Michael Grøndahl Nielsen

Broadband Focusing Flat Mirrors Based on Plasmonic Gradient Metasurfaces

We demonstrate that metal-insulator-metal configurations, with the top metal layer consisting of a periodic arrangement of differently sized nanobricks, can be designed to function as broadband focusing flat mirrors. Using 50-nm-high gold nanobricks arranged in a 240-nm-period lattice on the top of a 50-nm-thick layer of silicon dioxide deposited on a continuous 100-nm-thick gold film, we realize a 17.3 × 17.3 μm(2) flat mirror that efficiently reflects (experiment: 14-27%; theory: 50-78%) and focuses a linearly polarized (along the direction of nanobrick size variation) incident beam in the plane of its polarization with the focal length, which changes from ~15 to 11 μm when tuning the light wavelength from 750 to 950 nm, respectively. Our approach can easily be extended to realize the radiation focusing in two dimensions as well as other optical functionalities by suitably controlling the phase distribution of reflected light.

Efficient absorption of visible radiation by gap plasmon resonators

We demonstrate experimentally a periodic array of differently-sized and circularly-shaped gap plasmon resonators (GPRs) with the average absorption ~94% for unpolarized light in the entire visible wavelength range (400-750 nm). Finite-element simulations verify that the polarization insensitive broadband absorption originates from localized gap surface plasmons whose resonant excitations only weakly depend on the angle of incidence. Arrays of GPRs also exhibit enhanced local field intensities (~115) as revealed by scanning two-photon photoluminescence microscopy, that are spectrally correlated with the minima in corresponding linear reflection spectra.

Plasmonic metamaterial wave retarders in reflection by orthogonally oriented detuned electrical dipoles

We demonstrate that a pair of perpendicular electrical dipolar scatterers resonating at different frequencies can be used as a metamaterial unit cell to construct a nanometer-thin retarder in reflection, designing nanocross and nanobrick plasmonic configurations to function as reflecting quarter-wave plates at ~1520 and 770 nm, respectively. The design is corroborated experimentally with a monolayer of gold nanobricks, transforming linearly polarized incident radiation into circularly polarized radiation at ~780 nm.

Broadband plasmonic half-wave plates in reflection

We demonstrate, both numerically and experimentally, that metal-insulator-metal configurations in which the top metal layer consists of a periodic arrangement of nanobricks, thus supporting gap-surface plasmon resonances, can be designed to function as reflective broadband half-wave plates. Using gold as the metal, the constructed wave plates in the near-infrared regime show scalability, bandwidth of ~20% of the design wavelength, and theoretical reflectivity above 85%, while a reflectivity of ~50% is experimentally measured.

Plasmonic metagratings for simultaneous determination of Stokes parameters

Measuring lights state of polarization is an inherently difficult problem, since the phase information between orthogonal polarization states is typically lost in the detection process. In this work, we bring to the fore the equivalence between normalized Stokes parameters and diffraction contrasts in appropriately designed phase-gradient birefringent metasurfaces and introduce a concept of all-polarization birefringent metagratings. The metagrating, which consists of three interweaved metasurfaces, allows one to easily analyze an arbitrary state of light polarization by conducting simultaneous (i.e., parallel) measurements of the correspondent diffraction intensities that reveal immediately the Stokes parameters of the polarization state under examination. Based on plasmonic metasurfaces operating in reflection at the wavelength of 800 nm, we design and realize phase-gradient birefringent metasurfaces and the correspondent metagrating, while experimental characterization of the fabricated components convincingly demonstrates the expected functionalities. We foresee the use of the metagrating in compact polarimetric setups at any frequency regime of interest.

Detuned Electrical Dipoles for Plasmonic Sensing

We demonstrate that a pair of electrical dipolar scatterers resonating at different frequencies, i.e., detuned electrical dipoles, can be advantageously employed for plasmonic sensing of the environment, both as an individual subwavelength-sized sensor and as a unit cell of a periodic array. It is shown that the usage of the ratio between the powers of light scattered into opposite directions (or into different diffraction orders), which peaks at the intermediate frequency, allows one to reach a sensitivity of ≈ 400 nm/RIU with record high levels of figure of merit exceeding 200. Qualitative considerations are supported with detailed simulations and proof-of-principle experiments using lithographically fabricated gold nanorods with resonances at 800 nm.

Long-range dielectric-loaded surface plasmon polariton waveguides operating at telecommunication wavelengths

We report on the realization of long-range dielectric-loaded surface plasmon polariton waveguides (LR-DLSPPWs) consisting of straight and bent subwavelength dielectric ridges deposited on thin and narrow metal stripes supported by a dielectric buffer layer covering a low-index substrate. Using imaging with a near-field optical microscope and end-fire coupling with a tapered fiber connected to a tunable laser at telecommunication wavelengths (1425-1545 nm), we demonstrate low-loss (propagation length ∼500 μm) and well-confined (mode width ∼1 μm) LR-DLSPPW mode guiding and determine the propagation and bend loss.

Analog computing using reflective plasmonic metasurfaces

Motivated by the recent renewed interest in compact analog computing using light and metasurfaces ( Silva, A. et al. Science 2014 , 343, 160 - 163), we suggest a practical approach to its realization that involves reflective metasurfaces consisting of arrayed gold nanobricks atop a subwavelength-thin dielectric spacer and optically thick gold film, a configuration that supports gap-surface plasmon resonances. Using well-established numerical routines, we demonstrate that these metasurfaces enable independent control of the light phase and amplitude, and design differentiator and integrator metasurfaces featuring realistic system parameters. Proof-of-principle experiments are reported along with the successful realization of a high-quality poor-mans integrator metasurface operating at the wavelength of 800 nm.

Continuous layer gap plasmon resonators.

We demonstrate both theoretically and experimentally that a gold nanostrip supported by a thin dielectric (silicon dioxide) film and a gold underlay forms an efficient (Fabry-Perot) resonator for gap surface plasmons. Periodic nanostrip arrays are shown to exhibit strong and narrow resonances with nearly complete absorption and quality factors of ~15-20 in the near-infrared. Two-photon luminescence microscopy measurements reveal intensity enhancement factors of ~120 in the 400-nm-period array of 85-nm-wide gold strips atop a 23-nm-thick silica film at the resonance wavelength of ~770 nm. Excellent resonant characteristics, the simplicity of tuning the resonance wavelength by adjusting the nanostrip width and/or the dielectric film thickness and the ease of fabrication with (only) one lithography step required make the considered plasmonic configuration very attractive for a wide variety of applications, ranging from surface sensing to photovoltaics.

Stimulated emission of surface plasmon polaritons by lead-sulphide quantum dots at near infra-red wavelengths.

Amplification of surface plasmon polaritons in planar metal-dielectric structure through stimulated emission is investigated using leakage-radiation microscopy configuration. The gain medium is a thin polymethylmethacrylate layer doped with lead-sulphide nanocrystals emitting at near-infrared wavelengths. We demonstrate an optical gain of ~200 cm(-1) for the mode under consideration, which corresponds to ~32% compensation of SPP loss.