Luca Razzari

Generation of 1.5 µJ single-cycle terahertz pulses by optical rectification from a large aperture ZnTe crystal

We demonstrate the generation muJ-level, single-cycle terahertz pulses by optical rectification from a large-aperture ZnTe single crystal wafer. Energies up to 1.5 muJ per pulse and a spectral range extending to 3 THz were obtained using a 100 Hz Ti:sapphire laser source and a 75-mmdiameter, 0.5-mm-thick, (110) ZnTe crystal, corresponding to an average power of 150 muW and an energy conversion efficiency of 3.1 x 10(-5). We also demonstrate real-time imaging of the focused terahertz beam using a pyroelectric infrared camera.

Z-scan measurements using high repetition rate lasers: how to manage thermal effects

We demonstrate the effectiveness of a simple method for using Z-scan technique with high repetition rate lasers managing cumulative thermal effects. Following Falconieri [J. Opt. A, 1 (1999) 662], time evolution of Z-scan signal is recorded. We use data time correlation to extrapolate with accuracy the instantaneous nonlinear optical response of the sample. The method employed allows us to clearly evaluate the order of the absorption process underlying the thermo-optical nonlinearities. Using a 76 MHz repetition rate laser with 120 fs pulsewidth we measure third order nonlinearities and thermal properties of CS2 and toluene in accordance with values obtained with low repetition rate light sources.

On-chip CMOS-compatible all-optical integrator

One reason for using photonic devices is their speed—much faster than electronic circuits—but there are many challenges in integrating the two technologies. Ferrera et al. construct a CMOS-compatible monolithic optical waveform integrator, a key building block for photonic circuits.

Engineering the Absorption and Field Enhancement Properties of Au-TiO2 Nanohybrids via Whispering Gallery Mode Resonances for Photocatalytic Water Splitting.

Recently, surface plasmon resonance (SPR) effects have been widely used to construct photocatalysts which are active in the visible spectral region. Such plasmonic photocatalysts usually comprise a semiconductor material transparent in the visible range (such as TiO2) and plasmonic nano-objects (e.g., Au nanoparticles (Au NPs)). Specific SPRs, though, only partially cover the visible spectrum and feature weak light absorption. Here, we explore the unique role played by whispering gallery mode (WGM) resonances in the expression of the photocatalytic activity of plasmonic photocatalysts. Using numerical simulations, we demonstrate that, by solely exploiting a proper geometrical arrangement and WGM resonances in a TiO2 sphere, the plasmonic absorption can be extended over the entire visible range and can be increased by more than 40 times. Furthermore, the local electric field at the Au-TiO2 interface is also considerably enhanced. These results are experimentally corroborated, by means of absorption spectroscopy and Raman measurements. Accordingly, such WGM-assisted plasmonic photocatalysts, when employed in water splitting experiments, exhibit enhanced activity in the visible range. Our findings show a promising and straightforward way to design full solar spectrum photocatalysts.

Reduced photorefraction in hafnium-doped single-domain and periodically poled lithium niobate crystals

Measurements of photo-induced birefringence n single domain and periodically poled lithium niobate (LN) crystals containing different non-photorefractive impurities are presented. We find that doping by HfO/sub 2/ is very effective in reducing the photorefraction.

Integrated frequency comb source of heralded single photons

We report an integrated photon pair source based on a CMOS-compatible microring resonator that generates multiple, simultaneous, and independent photon pairs at different wavelengths in a frequency comb compatible with fiber communication wavelength division multiplexing channels (200 GHz channel separation) and with a linewidth that is compatible with quantum memories (110 MHz). It operates in a self-locked pump configuration, avoiding the need for active stabilization, making it extremely robust even at very low power levels.We report an integrated photon pair source based on a CMOS-compatible microring resonator that generates multiple, simultaneous, and independent photon pairs at different wavelengths in a frequency comb compatible with fiber communication wavelength division multiplexing channels (200 GHz channel separation) and with a linewidth that is compatible with quantum memories (110 MHz). It operates in a self-locked pump configuration, avoiding the need for active stabilization, making it extremely robust even at very low power levels.

Low power four wave mixing in an integrated, micro-ring resonator with Q = 1.2 million

We demonstrate efficient, low power, continuous-wave four-wave mixing in the C-band, using a high index doped silica glass micro ring resonator having a Q-factor of 1.2 million. A record high conversion efficiency for this kind of device is achieved over a bandwidth of 20 nm. We show theoretically that the characteristic low dispersion enables phase-matching over a tuning range > 160 nm.We demonstrate efficient, low power, continuous-wave fourwave mixing in the C-band, using a high index doped silica glass micro ring resonator having a Q-factor of 1.2 million. A record high conversion efficiency for this kind of device is achieved over a bandwidth of 20nm. We show theoretically that the characteristic low dispersion enables phasematching over a bandwidth > 160nm.

Efficient self-phase modulation in low loss, high index doped silica glass integrated waveguides

We demonstrate efficient self phase modulation, as well as negligible nonlinear absorption, in low loss (<0.06 dB/cm), high index silica glass-based waveguides. Using approximately 1 ps pulses near 1560 nm we achieve a 1.5pi nonlinear phase shift in an integrated 45 cm long spiral waveguide with <60 W of peak input power, corresponding to a large nonlinearity (gamma) of 220 W(-1)km(-1). Further, we observe negligible nonlinear absorption for input intensities > 25 GW/cm(2). The high nonlinearity and low linear and nonlinear losses of these waveguides make them promising for nonlinear all-optical signal processing applications.

Nonlinear ultrafast modulation of the optical absorption of intense few-cycle terahertz pulses in n-doped semiconductors

We use an open-aperture

Generation of Intense Terahertz Radiation via Optical Methods

Z