Nader Abuhassan

An emerging ground‐based aerosol climatology: Aerosol optical depth from AERONET

Long-term measurements by the AERONET program of spectral aerosol optical depth, precipitable water, and derived Angstrom exponent were analyzed and compiled into an aerosol optical properties climatology. Quality assured monthly means are presented and described for 9 primary sites and 21 additional multiyear sites with distinct aerosol regimes representing tropical biomass burning, boreal forests, midlatitude humid climates, midlatitude dry climates, oceanic sites, desert sites, and background sites. Seasonal trends for each of these nine sites are discussed and climatic averages presented.

A High-Accuracy Multiwavelength Radiometer for In Situ Measurements in the Thermal Infrared. Part I: Characterization of the Instrument

Abstract The new infrared radiometer (conveyable low-noise infrared radiometer for measurements of atmosphere and ground surface targets, or CLIMAT) is a highly sensitive field instrument designed to measure brightness temperatures or radiances in the infrared, from the ground level, or from an aircraft. It can be equipped with up to six channels in the 8–14-μm range. This instrument is characterized by its portability (total mass less than 5 kg), its self-sufficiency, and its automated operation. It can be operated either manually or automatically. The optical head of the instrument contains an objective lens and a condenser mounted according to the Kohler design, providing a uniform irradiation on the detector and a well-delimited field of view. The radiation is measured by a low-noise fast thermopile whose responsivity is slightly temperature dependent. The radiometric noise expressed as an equivalent brightness temperature is on the order of 50 mK for a 1-μm bandwidth at room temperature. The applicat...

Thermal-infrared field radiometer for vicarious cross-calibration: characterization and comparisons with other field instruments

A four-band (8.2 to 9.2, 10.5 to 11.5, 11.5 to 12.5, and 8 to 14 mm), prototype, thermal-IR radiometer, model CE 312 (CE 312 is the company model number. In previous papers, the CE 312 was called the CLIMAT (conveyable low-noise IR radiometer for measurements of at- mosphere and ground-surface targets)), with a built-in radiance refer- ence is been fabricated by CIMEL Electronique (Paris, France) for use as a field instrument. The instrument is briefly described, laboratory char- acterization is detailed, and its field measurements are compared with those from three other radiometers. The CE 312s main characteristics are linearity of better than 0.8%, field of view of 9.5 deg; noise-equivalent temperature difference of 0.06 to 0.2 K (depending on the band) for brightness temperatures of 0 to 75°C; SNR greater than 1100 for the broadband and greater than 400 for the other bands for brightness tem- peratures between 10 and 80°C; and repeatability of the measured radi- ance smaller than 0.35% after four field campaigns, corresponding to 0.2 K in terms of brightness temperature. Field measurements were con- ducted over different periods during 1996 at Jornada Experimental Range, New Mexico, Lunar Lake and Railroad Valley, Nevada, and Lake Tahoe, California. The CE 312 compares quite favorably with the other instruments: the brightness temperature at two different sites compared to within 0.3 K with two instruments. These measurements show that the CE 312 thermal-IR radiometer is very stable for ambient temperatures varying between 15 and 60°C and that the availability of several filters in the thermal-IR region can help tremendously to improve the accuracy of the radiance determination.

Spatial and temporal variability of ozone and nitrogen dioxide over a major urban estuarine ecosystem

Spatial and temporal dynamics in trace gas pollutants were examined over a major urban estuarine ecosystem, using a new network of ground-based Pandora spectrometers deployed at strategic locations along the Washington-Baltimore corridor and the Chesapeake Bay. Total column ozone (TCO3) and nitrogen dioxide (TCNO2) were measured during NASA’s DISCOVER-AQ and GeoCAPE-CBODAQ campaigns in July 2011. The Pandora network provided high-resolution information on air-quality variability, local pollution conditions, large-scale meteorological influences, and interdependencies of ozone and its major precursor, NO2. Measurements were used to compare with air-quality model simulations (CMAQ), evaluate Aura-OMI satellite retrievals, and assess advantages and limitations of space-based observations under a range of conditions. During the campaign, TCNO2 varied by an order of magnitude, both spatially and temporally. Although fairly constant in rural regions, TCNO2 showed clear diurnal and weekly patterns in polluted urban areas caused by changes in near-surface emissions. With a coarse resolution and an overpass at around 13:30 local time, OMI cannot detect this strong variability in NO2, missing pollution peaks from industrial and rush hour activities. Not as highly variable as NO2, TCO3 was mostly affected by large-scale meteorological patterns as observed by OMI. A clear weekly cycle in TCO3, with minima over the weekend, was due to a combination of weekly weather patterns and changes in near-surface NOx emissions. A Pandora instrument intercomparison under the same conditions at GSFC showed excellent agreement, within ±4.8DU for TCO3 and ±0.07DU for TCNO2 with no air-mass-factor dependence, suggesting that observed variability during the campaign was real.

Tracking elevated pollution layers with a newly developed hyperspectral Sun/Sky spectrometer (4STAR): Results from the TCAP 2012 and 2013 campaigns

Total columnar water vapor (CWV), nitrogen dioxide (NO2), and ozone (O3) are derived from a newly developed, hyperspectral airborne Sun-sky spectrometer (4STAR) for the first time during the two intensive phases of the Two-Column Aerosol Project (TCAP) in summer 2012 and winter 2013 aboard the DOE G-1 aircraft. We compare results with coincident measurements. We find 0.045 g/cm2 (4.2%) negative bias and 0.28 g/cm2 (26.3%) root-mean-square difference (RMSD) in water vapor layer comparison with an in situ hygrometer and an overall RMSD of 1.28 g/m3 (38%) water vapor amount in profile by profile comparisons, with differences distributed evenly around zero. RMSD for O3 columns average to 3%, with a 1% negative bias for 4STAR compared with the Ozone Measuring Instrument along aircraft flight tracks for 14 flights during both TCAP phases. Ground-based comparisons with Pandora spectrometers at the Goddard Space Flight Center, Greenbelt, Maryland, showed excellent agreement between the instruments for both O3 (1% RMSD and 0.1% bias) and NO2 (17.5% RMSD and −8% bias). We apply clustering analysis of the retrieved products as a case study during the TCAP summer campaign to identify variations in atmospheric composition of elevated pollution layers and demonstrate that combined total column measurements of trace gas and aerosols can be used to define different pollution layer sources, by comparing our results with trajectory analysis and in situ airborne miniSPLAT (single-particle mass spectrometer) measurements. Our analysis represents a first step in linking sparse but intense in situ measurements from suborbital campaigns with total column observations from space.

Development and qualification of the conveyable thermal infrared field radiometer CLIMAT

The radiometer CLIMAT is a highly sensitive field instrument designed for multispectral thermal infrared measurements. Ground-based measurements can be performed. but the instrument has capabilities for operating from aircraft or balloon. The optics consist of an objective lens and a condenser mounted according to the Koehler principle to provide uniform irradiation over the detector surface. The radiometric signal is treated by a fast thermopile detector characterized by a low noise and a very weak temperature dependence of its responsivity. The managing system allows either manual or automated measurements. The energy consumption of the instrument is optimized for a maximum autonomy. The optical and electrical units of the instrument are described. Different experimental studies for measuring the sensitivity accuracy, spectral characteristics, thermal behavior and, field of view of the instrument are described. The instrument is dedicated to ground and vegetation on the one hand. and on the other hand, clouds and atmospheric soundings. The radiometer is also designed for calibrations or analyses of satellite radiometry data. Some atmospheric measurements obtained with a prototype are presented. Prospects are the development and the qualification of a narrow field-of-view instrument adapted to inhomogeneous targets such as cirrus clouds. A 3.7-tim channel and an internal blackbody are under study.

Solar viewing interferometer prototype

The Earth Atmospheric Solar-Occultation Imager (EASI) is a proposed interferometer with 5 telescopes on an 8-meter boom in a 1D Fizeau configuration. Placed at the Earth-Sun L2 Lagrange point, EASI would perform absorption spectroscopy of the Earth’s atmosphere occulting the Sun. Fizeau interferometers give spatial resolution comparable to a filled aperture but lower collecting area. Even with the small collecting area the high solar flux requires most of the energy to be reflected back to space. EASI will require closed loop control of the optics to compensate for spacecraft and instrument motions, thermal and structural transients and pointing jitter. The Solar Viewing Interferometry Prototype (SVIP) is a prototype ground instrument to study the needed wavefront control methods. SVIP consists of three 10 cm aperture telescopes, in a linear configuration, on a 1.2-meter boom that will estimate atmospheric abundances of O2, H2O, CO2, and CH4 versus altitude and azimuth in the 1.25 - 1.73 micron band. SVIP measures the Greenhouse Gas absorption while looking at the sun, and uses solar granulation to deduce piston, tip and tilt misalignments from atmospheric turbulence and the instrument structure. Tip/tilt sensors determine relative/absolute telescope pointing and operate from 0.43 - 0.48 microns to maximize contrast. Two piston sensors, using a robust variation of dispersed fringes, determine piston shifts between the baselines and operate from 0.5 - 0.73 microns. All sensors are sampled at 800 Hz and processed with a DSP computer and fed back at 200 Hz (3 dB) to the active optics. A 4 Hz error signal is also fed back to the tracking platform. Optical performance will be maintained to better than λ/8 rms in closed-loop.