N. V. Tcherniega

Experimental observation of stimulated low-frequency Raman scattering in water suspensions of silver and gold nanoparticles.

In this Letter we report on experimental observation of stimulated low-frequency Raman scattering (SLFRS) in gold and silver nanoparticle suspensions excited by 20 ns ruby laser pulses, SLFRS propagated in forward and backward directions with a maximum conversion efficiency up to 20%. Frequency shift for silver nanoparticle suspension was found to be 0.33 THz and for gold nanoparticle suspension 0.435 THz. This type of stimulated scattering of light can be used as an effective source of biharmonic pumping for solving a large number of practical tasks.

Spectral Characteristics of the Radiation of Artificial Opal Crystals in the Presence of the Photonic Flame Effect

The results of investigation of the spectral characteristics of radiation in the presence of the photonic flame effect recently discovered experimentally are presented. Radiation from a ruby laser operating in the Q-factor modulation regime with a generation wavelength of 694.3 nm is focused near the oriented surface of a globular photon crystal (artificial opal with a globule size of 230 nm) placed on a copper cold guide whose temperature is close to the liquid-nitrogen boiling point (77 K). The spectrum of long-term afterglow (with a duration of about several seconds when the duration of a pump pulse is equal to 20 ns) appearing in the photonic flame effect is detected using a fiber optic minispectrometer and consists of several comparatively narrow lines whose intensity strongly varies with the pumping power. A similar glow is observed in opal samples filled with acetone or ethanol.

Reduction of the threshold of stimulated Raman scattering in Raman-active media introduced into pores of a globular photonic crystal

The characteristics of stimulated Raman scattering in benzene and carbon disulfide introduced in pores of globular photonic crystals—opal matrices formed from close-packed balls (globules) of amorphous quartz (silica)—have been experimentally studied. Stimulated Raman scattering spectra have been excited by giant pulses of the second optical harmonic (532 nm) of a YAG laser. The spectra have been recorded in the direction of mirror reflection from the (111) growth surface of a globular photonic crystal at various angles of incidence (10°–70°) of laser radiation. It has been shown that the threshold of stimulated Raman scattering decreases sharply (by more than an order of magnitude) at a certain angle of mirror reflection and additional Stokes and anti-Stokes Raman satellites appear in the spectrum. The observed sharp decrease in the threshold of stimulated Raman scattering has been explained by an increase in the spectral density of the electromagnetic field in the surface region of the photonic crystal because of the approach of the spectral position of the stopband of the photonic crystal to the exciting line (532 nm) under variation of the angle of incidence of pump radiation on the (111) surface.

Photon distribution function for stokes wave for stimulated Raman scattering

New time-dependent integrals of motion are found for stimulated Raman scattering. An explicit formula for the photon-number probability distribution as a function of the laser-field intensity and the medium parameters is obtained in terms of Hermite polynomials of two variables.

Spatial, Spectral, and Temporal Characteristics of Stimulated Light Scattering in Water

Spatial, temporal, and spectral characteristics of stimulated light scattering (SS) in water were investigated in both nano- and picosecond ranges under different experimental conditions and compared with the analogous characteristics of stimulated light scattering in other liquids. Stimulated Raman scattering (SRS) and stimulated Brillouin scattering (SBS) of light were studied. The results obtained provide useful information on the structure of water, its purity, and additions, which can result in its pollution. The excitation conditions of stimulated light scattering (SS) in one spatial mode and with maximum pulse energy conversion were determined. It is shown that stimulated light scattering can be successfully applied to control water quality (and it can be done very fast) as well as for information processing, i.e., the amplitude–phase structure of complex light fields can be registered in water as a dynamic hologram and reconstructed in real time.

Tomographic Description of Stimulated Brillouin Scattering of Light

The process of stimulated Brillouin scattering is described by the two‐dimensional oscillator model. Photons of the Stokes mode are described by one mode of the oscillator, and acoustic phonons are described by the other mode. The interaction of photons and acoustic phonons is assumed to be quadratic in the creation and annihilation operators of photons and phonons. The laser is considered as a classical light source and its depletion is neglected. New time‐dependent integrals of motion and the photon–phonon probability distribution function are found. The mean Stokes photon number and the mean acoustic phonon number are expressed as functions of the medium parameters (initial dispersions) and the interaction parameter (coupling constant). The classical propagator for stimulated Brillouin scattering and tomograms of the photon and phonon states are investigated within the framework of the symplectic‐tomography scheme.

Lowering of stimulated Raman scattering threshold as a result of light capture

Stimulated Raman Scattering in globular photonic crystals and globular photonic glasses at different diameters of globules (250 – 400 nm) with embedded molecular liquids is studied under excitation by nanosecond or picoseconds laser pulses. Substantial decrease of Stimulated Raman Scattering threshold was observed. Such phenomenon was explained as the result of laser radiation field increase in globular photonic structures due to photonic density of states enhancement near the edges of photonic stop bands of photonic crystals and due to Mie resonance or whispering gallery modes effect revealing in photonic glasses. Stimulated Raman Scattering threshold lowering as a result of light capture in globular photonic crystals and photonic glasses opens the way to new efficient laser sources created on the base of composite globular photonic structures. Experimental data on spectra of Stimulated Raman Scattering in light and heavy waters are presented. As sources of exciting light the powerful ultra short solid state laser pulses with 532.0 nm wavelength and giant pulses of Ruby laser (694.3 nm) have been used. Several Stokes and anti-Stokes satellites were observed. Libration modes have been excited and resulted in some additional Raman bands at low frequency region and also as combining tones.

Stimulated low-frequency Raman scattering in nanostructures

A new type of stimulated scattering of light (stimulated low-frequency Raman scattering (SLFRS)) is found. SLFRS appears as a result of interaction of laser pulses with acoustic vibrations of structural elements of nanostructured materials. SLFRS is shown to arise in materials with different compositions and different degrees of morphology, both ordered and random. Frequency shifts of SLFRS components are measured. A number of practical applications of the effect are proposed, in particular, biharmonic pumping with the help of SLFRS.

Multifrequency stimulated Raman scattering of light in liquid nitrogen infiltrated into 3D photonic crystals

Spectral characteristics of stimulated Raman scattering at least in synthetic opal matrices infiltrated with liquid nitrogen upon excitation by nanosecond laser pulses are studied. The effect of the stop band position on the generation efficiency of anti-Stokes components of stimulated Raman scattering up to the third order is demonstrated. The excitation threshold of stimulated Raman scattering in liquid nitrogen infiltrated into opals is significantly lower in comparison with the generation in bulk samples.

Stimulated light scattering in synthetic opal filled with dielectrics

We have studied characteristics of stimulated light scattering in synthetic opal crystals made up of silica spheres. This type of light scattering results from interaction between pulsed laser radiation and dielectric nanoparticles, such as silica (SiO2) spheres in the structure of synthetic opal. The Stokes shift in the scattered radiation spectrum was 0.4–1.0 cm−1. The Stokes shift was determined as a function of scattering geometry, sphere diameter, sample temperature, and the type of dielectric in the opal pores. The results are of interest for assessing the size of nanoparticles in spatially ordered inorganic structures.