N. Leefer

Search for Ultralight Scalar Dark Matter with Atomic Spectroscopy.

We report new limits on ultralight scalar dark matter (DM) with dilatonlike couplings to photons that can induce oscillations in the fine-structure constant α. Atomic dysprosium exhibits an electronic structure with two nearly degenerate levels whose energy splitting is sensitive to changes in α. Spectroscopy data for two isotopes of dysprosium over a two-year span are analyzed for coherent oscillations with angular frequencies below 1  rad s-1. No signal consistent with a DM coupling is identified, leading to new constraints on dilatonlike photon couplings over a wide mass range. Under the assumption that the scalar field comprises all of the DM, our limits on the coupling exceed those from equivalence-principle tests by up to 4 orders of magnitude for masses below 3×10(-18)  eV. Excess oscillatory power, inconsistent with fine-structure variation, is detected in a control channel, and is likely due to a systematic effect. Our atomic spectroscopy limits on DM are the first of their kind, and leave substantial room for improvement with state-of-the-art atomic clocks.

Cavity-enhanced room-temperature magnetometry using absorption by nitrogen-vacancy centers in diamond.

We demonstrate a cavity-enhanced room-temperature magnetic field sensor based on nitrogen-vacancy centers in diamond. Magnetic resonance is detected using absorption of light resonant with the 1042 nm spin-singlet transition. The diamond is placed in an external optical cavity to enhance the absorption, and significant absorption is observed even at room temperature. We demonstrate a magnetic field sensitivity of 2.5  nT/Hz, and project a photon shot-noise-limited sensitivity of 70  pT/Hz for a few mW of infrared light, and a quantum projection-noise-limited sensitivity of 250  fT/Hz for the sensing volume of ∼90  μm×90  μm×200  μm.

Parity-violating interactions of cosmic fields with atoms, molecules, and nuclei: Concepts and calculations for laboratory searches and extracting limits

We propose methods and present calculations that can be used to search for evidence of cosmic fields by investigating the parity-violating effects, including parity nonconservation amplitudes and electric dipole moments, that they induce in atoms. The results are used to constrain important fundamental parameters describing the strength of the interaction of various cosmic fields with electrons, protons, and neutrons. Candidates for such fields are dark matter (including axions) and dark energy, as well as several more exotic sources described by standard-model extensions. Calculations of the effects induced by pseudoscalar and pseudovector fields are performed for H, Li, Na, K, Cu, Rb, Ag, Cs, Ba, Ba+, Dy, Yb, Au, Tl, Fr, and Ra+. Existing parity nonconservation experiments in Cs, Dy, Yb, and Tl are combined with these calculations to directly place limits on the interaction strength between the temporal component, b(0), of a static pseudovector cosmic field and the atomic electrons, with the most stringent limit of vertical bar b(0)(e)vertical bar < 7 x 10(-15) GeV, in the laboratory frame of reference, coming from Dy. From a measurement of the nuclear anapole moment of Cs, and a limit on its value for Tl, we also extract limits on the interaction strength between the temporal component of this cosmic field, as well as a related tensor cosmic-field component d(00), with protons and neutrons. The most stringent limits of vertical bar b(0)(p)vertical bar < 4 x 10(-8) GeV and vertical bar d(00)(p)vertical bar < 5 x 10(-8) for protons and vertical bar b(0)(n)vertical bar < 2 x 10(-7) GeV and vertical bar d(00)(n)vertical bar < 2 x 10(-7) for neutrons (in the laboratory frame) come from the results using Cs. Axions may induce oscillating parity-and time reversal-violating effects in atoms and molecules through the generation of oscillating nuclear magnetic quadrupole and Schiff moments, which arise from P- and T-odd intranuclear forces and from the electric dipole moments of constituent nucleons. Nuclear spin-independent parity nonconservation effects may be enhanced in diatomic molecules possessing close pairs of opposite-parity levels in the presence of time-dependent interactions.

Limit on the temporal variation of the fine-structure constant using atomic dysprosium

Over 8 months, we monitored transition frequencies between nearly degenerate, opposite-parity levels in two isotopes of atomic dysprosium (Dy). These frequencies are sensitive to variation of the fine-structure constant (alpha) due to relativistic corrections of opposite sign for the opposite-parity levels. In this unique system, in contrast to atomic-clock comparisons, the difference of the electronic energies of the opposite-parity levels can be monitored directly utilizing a rf electric-dipole transition between them. Our measurements show that the frequency variation of the 3.1-MHz transition in (163)Dy and the 235-MHz transition in (162)Dy are 9.0+/-6.7 Hz/yr and -0.6+/-6.5 Hz/yr, respectively. These results provide a rate of fractional variation of alpha of (-2.7+/-2.6) x 10(-15) yr(-1) (1 sigma) without assumptions on constancy of other fundamental constants, indicating absence of significant variation at the present level of sensitivity.

Limiting P-odd interactions of cosmic fields with electrons, protons and neutrons

We propose methods for extracting limits on the strength of P-odd interactions of pseudoscalar and pseudovector cosmic fields with electrons, protons, and neutrons, by exploiting the static and dynamic parity-nonconserving amplitudes and electric dipole moments they induce in atoms. Candidates for such fields are dark matter (including axions) and dark energy, as well as several more exotic sources described by Lorentz-violating standard model extensions. Atomic calculations are performed for H, Li, Na, K, Rb, Cs, Ba(+), Tl, Dy, Fr, and Ra(+). From these calculations and existing measurements in Dy, Cs, and Tl, we constrain the interaction strengths of the parity-violating static pseudovector cosmic field to be 7 × 10(-15) GeV with an electron, and 3 × 10(-8) GeV with a proton.

Limits on violations of Lorentz symmetry and the Einstein equivalence principle using radio-frequency spectroscopy of atomic dysprosium.

We report a joint test of local Lorentz invariance and the Einstein equivalence principle for electrons, using long-term measurements of the transition frequency between two nearly degenerate states of atomic dysprosium. We present many-body calculations which demonstrate that the energy splitting of these states is particularly sensitive to violations of both special and general relativity. We limit Lorentz violation for electrons at the level of 10(-17), matching or improving the best laboratory and astrophysical limits by up to a factor of 10, and improve bounds on gravitational redshift anomalies for electrons by 2 orders of magnitude, to 10(-8). With some enhancements, our experiment may be sensitive to Lorentz violation at the level of 9 × 10(-20).

New limits on variation of the fine-structure constant using atomic dysprosium.

We report on the spectroscopy of radio-frequency transitions between nearly degenerate, opposite-parity excited states in atomic dysprosium (Dy). Theoretical calculations predict that these states are very sensitive to variation of the fine-structure constant α owing to large relativistic corrections of opposite sign for the opposite-parity levels. The near degeneracy reduces the relative precision necessary to place constraints on variation of α, competitive with results obtained from the best atomic clocks in the world. Additionally, the existence of several abundant isotopes of Dy allows isotopic comparisons that suppress common-mode systematic errors. The frequencies of the 754-MHz transition in 164Dy and 235-MHz transition in 162Dy are measured over the span of two years. The linear variation of α is α·/α=(-5.8±6.9([1σ]))×10(-17)  yr(-1), consistent with zero. The same data are used to constrain the dimensionless parameter kα characterizing a possible coupling of α to a changing gravitational potential. We find that kα=(-5.5±5.2([1σ]))×10(-7), essentially consistent with zero and the best constraint to date.

Infrared absorption band and vibronic structure of the nitrogen-vacancy center in diamond

Negatively charged nitrogen-vacancy (NV

Measurement of hyperfine structure and isotope shifts in the Dy 421 nm transition

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Investigation of the gravitational-potential dependence of the fine-structure constant using atomic dysprosium

) color centers in diamond have generated much interest for use in quantum technology. Despite the progress made in developing their applications, many questions about the basic properties of NV