Matthias Widmann

Coherent control of single spins in silicon carbide at room temperature

Spins in solids are cornerstone elements of quantum spintronics. Leading contenders such as defects in diamond or individual phosphorus dopants in silicon have shown spectacular progress, but either lack established nanotechnology or an efficient spin/photon interface. Silicon carbide (SiC) combines the strength of both systems: it has a large bandgap with deep defects and benefits from mature fabrication techniques. Here, we report the characterization of photoluminescence and optical spin polarization from single silicon vacancies in SiC, and demonstrate that single spins can be addressed at room temperature. We show coherent control of a single defect spin and find long spin coherence times under ambient conditions. Our study provides evidence that SiC is a promising system for atomic-scale spintronics and quantum technology.

Readout and control of a single nuclear spin with a metastable electron spin ancilla

Electron and nuclear spins associated with point defects in insulators are promising systems for solid-state quantum technology. The electron spin is usually used for readout and addressing, and nuclear spins are used as exquisite quantum bits and memory systems. With these systems, single-shot readout of single nuclear spins as well as entanglement, aided by the electron spin, have been shown. Although the electron spin in this example is essential for readout, it usually limits the nuclear spin coherence, leading to a quest for defects with spin-free ground states. Here, we isolate a hitherto unidentified defect in diamond and use it at room temperature to demonstrate optical spin polarization and readout with exceptionally high contrast (up to 45%), coherent manipulation of an individual excited triplet state spin, and coherent nuclear spin manipulation using the triplet electron spin as a metastable ancilla. We demonstrate nuclear magnetic resonance and Rabi oscillations of the uncoupled nuclear spin in the spin-free electronic ground state. Our study demonstrates that nuclei coupled to single metastable electron spins are useful quantum systems with long memory times, in spite of electronic relaxation processes.

Scalable quantum photonics with single color centers in silicon carbide

We develop a scalable array of 4H-SiC nanopillars incorporating single silicon vacancy centers, readily available to serve as efficient single photon sources or quantum bits interfaced with free-space or lensed-fiber optics.

Vector Magnetometry Using Silicon Vacancies in 4 H -SiC Under Ambient Conditions

The spins of point defects in silicon carbide are promising candidates for qubits and sensors under

Simultaneous Faraday filtering of the Mollow triplet sidebands with the Cs-D1 clock transition.

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Bright single photon sources in lateral silicon carbide light emitting diodes

conditions. Unlike defect-bearing diamond, SiC is regarded as an industry-friendly platform, with an existing market for high-purity SiC wafers and a mature fabrication technology. The authors detect the magnitude and direction of a magnetic field using magnetic resonance with optical readout of the spin-3/2 states of silicon-vacancy defects in SiC, plus optimized pulse sequences for spin manipulation. This yields a solid-state quantum vector magnetometer in a material available for wafer-scale production.

Quantum dots interfaced with alkali atoms: Filtering, delaying and quantum interfering single photons

Hybrid quantum systems integrating semiconductor quantum dots (QDs) and atomic vapours become important building blocks for scalable quantum networks due to the complementary strengths of individual parts. QDs provide on-demand single-photon emission with near-unity indistinguishability comprising unprecedented brightness—while atomic vapour systems provide ultra-precise frequency standards and promise long coherence times for the storage of qubits. Spectral filtering is one of the key components for the successful link between QD photons and atoms. Here we present a tailored Faraday anomalous dispersion optical filter based on the caesium-D1 transition for interfacing it with a resonantly pumped QD. The presented Faraday filter enables a narrow-bandwidth (Δω=2π × 1 GHz) simultaneous filtering of both Mollow triplet sidebands. This result opens the way to use QDs as sources of single as well as cascaded photons in photonic quantum networks aligned to the primary frequency standard of the caesium clock transition.

Quantum Properties of Dichroic Silicon Vacancies in Silicon Carbide

Single-photon emitting devices have been identified as an important building block for applications in quantum information and quantum communication. They allow to transduce and collect quantum information over a long distance via photons as so called flying qubits. In addition, substrates like silicon carbide provides an excellent material platform for electronic devices. In this work we combine these two features and show that one can drive single photon emitters within a silicon carbide p-i-n-diode. To achieve this, we specifically designed a lateral oriented diode. We find a variety of new color centers emitting non-classical lights in VIS and NIR range. One type of emitter can be electrically excited, demonstrating that silicon carbide can act as an ideal platform for electrically controllable single photon sources.

Faraday Filtering on the Cs-D1-Line for Quantum Hybrid Systems

Hybrid quantum systems are based on the capability to interface elements from complementary fields: only the best properties from all components are utilized, overcoming the limitation of each field. Semiconductor quantum dots (QDs) are well established as sources of bright, pure and highly indistinguishable on-demand single photons. A crucial limitation is given by the relatively short coherence time. This can be overtaken by interfacing them to alkali atoms, which display a very long coherence time and will benefit from the superior properties of QD-based non-classical light sources [1].