M. V. Romalis

NMR detection with an atomic magnetometer.

We demonstrate detection of NMR signals using a noncryogenic atomic magnetometer and describe several novel applications of this technique. A nuclear spin-precession signal from water is detected using a spin-exchange-relaxation-free potassium magnetometer. We also demonstrate detection of less than 10(13) 129Xe atoms whose NMR signal is enhanced by a factor of 540 due to Fermi-contact interaction with K atoms. The possibility of using a multichannel atomic magnetometer for fast 3D magnetic resonance imaging is also discussed.

Nuclear spin gyroscope based on an atomic comagnetometer.

We describe a nuclear spin gyroscope based on an alkali-metal-noble-gas comagnetometer. Optically pumped alkali-metal vapor is used to polarize the noble-gas atoms and detect their gyroscopic precession. Spin precession due to magnetic fields as well as their gradients and transients can be cancelled in this arrangement. The sensitivity is enhanced by using a high-density alkali-metal vapor in a spin-exchange relaxation free regime. With a K-3He comagnetometer we demonstrate rotation sensitivity of 5 x 10(-7) rad s(-1) Hz(-1/2), equivalent to a magnetic field sensitivity of 2.5 fT/Hz(1/2). The rotation signal can be increased by a factor of 10 using 21Ne with a smaller magnetic moment. The comagnetometer is also a promising tool in searches for anomalous spin couplings beyond the standard model.

Unshielded three-axis vector operation of a spin-exchange-relaxation-free atomic magnetometer

We describe a vector alkali–metal magnetometer that simultaneously and independently measures all three components of the magnetic field. Using a feedback system, the total field at the location of the magnetometer is kept near zero, suppressing the broadening due to spin-exchange collisions. The resonance linewidth and signal strength of the magnetometer compare favorably with two different scalar operation modes in which spin-exchange relaxation is only partially suppressed. Magnetic field sensitivity on the order of 1pT∕Hz is demonstrated in a laboratory environment without magnetic shields.

Subfemtotesla radio-frequency atomic magnetometer for detection of nuclear quadrupole resonance

A radio-frequency tunable atomic magnetometer is developed for detection of nuclear quadrupole resonance (NQR) from room temperature solids. It has a field sensitivity 0.24fT∕Hz1∕2 at the 423kHz N14 NQR frequency of ammonium nitrate. A potential application of the magnetometer is detection of nitrogen-containing explosives which is difficult with conventional tuned copper coils due to a poor signal-to-noise ratio (SNR) below a few megahertz. The NQR signal from 22g of powdered ammonium nitrate located 2cm away from the sensor is detected with a SNR of 9 in a 4.4-s-long multiple echo sequence, which represents an estimated order-of-magnitude improvement in sensitivity over the pickup coil detection.

New limit on Lorentz- and CPT-violating neutron spin interactions.

We performed a search for neutron spin coupling to a Lorentz- and CPT-violating background field using a magnetometer with overlapping ensembles of K and ³He atoms. The comagnetometer is mounted on a rotary platform for frequent reversal of its orientation. We measure sidereal oscillations in the signal to search for anomalous spin coupling of extra-solar origin. We determine the equatorial components of the background field interacting with the neutron spin to be b˜Xn=(0.1 ± 1.6) × 10⁻³³ GeV and b˜Yn=(2.5 ± 1.6) × 10⁻³³ GeV, improving on the previous limit by a factor of 30. This measurement represents the highest energy resolution of any spin anisotropy experiment.

New test of local Lorentz invariance using a 21Ne-Rb-K comagnetometer.

We develop a new comagnetometer using (21)Ne atoms with nuclear spin I=3/2 and Rb atoms polarized by spin exchange with K atoms to search for tensor interactions that violate local Lorentz invariance. We frequently reverse the orientation of the experiment and search for signals at the first and second harmonics of the sidereal frequency. We constrain 4 of the 5 spatial Lorentz-violating coefficients c(jk)(n) that parametrize anisotropy of the maximum attainable velocity of a neutron at a level of 10(-29), improving previous limits by 2 to 4 orders of magnitude and placing the most stringent constraint on deviations from local Lorentz invariance.

A low-noise ferrite magnetic shield

Ferrite materials provide magnetic shielding performance similar to commonly used high permeability metals but have lower intrinsic magnetic noise generated by thermal Johnson currents due to their high electrical resistivity. Measurements inside a ferrite shield with a spin-exchange relaxation-free atomic magnetometer reveal a noise level of 0.75fTHz−1∕2, 25 times lower than what would be expected in a comparable μ-metal shield. The authors identify a 1∕f component of the magnetic noise due to magnetization fluctuations and derive general relationships for the Johnson current noise and magnetization noise in cylindrical ferromagnetic shields in terms of their conductivity and complex magnetic permeability.

Limits on new long range nuclear spin-dependent forces set with a K-3He comagnetometer.

A magnetometer using spin-polarized K and 3He atoms occupying the same volume is used to search for anomalous nuclear spin-dependent forces generated by a separate 3He spin source. We measure changes in the 3He spin precession frequency with a resolution of 18 pHz and constrain anomalous spin forces between neutrons to be less than 2x10(-8) of their magnetic or less than 2x10(-3) of their gravitational interactions on a length scale of 50 cm. We present new limits on neutron coupling to light pseudoscalar and vector particles, including torsion, and constraints on recently proposed models involving unparticles and spontaneous breaking of Lorentz symmetry.

High Bandwidth Atomic Magnetometery with Continuous Quantum Nondemolition Measurements

We describe an experimental study of spin-projection noise in a high sensitivity alkali-metal magnetometer. We demonstrate a fourfold improvement in the measurement bandwidth of the magnetometer using continuous quantum nondemolition measurements. Operating in the scalar mode with a measurement volume of 2 cm3 we achieve magnetic field sensitivity of 22 fT/Hz(1/2) and a bandwidth of 1.9 kHz with a spin polarization of only 1%. Our experimental arrangement is naturally backaction evading and can be used to realize sub-fT sensitivity with a highly polarized spin-squeezed atomic vapor.

Stroboscopic backaction evasion in a dense alkali-metal vapor.

We explore experimentally quantum nondemolition measurements of atomic spin in a hot potassium vapor in the presence of spin-exchange relaxation. We demonstrate a new technique for backaction evasion by stroboscopic modulation of the probe light. With this technique we study spin noise as a function of polarization for atoms with spin greater than 1/2 and obtain good agreement with a simple theoretical model. We point that, in a system with fast spin exchange, where the spin-relaxation rate is changing with time, it is possible to improve the long-term sensitivity of atomic magnetometry by using quantum nondemolition measurements.