M. Kronseder

Entropy-limited topological protection of skyrmions

Entropic effects counteract the topological protection of magnetic skyrmions, leading to faster decay rates than expected. Magnetic skyrmions are topologically protected whirls that decay through singular magnetic configurations known as Bloch points. We used Lorentz transmission electron microscopy to infer the energetics associated with the topological decay of magnetic skyrmions far from equilibrium in the chiral magnet Fe1−xCoxSi. We observed that the lifetime τ of the skyrmions depends exponentially on temperature, τ~τ0 exp(ΔEkBT). The prefactor τ0 of this Arrhenius law changes by more than 30 orders of magnitude for small changes of the magnetic field, reflecting a substantial reduction of the lifetime of skyrmions by entropic effects and, thus, an extreme case of enthalpy-entropy compensation. Such compensation effects, being well known across many different scientific disciplines, affect topological transitions and, thus, topological protection on an unprecedented level.

Robust spin-orbit torque and spin-galvanic effect at the Fe/GaAs (001) interface at room temperature

Interfacial spin-orbit torques (SOTs) enable the manipulation of the magnetization through in-plane charge currents, which has drawn increasing attention for spintronic applications. The search for material systems providing efficient SOTs, has been focused on polycrystalline ferromagnetic metal/non-magnetic metal bilayers. In these systems, currents flowing in the non-magnetic layer generate—due to strong spin–orbit interaction—spin currents via the spin Hall effect and induce a torque at the interface to the ferromagnet. Here we report the observation of robust SOT occuring at a single crystalline Fe/GaAs (001) interface at room temperature. We find that the magnitude of the interfacial SOT, caused by the reduced symmetry at the interface, is comparably strong as in ferromagnetic metal/non-magnetic metal systems. The large spin-orbit fields at the interface also enable spin-to-charge current conversion at the interface, known as spin-galvanic effect. The results suggest that single crystalline Fe/GaAs interfaces may enable efficient electrical magnetization manipulation.

Dipolar-energy-activated magnetic domain pattern transformation driven by thermal fluctuations

Two-dimensional ferromagnetic layers can serve as a playground for the study of basic physical properties of various pattern forming systems by virtue of their tuneable magnetic properties. Here we use threshold photoemission magnetic circular dichroism in combination with photoemission electron microscopy to investigate ultra-thin ferromagnetic Fe/Ni/Cu(001) films in the stripe domain phase near the spin reorientation transition as a function of film thickness, temperature and effective anisotropy. Here we report a metastable domain state with domain width larger than the thermodynamically stable one as a result of a rapid reduction of the anisotropy. The transformation into the equilibrium state takes place via the propagation of a transition front, which originates from defined steps in the film thickness.

Real-time observation of domain fluctuations in a two-dimensional magnetic model system

Domain patterns of perpendicularly magnetized ultra-thin ferromagnetic films are often determined by the competition of the short range but strong exchange interaction favouring ferromagnetic alignment of magnetic moments and the long range but weak antiferromagnetic dipolar interaction. Detailed phase diagrams of the resulting stripe domain patterns have been evaluated in recent years; however, the domain fluctuations in these pattern forming systems have not been studied in great detail so far. Here we show that domain fluctuations can be observed in ultra-thin two-dimensional ferromagnetic Fe/Ni/Cu(001) films with perpendicular magnetization in the stripe domain phase. Non-stroboscopic time-resolved threshold photoemission electron microscopy with high temporal resolution allows analysing the dynamic fingerprint of the topological excitations in the nematic domain phase. Furthermore, proliferation of domain ending defects in the vicinity of the spin reorientation transition is witnessed.

Time Resolved Measurements of the Switching Trajectory of Pt/Co Elements Induced by Spin-Orbit Torques

We report the experimental observation of spin-orbit torque induced switching of perpendicularly magnetized Pt/Co elements in a time resolved stroboscopic experiment based on high resolution Kerr microscopy. Magnetization dynamics is induced by injecting subnanosecond current pulses into the bilayer while simultaneously applying static in-plane magnetic bias fields. Highly reproducible homogeneous switching on time scales of several tens of nanoseconds is observed. Our findings can be corroborated using micromagnetic modeling only when including a fieldlike torque term as well as the Dzyaloshinskii-Moriya interaction mediated by finite temperature.

Co-sputtered MoRe thin films for carbon nanotube growth-compatible superconducting coplanar resonators

Molybdenum rhenium alloy thin films can exhibit superconductivity up to critical temperatures of T(c)=15K. At the same time, the films are highly stable in the high-temperature methane/hydrogen atmosphere typically required to grow single wall carbon nanotubes. We characterize molybdenum rhenium alloy films deposited via simultaneous sputtering from two sources, with respect to their composition as function of sputter parameters and their electronic dc as well as GHz properties at low temperature. Specific emphasis is placed on the effect of the carbon nanotube growth conditions on the film. Superconducting coplanar waveguide resonators are defined lithographically; we demonstrate that the resonators remain functional when undergoing nanotube growth conditions, and characterize their properties as function of temperature. This paves the way for ultra-clean nanotube devices grown in situ onto superconducting coplanar waveguide circuit elements.

Origin and Manipulation of Stable Vortex Ground States in Permalloy Nanotubes

We present a detailed study on the static magnetic properties of individual permalloy nanotubes (NTs) with hexagonal cross-sections. Anisotropic magnetoresistance (AMR) measurements and scanning transmission X-ray microscopy (STXM) are used to investigate their magnetic ground states and its stability. We find that the magnetization in zero applied magnetic field is in a very stable vortex state. Its origin is attributed to a strong growth-induced anisotropy with easy axis perpendicular to the long axis of the tubes. AMR measurements of individual NTs in combination with micromagnetic simulations allow the determination of the magnitude of the growth-induced anisotropy for different types of NT coatings. We show that the strength of the anisotropy can be controlled by introducing a buffer layer underneath the magnetic layer. The magnetic ground states depend on the external magnetic field history and are directly imaged using STXM. Stable vortex domains can be introduced by external magnetic fields and can be erased by radio-frequency magnetic fields applied at the center of the tubes via a strip line antenna.

Magnetic damping in poly-crystalline Co25Fe75: Ferromagnetic resonance vs. spin wave propagation experiments

We report on the investigation of the magnetic damping of a 10 nm thin, poly-crystalline Co25Fe75 film grown by molecular beam epitaxy. Ferromagnetic resonance (FMR) measurements reveal a low intrinsic magnetic damping αintFMR=(1.5±0.1)×10−3. In contrast, in patterned micrometer wide stripes, spin wave (SW) propagation experiments performed by time resolved scanning magneto-optical Kerr microscopy yield attenuation lengths on the order of 5–8 μm. From this quantity, we deduce an effective magnetic SW damping αeffSW, exp =(3.9±0.3)×10−3. For the system studied, this significant difference between both damping parameters is attributed to the non-negligible extrinsic contributions (local inhomogeneities and two-magnon scattering) to the magnetic losses which manifest themselves as a distinct inhomogeneous FMR linewidth broadening. This explanation is supported by micromagnetic simulations. Our findings prove that poly-crystalline Co25Fe75 represents a promising binary 3d transition metal alloy to be employed in magnonic devices with much longer SW attenuation lengths compared to other metallic systems.We report on the investigation of the magnetic damping of a 10 nm thin, poly-crystalline Co25Fe75 film grown by molecular beam epitaxy. Ferromagnetic resonance (FMR) measurements reveal a low intrinsic magnetic damping αintFMR=(1.5±0.1)×10−3. In contrast, in patterned micrometer wide stripes, spin wave (SW) propagation experiments performed by time resolved scanning magneto-optical Kerr microscopy yield attenuation lengths on the order of 5–8 μm. From this quantity, we deduce an effective magnetic SW damping αeffSW, exp =(3.9±0.3)×10−3. For the system studied, this significant difference between both damping parameters is attributed to the non-negligible extrinsic contributions (local inhomogeneities and two-magnon scattering) to the magnetic losses which manifest themselves as a distinct inhomogeneous FMR linewidth broadening. This explanation is supported by micromagnetic simulations. Our findings prove that poly-crystalline Co25Fe75 represents a promising binary 3d transition metal alloy to be employ...