M. A. F. Silva Dias

Transport of biomass burning smoke to the upper troposphere by deep convection in the equatorial region

During LBA-CLAIRE-98, we found atmospheric layers with aged biomass smoke at altitudes >10 km over Suriname. CO, CO2, acetonitrile, methyl chloride, hydrocarbons, NO, O3, and aerosols were strongly enhanced in these layers. We estimate that 80-95% of accumulation mode aerosols had been removed during convective transport. Trajectories show that the plumes originated from large fires near the Brazil/Venezuela border during March 1998. This smoke was entrained into deep convection over the northern Amazon, transported out over the Pacific, and then returned to South America by the circulation around a large upper-level anticyclone. Our observations provide evidence for the importance of deep convection in the equatorial region as a mechanism to transport large amounts of pyrogenic pollutants into the upper troposphere. The entrainment of biomass smoke into tropical convective clouds may have significant effects on cloud microphysics and climate dynamics.

Sources and properties of Amazonian aerosol particles

This review provides a comprehensive account of what is known presently about Amazonian aerosol particles and concludes by formulating outlook and priorities for further research. The review is organized to follow the life cycle of Amazonian aerosol particles. It begins with a discussion of the primary and secondary sources relevant to the Amazonian particle burden, followed by a presentation of the particle properties that characterize the mixed populations present over the Amazon Basin at different times and places. These properties include number and mass concentrations and distributions, chemical composition, hygroscopicity, and cloud nucleation ability. The review presents Amazonian aerosol particles in the context of natural compared to anthropogenic sources as well as variability with season and meteorology. This review is intended to facilitate an understanding of the current state of knowledge on Amazonian aerosol particles specifically and tropical continental aerosol particles in general and thereby to enhance future research in this area. Copyright

THE SOUTH AMERICAN LOW-LEVEL JET EXPERIMENT

Abstract Moisture is transported in South America westward from the tropical Atlantic Ocean to the Amazon basin, and then southward toward the extratropics. A regional intensification of this circulation to the east of the Andes Mountains is called the South American low-level jet (SALLJ), with the strongest winds found over eastern Bolivia. SALLJ is present all year and channels moisture to the La Plata basin, which is analogous to the better-known Amazon basin in terms of its biological and habitat diversity, and far exceeds the latter in its economic importance to southern and central South America in terms of hydroelectricity and food production. The relatively small SALLJ spatial scale (compared with the density of the available sounding network) has a limited understanding of and modeling capability for any variations in the SALLJ intensity and structure as well as its possible relationship to downstream rainfall. The SALLJ Experiment (SALLJEX), aimed at describing many aspects of SALLJ, was carried...

A convective kinematic trajectory technique for low-resolution atmospheric models

This paper presents a simple methodology to take into account the subgrid effects of wet convective processes to trace vertical motion of air parcels for low-resolution atmospheric models. Such models are used for wind field simulations that serve as input for trajectory models. Air parcels in moist convective regions can thus be vertically transported to the cumulus top level with the short timescale associated with cumulus updrafts. Two cases are presented: wet and dry seasons in Amazonia, showing the differences of trajectories followed by air parcels with and without the methodology. The implications for the interpretation of air chemistry measurements are discussed, and an example using LBA/CLAIRE data is used to point out the usefulness of the convective kinematic trajectory technique presented here.

Impact of biomass burning aerosols on precipitation in the Amazon: A modeling case study

[1] A study of the potential role of aerosols in modifying clouds and precipitation is presented using a numerical atmospheric model. Measurements of cloud condensation nuclei (CCN) and cloud size distribution properties taken in the southwestern Amazon region during the transition from dry to wet seasons were used as guidelines to define the microphysical parameters for the simulations. Numerical simulations were carried out using the Brazilian Development on Regional Atmospheric Modeling System, and the results presented considerable sensitivity to changes in these parameters. High CCN concentrations, typical of polluted days, were found to result in increases or decreases in total precipitation, depending on the level of pollution used as a reference, showing a complexity that parallels the aerosol-precipitation interaction. Our results show that on the grids evaluated, higher CCN concentrations reduced low-to-moderate rainfall rates and increased high rainfall rates. The principal consequence of the increased pollution was a change from a warm to a cold rain process, which affected the maximum and overall mean accumulated precipitation. Under polluted conditions, cloud cover diminished, allowing greater amounts of solar radiation to reach the surface. Aerosol absorption of radiation in the lower layers of the atmosphere delayed convective evolution but produced higher maximum rainfall rates due to increased instability. In addition, the intensity of the surface sensible heat flux, as well as that of the latent heat flux, was reduced by the lower temperature difference between surface and air, producing greater energy stores at the surface.

The Green Ocean Amazon Experiment (GoAmazon2014/5) Observes Pollution Affecting Gases, Aerosols, Clouds, and Rainfall over the Rain Forest

AbstractThe Observations and Modeling of the Green Ocean Amazon 2014–2015 (GoAmazon2014/5) experiment took place around the urban region of Manaus in central Amazonia across 2 years. The urban pollution plume was used to study the susceptibility of gases, aerosols, clouds, and rainfall to human activities in a tropical environment. Many aspects of air quality, weather, terrestrial ecosystems, and climate work differently in the tropics than in the more thoroughly studied temperate regions of Earth. GoAmazon2014/5, a cooperative project of Brazil, Germany, and the United States, employed an unparalleled suite of measurements at nine ground sites and on board two aircraft to investigate the flow of background air into Manaus, the emissions into the air over the city, and the advection of the pollution downwind of the city. Herein, to visualize this train of processes and its effects, observations aboard a low-flying aircraft are presented. Comparative measurements within and adjacent to the plume followed t...

In-cloud and below-cloud numerical simulation of scavenging processes at Serra Do Mar region, SE Brazil

Abstract Atmospheric scavenging processes have been investigated, taking into consideration a numerical simulation through the model Regional Atmospheric Modeling System (RAMS), the below-cloud scavenging model, local atmospheric conditions and local emissions in the Serra do Mar region in southeastern Brazil. The RAMS modeling was coupled with a one-dimensional (1-D) below-cloud scavenging model in order to simulate the in-cloud and below-cloud scavenging processes. RAMS modeling was also used in order to simulate the cloud structures. The aim of the modeling was to predict the average concentration of three chemical species found in rainwater: SO 4 = , NO 3 − and NH 4 + , scavenged from the atmosphere. The concentrations of gases and particles in the samplings, as well as the meteorological parameters obtained during the March 1993 Campaign, were the input data in both models. Another objective was to compare the modeled and the observed rainwater and determine the variability in concentration. Rainwater was obtained by using fractionated rain samplers. Variability was determined through chemical analysis. Urban and rural aerosol spectra modeling were also used in order to compare the rainwater concentration species variability. When both in-cloud and below-cloud processes are included, the general result of the March 1993 events presents a better agreement between modeled and observed data sets than only below-cloud . Preliminary results lead us to conclude that the rainwater variability of nitrate is explained by the scavenging of particles from urban spectrum size distribution, whereas rural spectra explain ammonium rainwater variability—indicating the different sources of those species. Comparing to the March 1992 events, these case studies present a significant contribution from the in-cloud scavenging, supported by the Weather Radar maps and RAMS modeling. In particular, the almost constant rainwater concentrations on 16 March (an indication of strong in-cloud contribution) are related to the rainfall event, which crossed the study area on that day. These results add an important understanding to the atmospheric wet removal processes in the region studied.

Emissões de queimadas em ecossistemas da América do Sul

THE VEGETATION fires in tropical areas of the Earth are important sources of pollutants to the atmosphere. In South America, during the winter months, an area, mainly of cerrado and forest ecosystems, of approximately 40 thousand square kilometers is burned annually. The biomass burning occurs primarily in Amazon and Central of Brazil regions, but through atmospheric transport these emissions results in a spatial distribution of smoke over an extent area, of about 4-5 millions of square kilometers, much higher than the area where the fires are concentrated. During the combustion process are emitted to the atmosphere gases pollutants and aerosol particles that interact efficiently with radiation, microphysics process, dynamic of cloud formation and the air quality. The effects of these emissions exceed, therefore, the local scale and affect regionally the composition and physical and chemical properties of the South America atmosphere and neighborhood oceanic areas, with potential impact in a global scale.

Impacts of Agulhas Leakage on the Tropical Atlantic western boundary systems

AbstractThe influx of warmer and saltier Indian Ocean waters into the Atlantic—the Agulhas leakage—is now recognized to play an important role in the global thermohaline circulation and climate. In this study the results of a ⅞° simulation with the Hybrid Coordinate Ocean Model, which exhibit an augmentation in the Agulhas leakage, is investigated. This increase in the leakage ought to have an impact on the meridional oceanic volume and heat transports in the Atlantic Ocean. Significant linear trends found in the integrated transport at 20°, 15°, and 5°S correlate well with decadal fluctuations of the Agulhas leakage. The augmented transport also seems to be related to an increase in the latent heat flux observed along the northeastern coastline of Brazil since 2003. This study shows that the precipitation on the Brazilian coast has been increasing since 2005, at the same location and with the same regime shift observed for the latent heat flux and the volume transport. This suggests that the increase of ...