find that the specific topography of the depression combined with the prevailing wind direction in the winter provides perfect conditions for aerosol saltation, uplift and transport. The winter Bod?l? dust is carried over the populated regions of west Africa where it can be affected by smoke and urban pollution before it continues transport over the Atlantic and towards Amazonia. Although Koren et al do not speculate on the chemical possibilities in their paper, the interaction between the dust and the pollutants provides opportunity for acids to coat the dust particles and to mobilize the iron compounds, creating a highly efficient fertilizing agent for ocean phytoplankton and the biota of the Amazon forest. Koren et al do quantify the dust emission of the Bod?l? depression, estimating that this small area produces approximately 50% of the Saharan dust deposited in the Amazon. The findings of Koren and his co-authors suggest that dust emission sources may be highly localized spots in the Earths deserts that can be mapped precisely by satellites of moderate to fine resolution. Like fire hot spots that localize smoke emission, desert dust hot spots can be identified with great detail. This can provide aerosol transport models with better source emission information and improve estimates that will help in making estimates concerning biogeochemical processes and also estimates of climate forcing and response. References [1] Swap R et al 1992 Saharan dust in the Amazon basin Tellus B 44 133-49 (doi:10.1034/j.1600-0889.1992.t01-1-00005.x) [2] Kaufman Y J, Koren I, Remer L A, Tanr? D, Ginoux P and Fan S 2005 Dust transport and deposition observed from the Terra-MODIS space observations J. Geophys. Res. 110 D10S12 (doi:10.1029/2003JD004436) [3] Meskhidze N, Chameides W L and Nenes A 2005 Dust and pollution: a recipe for enhanced ocean fertizilation? J. Geophys. Res. 110 (D3) D03301 (doi:10.1029/2004JD005082) [4] Cakur R V et al 2006 Constraining the magnitude of the global dust cycle by minimizing the difference between a model and observations J. Geophys. Res. 111 D06207 (doi:10.1029/2005JD005791) [5] Ginoux P et al 2001 Sources and distribution of dust aerosol simulated with the GOCART model J. Geophys. Res. 106 20255-74 (doi:10.1029/2000JD000053) [6] Prospero J M, Ginoux P, Torres O, Nicholson S E and Gill T E 2002 Environmental characterization of global sources of atmospheric soil dust identified with the NIMBUS 7 total Ozone Mapping Spectrometer (TOMS) absorbing aerosol product Rev. Geophys. 40 (1) 1002 (doi:10.1029/2000RG000095) [7] Koren I, Kaufman Y J, Washington R, Todd M C, Rudich Y, Martins J V and Rosenfeld D 2006 The Bod?l? depression: a single spot in the Sahara that provides most of the mineral dust to the Amazon forest Environ. Res Lett. 1 014005 (doi:10.1088/1748-9326/1/1/014005) Lorraine A Remer received a BS degree in atmospheric science from the University of California, Davis, in 1980, an MS degree in oceanography from the Scripps Institution of Oceanography, University of California, San Diego, in 1983, and a PhD degree, also in atmospheric science from the University of California, Davis, in 1991. She became involved with the MODIS retrievals of atmospheric aerosols in 1991, first as a Research Scientist with Science Systems and Applications, Inc., and subsequently with the National Aeronautics and Space Administration, which she joined in 1998. She is an Associate Member of the MODIS Science Team and a Member of the Global Aerosol Climatology Project Science Team.