N. A. Vorona

Study of charged particle motion in fields of different configurations for developing the concept of plasma separation of spent nuclear fuel

The concept of plasma separation of spent nuclear fuel in a plane perpendicular to the magnetic field in an electric potential of special configuration is developed. A specific feature of the proposed approach consists in using an accelerating potential for reducing energy and angular spread of plasma ions at the entrance to the separator chamber and a potential well for the spatial separation of ions with different masses. The trajectories of ions of the substance imitating spent nuclear fuel are calculated. The calculations are performed for azimuthal and axial magnetic fields and model electric field configurations corresponding to different geometries of the separator chamber. It is shown that, using magnetic fields with a characteristic strength of 1 kG and electric potentials of up to 1 kV inside a region with a linear size less than 100 cm, it is possible to separate ions of spent nuclear fuel with energies from 0.2 to 3 eV. The calculations were performed for a collisionless mode in the single-particle approximation. Possible variants of the experimental facility for plasma separation of spent nuclear fuel are proposed.

On the possibility of reprocessing spent nuclear fuel and radioactive waste by plasma methods

The concept of plasma separation of spent nuclear fuel and radioactive waste is presented. An approach that is based on using an accelerating potential to overcome the energy and angular spread of plasma ions at the separation region inlet and utilizing a potential well to separate spatially the ions of different masses is proposed. It is demonstrated that such separation may be performed at distances of about 1 m with electrical potentials of about 1 kV and a magnetic field of about 1 kG. The estimates of energy consumption and performance of the plasma separation method are presented. These estimates illustrate its potential for technological application. The results of development and construction of an experimental setup for testing the method of plasma separation are presented.

Vacuum arc with a distributed cathode spot as a plasma source for plasma separation of spent nuclear fuel and radioactive waste

Results from experimental studies of a vacuum arc with a distributed cathode spot on the heated cathode are presented. Such an arc can be used as a plasma source for plasma separation of spent nuclear fuel and radioactive waste. The experiments were performed with a gadolinium cathode, the properties of which are similar to those of an uranium arc cathode. The heat flux from the plasma to the cathode (and its volt equivalent) at discharge voltages of 4-15 V and discharge currents of 44-81 A, the radial distribution of the emission intensity of gadolinium atoms and singly charged ions in the arc channel at a voltage of 4.3 V, and the plasma electron temperature behind the anode were measured. The average charge of plasma ions at arc voltages of 3.5-8 V and a discharge current of 52 A and the average rate of gadolinium evaporation in the discharge were also determined.

Possibility of separating spent nuclear fuel components by a plasma method in azimuthal magnetic and radial electric fields

We consider the method of plasma separation of spent nuclear fuel in a system with an azimuthal magnetic field and the electric potential produced by electrodes located in a magnetized plasma. The results of calculation of trajectories of ions simulating uranium and the first peak of its fission products in the oneparticle approximation are described. The effect of the initial position and the initial velocity of ions on their trajectories is analyzed. The conditions ensuring the spatial separation of ions in the groups of masses admissible for practical realization are specified; it is shown that currents on the order of 100 kA through the central conductor and electrostatic potentials on the order of 1 kV are required for this purpose.

Designing of a lead ion model source for plasma separation of spent nuclear fuel

Plasma sources of model substances are required for solving problems associated with the development of a plasma separation method for spent nuclear fuel (SNF). Lead is chosen as the substance simulating the kinetics and dynamics of the heavy SNF component. We report on the results of analysis of the discharge in lead vapor with a concentration of 1012–1013 cm–3. Ionization is produced by an electron beam (with electron energy up to 500 eV) in the centimeter gap between planar electrodes. The discharge is simulated using the hydrodynamic and one-particle approximations. The current–voltage characteristics and efficiencies of single ionization depending on the vapor concentrations and thermoelectron current are obtained. The experimentally determined ion currents on the order of 100 μA for an ionization efficiency on the order of 0.1% are in conformity with the result of simulation.

Diffuse Vacuum Arc on the Nonthermionic Lead Cathode

Experimental study of the diffuse vacuum arc discharge on the nonthermionic lead cathode is presented. At the working cathode temperatures of 1.2-1.6-kK current-voltage characteristic of the discharge, cathode heat operation regime and its erosion rate were measured. Using probe methods, electron temperature (0.3-1.2 eV) and heavy particles (atoms and ions) mean charge (0.17-0.28 e) were determined in after-anode plasma. Evaluated current densities on the cathode are in agreement with a hypothesis on the ion mechanism of charge transfer on its surface. Parameters of the obtained discharge have been compared with the characteristics of the earlier investigated diffuse vacuum arcs on nonthermionic chromium and on thermionic gadolinium cathodes. The obtained data might be useful when creating plasma sources for verifying the plasma separation method of the spent nuclear fuel using the nonradioactive substances.

Study of the feasibility of distributed cathodic arc as a plasma source for development of the technology for plasma separation of SNF and radioactive wastes

One of the key problems in the development of plasma separation technology is designing a plasma source which uses condensed spent nuclear fuel (SNF) or nuclear wastes as a raw material. This paper covers the experimental study of the evaporation and ionization of model materials (gadolinium, niobium oxide, and titanium oxide). For these purposes, a vacuum arc with a heated cathode on the studied material was initiated and its parameters in different regimes were studied. During the experiment, the cathode temperature, arc current, arc voltage, and plasma radiation spectra were measured, and also probe measurements were carried out. It was found that the increase in the cathode heating power leads to the decrease in the arc voltage (to 3 V). This fact makes it possible to reduce the electron energy and achieve singly ionized plasma with a high degree of ionization to fulfill one of the requirements for plasma separation of SNF. This finding is supported by the analysis of the plasma radiation spectrum and the results of the probe diagnostics.

Diffuse vacuum arc on cerium dioxide hot cathode

A diffuse (spotless) vacuum arc was investigated on a hot cathode made from cerium dioxide. The discharge is obtained in the following range of current, voltage, and cathode temperature of I = 15–150 A, Va = 9–14 V, and Tc = 2.1–2.4 kK. The main characteristics of the plasma flow in space behind the anode with a hole were determined: it was found that the electron temperature at the working parameters lies in the range of 0.4–1 eV, the ions are predominantly singly charged, the average charge of the outgoing heavy particles reaches 0.9 e (elementary charge), and the most probable kinetic energy of the ions does not exceed 9 eV. Potentially found regimes of vacuum arc operation are promising for use in the work on implementation of the plasma method for spent nuclear fuel and/or radioactive waste reprocessing.

Diffuse vacuum arc with cerium oxide hot cathode

Diffuse vacuum arc with hot cathode is one of the perspective plasma sources for the development of spent nuclear fuel plasma reprocessing technology. Experimental data is known for such type of discharges on metal cathodes. In this work discharge with cerium dioxide hot cathode was studied. Cerium dioxide properties are similar to uranium dioxide. Its feature as dielectric is that it becomes conductive in oxygen-free atmosphere. Vacuum arc was studied at following parameters: cathode temperatures were between 2.0 and 2.2 kK, discharge currents was between 30 and 65 A and voltages was in range from 15 to 25 V. Power flows from plasma to cathode were estimated in achieved regimes. Analysis of generated plasma component composition was made by radiation spectrum diagnostics. These results were compared with calculations of equilibrium gaseous phase above solid sample of cerium dioxide in close to experimental conditions. Cerium dioxide vacuum evaporation rate and evaporation rate in arc were measured.

Experimental study of vacuum arc with low cathode current density as a source of metal plasma

Summary form only given. Sources of metal plasma are applied in plenty of technological tasks, for example, in coatings deposition or electromagnetic separation of isotopes. Vacuum arc may be used as one of such source. Its main advantages are high productivity and ionization degree, but plasma of usual vacuum arc contains micro particles of cathode erosion products. External cathode heating decreases its current density and problem of micro particles disappears. In this work such diffusive vacuum arc was studied. Gadolinium and plumbum were used as cathode materials. For gadolinium 90% of arc current consist of thermal electron emission from cathode, and for plumbum this part is less than 0.01%.Arc was initiated in vacuum chamber with pressure of residual gases less than 10 mPa. The investigated substance which was the arc cathode was placed in molybdenum crucible with outer diameter 25 mm. Under the crucible there was an electron-beam heater with maximum power about 1 kW. Heater allowed changing the cathode temperature at fixed arc current. A stainless steel water-cooling disk was used as the anode. It had a hole with the diameter of 32 or 15 mm. The distance between electrodes was about 30 mm. Arc plasma was studied by spectrometric and probe methods. The discharge with plumbum cathode was studied in current range from 20 to 70 A and cathode temperatures from 1.2 kK to 1.4 kK. Typical discharge voltage was about 15 V. The arc with gadolinium cathode was studied in current range from 15 to 150 A, cathode temperatures from 1.9 to 2.1 kK and voltages form 3 to 50 V. Arc regime with singly high ionized (ionization degree is about 100%) gadolinium plasma was revealed. The average ion charge of plumbum plasma was estimated at the arc current 40 A. Average evaporation speed of gadolinium and plumbum was measured in arc conditions. It was almost two times less than without discharge at the same cathode temperature.