Ming K. Tan

Particle concentration and mixing in microdrops driven by focused surface acoustic waves

We report the use of focused surface acoustic waves (SAWs) generated on 128° rotated Y-cut X-propagating lithium niobate (LiNbO3) for enhancing the actuation of fluids and the manipulation of particle suspensions at microscale dimensions. In particular, we demonstrate increased efficiency and speed in carrying out particle concentration/separation and in generating intense micromixing in microliter drops within which acoustic streaming is induced due to the focused SAW beneath the drop. Concentric circular and elliptical single-phase unidirectional transducers (SPUDTs) were used to focus the SAW. We benchmark our results against a straight SPUDT which does not cause focusing of the SAW. Due to the increased wave intensity and asymmetry of the wave, we found both circular and elliptical SPUDTs concentrate particles in under 1 s, which is one order of magnitude faster than the straight SPUDT and several orders of magnitude faster than conventional microscale devices. The concentric circular SPUDT was found ...

Microparticle collection and concentration via a miniature surface acoustic wave device

The ability to detect microbes, pollens and other microparticles is a critically important ability given the increasing risk of bioterrorism and emergence of antibiotic-resistant bacteria. The efficient collection of microparticles via a liquid water droplet moved by a surface acoustic wave (SAW) device is demonstrated in this study. A fluidic track patterned on the SAW device directs the water droplets motion, and fluid streaming induced inside the droplet as it moves along is a key advantage over other particle collection approaches, because it enhances microparticle collection and concentration. Test particles consisted of 2, 10, 12 and 45 microm diameter monodisperse polystyrene and melamine microparticles; pollen from the Populus deltoides, Kochia scoparia, Secale cerale, and Broussonetia papyrifera (Paper Mulberry) species; and Escherichia coli bacteria. The collection efficiency for the synthetic particles ranged from 16 to 55%, depending on the particle size and surface tension of the collection fluid. The method was more effective in collecting pollen and the bacteria with an efficiency of 45-68% and 61.0-69.8%, respectively. Pollen collection was strongly influenced by its diameter, size, and surface geometry in a manner contrary to initial expectations. Reasons for the consistent yet unexpected collection results include leaky SAW pressure boundary segregation and shear-induced concentration of larger particles, and the subtle effects of wetting interactions. These results demonstrate a new method for collecting microparticles requiring only about one second per run, and illustrate the inadequacy of using synthetic microparticles as a substitute for their biological counterparts in experiments studying particle collection and behavior.

Paper-based microfluidic surface acoustic wave sample delivery and ionization source for rapid and sensitive ambient mass spectrometry

A surface acoustic wave-based sample delivery and ionization method that requires minimal to no sample pretreatment and that can operate under ambient conditions is described. This miniaturized technology enables real-time, rapid, and high-throughput analysis of trace compounds in complex mixtures, especially high ionic strength and viscous samples that can be challenging for conventional ionization techniques such as electrospray ionization. This technique takes advantage of high order surface acoustic wave (SAW) vibrations that both manipulate small volumes of liquid mixtures containing trace analyte compounds and seamlessly transfers analytes from the liquid sample into gas phase ions for mass spectrometry (MS) analysis. Drugs in human whole blood and plasma and heavy metals in tap water have been successfully detected at nanomolar concentrations by coupling a SAW atomization and ionization device with an inexpensive, paper-based sample delivery system and mass spectrometer. The miniaturized SAW ionization unit requires only a modest operating power of 3 to 4 W and, therefore, provides a viable and efficient ionization platform for the real-time analysis of a wide range of compounds.

Rapid fluid flow and mixing induced in microchannels using surface acoustic waves

Very-high-frequency surface acoustic waves, generated and transmitted along single-crystal lithium niobate, are used to drive homogeneous aqueous suspensions of polystyrene nanoparticles along microchannels. At a few hundred milliwatts, uniform and mixing flows with speeds of up to 10 mm/s were obtained in centimetres-long rectangular channels with cross-sectional dimensions of tens to a few hundreds of microns. A transition from uniform to mixing flow occurs as the channel width grows beyond the wavelength of sound in the fluid at the chosen excitation frequency. At far lower input powers, the suspension agglomerates into equally spaced, serpentine lines coincident with nodal lines in the acoustic pressure field. We expose the physics underlying these disparate phenomena with experimental results aided by numerical models.

Capillary wave motion excited by high frequency surface acoustic waves

This paper presents a numerical and experimental study of capillary wave motion excited by high frequency surface acoustic waves (SAWs). The objective of this study is to provide insight into the dynamic behavior of the fluid free surface and its dependence on the excitation amplitude. A two-dimensional numerical model that couples the motion of the piezoelectric substrate to a thin liquid layer atop the substrate is constructed. A perturbation method, in the limit of small-amplitude acoustic waves, is used to decompose the equations governing fluid motion to resolve the widely differing time scales associated with the high frequency excitation. While this model focuses on the free surface dynamics in the low-amplitude flow regime, the experimental study focuses on the high-amplitude flow regime. Transformation of time series data from both experiments and simulations into the frequency domain reveals that, in the low-amplitude regime, a fundamental resonant frequency and a superharmonic frequency are fou...

Direct visualization of surface acoustic waves along substrates using smoke particles

Smoke particles (SPs) are used to directly visualize surface acoustic waves (SAWs) propagating on a 128°-rotated Y-cut X-propagating lithium niobate (LiNbO3) substrate. By electrically exciting a SAW device in a compartment filled with SP, the SP were found to collect along the regions where the SAW propagates on the substrate. The results of the experiments show that SPs are deposited adjacent to regions of large vibration amplitude and form a clear pattern corresponding to the surface wave profile on the substrate. Through an analysis of the SAW-induced acoustic streaming in the air adjacent to the substrate and the surface acceleration measured with a laser Doppler vibrometer, we postulate that the large transverse surface accelerations due to the SAW ejects SP from the surface and carries them aloft to relatively quiescent regions nearby via acoustic streaming. Offering finer detail than fine powders common in Chladni figures [E. Chladni, Entdeckungen uber die Theorie des Klanges (Weidmanns, Erben und...

Unique flow transitions and particle collection switching phenomena in a microchannel induced by surface acoustic waves

We present an experimental approach for controlled switching between uniform flow for pumping and vortical flow for mixing in a microchannel fabricated onto a piezoelectric substrate. For particle laden fluids, this arrangement permits a choice between transport and alignment of microparticles. Using surface acoustic waves with amplitudes beyond 1 nm, the transition from uniform to mixing flows occurs when the acoustic wavelength in the fluid is reduced to a dimension smaller than the channel width, i.e., λf≥Wch for uniform flow and λf<Wch for mixing flow. On the other hand, using relatively weak surface acoustic waves with amplitudes below 1 nm, particles in an initially homogeneous suspension agglomerate into equally spaced lines with a separation of λf/2. Switching the transducer between its fundamental resonant frequency f0 and its first harmonic frequency f1+∼2f0 causes a switch between uniform and mixing flow, while switching between large and small amplitude excitation allows one to choose whether ...

Double aperture focusing transducer for controlling microparticle motions in trapezoidal microchannels with surface acoustic waves

We present a method for controlling the motion of microparticles suspended in an aqueous solution, which fills in a microchannel fabricated into a piezoelectric substrate, using propagating surface acoustic waves. The cross-sectional shape of this microchannel is trapezoidal, preventing the formation of acoustic standing waves across the channel width and therefore allowing the steering of microparticles. The induced acoustic streaming transports these particles to eliminate the use of external pumps for fluid actuation.

Enhanced Evaporation Strength through Fast Water Permeation in Graphene-Oxide Deposition

The unique characteristic of fast water permeation in laminated graphene oxide (GO) sheets has facilitated the development of ultrathin and ultrafast nanofiltration membranes. Here we report the application of fast water permeation property of immersed GO deposition for enhancing the performance of a GO/water nanofluid charged two-phase closed thermosyphon (TPCT). By benchmarking its performance against a silver oxide/water nanofluid charged TPCT, the enhancement of evaporation strength is found to be essentially attributed to the fast water permeation property of GO deposition instead of the enhanced surface wettability of the deposited layer. The expansion of interlayer distance between the graphitic planes of GO deposited layer enables intercalation of bilayer water for fast water permeation. The capillary force attributed to the frictionless interaction between the atomically smooth, hydrophobic carbon structures and the well-ordered hydrogen bonds of water molecules is sufficiently strong to overcome the gravitational force. As a result, a thin water film is formed on the GO deposited layers, inducing filmwise evaporation which is more effective than its interfacial counterpart, appreciably enhanced the overall performance of TPCT. This study paves the way for a promising start of employing the fast water permeation property of GO in thermal applications.

Coupled effects of hydrophobic layer and vibration on thermal efficiency of two-phase closed thermosyphons

Condensed droplets in a two-phase closed thermosyphon (TPCT) are subject to two competing forces: contact line pinning force between the droplet and the wall of the TPCT and the body force due to gravity. Either reducing the contact line pinning force or increasing the body force can lead to significant enhancement in the heat transport capability. This study aims to scrutinize the coupled effects of hydrophobic surface coating at the condenser wall and high-acceleration induced vibration on the thermal efficiency of a TPCT. We explore an approach to reduce the contact line pinning force by applying a thin layer of hydrophobic coating, which also facilitates dropwise condensation to further increase the heat transport capability. The body force of the condensed droplets can be increased by introducing a low-frequency (f ∼ 102 Hz) high-acceleration ( ∼ 103 m s−2) vibration. The formation of elongated liquid jets and entrainment of droplets induced by the high-acceleration vibration counteracts the enhancing effect from the increased body force of condensed droplets. Nanofluid with distinguished thermo-physical properties is charged to the TPCT to further enhance the thermal efficiency. By incorporating the coupled effects of hydrophobic layer and vibration, we can obtain a maximum augmentation in the heat transfer coefficient exceeding 47.7%. The factors contributing to the enhancement of thermal efficiency of a TPCT are identified and the underlying physical significance of the coupled effects is delineated.