M. Aliotta

Enhanced electron screening in d(d, p)t for deuterated Ta

Abstract:The recent observation of a large electron screening effect in the d(d, p)t reaction using a deuterated Ta target has been confirmed using somewhat different experimental approaches: Ue = 309±12 eV for the electron screening potential energy. The high Ue value arises from the environment of the deuterons in the Ta matrix, but a quantitative explanation is missing.

Electron screening effect in the reactions 3He(d, p)4He and d(3He, p)4He

The cross section of the reactions 3He(d, p)4He and d(3He, p)4He has been measured at the center-of-mass energies E=5 to 60 keV and 10 to 40 keV, respectively. The experiments were performed to determine the magnitude of the electron screening effect leading to the respective electron-screening potential energy Ue=219±7 and 109±9 eV, which are both significantly higher than the respective values from atomic physics models, Ue=120 and 65 eV.

Electron screening effect in the reactions 3 He(d, p) 4 He and d( 3 He, p) 4 He ☆ ☆ Supported in part by INFN, BMBF (06BO812), DFG (436UNG113-146) and OTKA (T025465).

The cross section of the reactions 3He(d, p)4He and d(3He, p)4He has been measured at the center-of-mass energies E=5 to 60 keV and 10 to 40 keV, respectively. The experiments were performed to determine the magnitude of the electron screening effect leading to the respective electron-screening potential energy Ue=219±7 and 109±9 eV, which are both significantly higher than the respective values from atomic physics models, Ue=120 and 65 eV.

Enhanced electron screening in d(d, p)t for deuterated metals: a possible classical explanation

Abstract The electron screening effect in the d(d, p)t reaction has been studied for several deuterated metals and insulators/semiconductors. As compared to measurements performed with a gaseous D 2 target, a large effect has been observed in all metals except in the noble metals Cu, Ag, and Au. In contrast, a comparatively small effect is found for the insulators and semiconductors. An explanation of the large effect in metals is possibly provided by the classical plasma screening of Debye applied to the quasi-free metallic electrons.

Electron screening in d(d, p)t for deuterated metals: temperature effects

The electron screening in the d(d, p)t reaction has been studied for the deuterated metal Pt at a sample temperature T = 20 °C–340 °C and for Co at T = 20 °C and 200 °C. The enhanced electron screening decreases with increasing temperature, where the data agree with the plasma model of Debye applied to the quasi-free metallic electrons. The data represent the first observation of a temperature dependence of a nuclear cross section. We also measured the screening effect for the deuterated metal Ti (an element of group 4 of the periodic table) at T = −10 °C–200 °C: above 50 °C, the hydrogen solubility dropped to values far below 1 and a large screening effect became observable. Similarly, all metals of groups 3 and 4 and the lanthanides showed a solubility of a few per cent at T = 200 °C (compared to T = 20 °C) and a large screening also became observable. Within the Debye model, the deduced number of valence electrons per metallic atom agrees with the corresponding number from the Hall coefficient, for all metals investigated.

First Direct Measurement of the 17O(p,γ)18F Reaction Cross Section at Gamow Energies for Classical Novae

Classical novae are important contributors to the abundances of key isotopes, such as the radioactive (18)F, whose observation by satellite missions could provide constraints on nucleosynthesis models in novae. The (17)O(p,γ)(18)F reaction plays a critical role in the synthesis of both oxygen and fluorine isotopes, but its reaction rate is not well determined because of the lack of experimental data at energies relevant to novae explosions. In this study, the reaction cross section has been measured directly for the first time in a wide energy range E(c.m.)~/= 200-370 keV appropriate to hydrogen burning in classical novae. In addition, the E(c.m.)=183 keV resonance strength, ωγ=1.67±0.12 μeV, has been measured with the highest precision to date. The uncertainty on the (17)O(p,γ)(18)F reaction rate has been reduced by a factor of 4, thus leading to firmer constraints on accurate models of novae nucleosynthesis.

Experimental study of proton-induced nuclear reactions in 6,7 Li

The 6Li(p,α)3He and 7Li(p,α)4He reaction cross sections were obtained for E = 90–580 keV and E = 90–1740 keV, respectively. R-matrix and polynomial fits to the bare astrophysical S-factor confirmed, with improved accuracy, previous work data, yielding Sb(0) = 3.52 ± 0.08 MeV b, and 55.6+0.8−1.7 keV b for the 6Li and 7Li reactions, respectively. Therefore, the astrophysical consequences related to these two isotopes remain essentially unchanged. With the present work Sb(E) data, a reanalysis of the low energy data for different environments—Li2WO4 insulator, Li metal, and PdLix alloys—confirms that the large electron screening effects can be explained by the plasma model of Debye applied to the quasi-free electrons in the metallic samples.

Neutron-induced background by an α-beam incident on a deuterium gas target and its implications for the study of the 2H(α, γ)6Li reaction at LUNA

Abstract.The production of the stable isotope 6Li in standard Big Bang nucleosynthesis has recently attracted much interest. Recent observations in metal-poor stars suggest that a cosmological 6Li plateau may exist. If true, this plateau would come in addition to the well-known Spite plateau of 7Li abundances and would point to a predominantly primordial origin of 6Li , contrary to the results of standard Big Bang nucleosynthesis calculations. Therefore, the nuclear physics underlying Big Bang 6Li production must be revisited. The main production channel for 6Li in the Big Bang is the 2H(α,γ)6Li reaction. The present work reports on neutron-induced effects in a high-purity germanium detector that were encountered in a new study of this reaction. In the experiment, an α-beam from the underground accelerator LUNA in Gran Sasso, Italy, and a windowless deuterium gas target are used. A low neutron flux is induced by energetic deuterons from elastic scattering and, subsequently, the 2H(d,n)3He reaction. Due to the ultra-low laboratory neutron background at LUNA, the effect of this weak flux of 2-3MeV neutrons on well-shielded high-purity germanium detectors has been studied in detail. Data have been taken at 280 and 400keV α-beam energy and for comparison also using an americium-beryllium neutron source.

Preparation and characterisation of isotopically enriched Ta2O5 targets for nuclear astrophysics studies

The direct measurement of reaction cross-sections at astrophysical energies often requires the use of solid targets of known thickness, isotopic composition, and stoichiometry that are able to withstand high beam currents for extended periods of time. Here, we report on the production and characterisation of isotopically enriched Ta2O5 targets for the study of proton-induced reactions at the Laboratory for Underground Nuclear Astrophysics facility of the Laboratori Nazionali del Gran Sasso. The targets were prepared by anodisation of tantalum backings in enriched water (up to 66% in 17O and up to 96% in 18O. Special care was devoted to minimising the presence of any contaminants that could induce unwanted background reactions with the beam in the energy region of astrophysical interest. Results from target characterisation measurements are reported, and the conclusions for proton capture measurements with these targets are drawn.

A new study of the 22Ne(p, γ)23Na reaction deep underground: Feasibility, setup and first observation of the 186 keV resonance

The 22Ne(p,γ)23Na reaction takes part in the neon-sodium cycle of hydrogen burning. This cycle is active in asymptotic giant branch stars as well as in novae and contributes to the nucleosythesis of neon and sodium isotopes. In order to reduce the uncertainties in the predicted nucleosynthesis yields, new experimental efforts to measure the 22Ne(p,γ)23Na cross section directly at the astrophysically relevant energies are needed. In the present work, a feasibility study for a 22Ne(p,γ)23Na experiment at the Laboratory for Underground Nuclear Astrophysics (LUNA) 400 kV accelerator deep underground in the Gran Sasso laboratory, Italy, is reported. The ion-beam-induced γ-ray background has been studied. The feasibility study led to the first observation of the Ep=186 keV resonance in a direct experiment. An experimental lower limit of 0.12 × 10−6 eV has been obtained for the resonance strength. Informed by the feasibility study, a dedicated experimental setup for the 22Ne(p,γ)23Na experiment has been developed. The new setup has been characterized by a study of the temperature and pressure profiles. The beam heating effect that reduces the effective neon gas density due to the heating by the incident proton beam has been studied using the resonance scan technique, and the size of this effect has been determined for a neon gas target.