Nicolas Forget

Parametric amplification of few-cycle carrier-envelope phase-stable pulses at 2.1 μm

We demonstrate an optical parametric chirped-pulse amplifier producing infrared 20 fs (3-optical-cycle) pulses with a stable carrier-envelope phase. The amplifier is seeded with self-phase-stabilized pulses obtained by optical rectification of the output of an ultrabroadband Ti:sapphire oscillator. Energies of -80 microJ with a well-suppressed background of parametric superfluorescence and up to 400 microJ with a superfluorescence background are obtained from a two-stage parametric amplifier based on periodically poled LiNbO3 and LiTaO3 crystals. The parametric amplifier is pumped by an optically synchronized 1 kHz, 30 ps, 1053 nm Nd:YLF amplifier seeded by the same Ti:sapphire oscillator.

Self-compression of millijoule 1.5 μm pulses

We demonstrate a four-stage optical parametric chirped-pulse amplification system that delivers carrier-envelope phase-stable approximately 1.5 microm pulses with energies up to 12.5 mJ before recompression. The system is based on a fusion of femtosecond diode-pumped solid-state Yb technology and a picosecond 100 mJ Nd:YAG pump laser. Pulses with 62 nm bandwidth are recompressed to a 74.4 fs duration close to the transform limit. To show the way toward a terawatt-peak-power single-cycle IR source, we demonstrate self-compression of 2.2 mJ pulses down to 19.8 fs duration in a single filament in argon with a 1.5 mJ output energy and 66% energy throughput.

Single-shot, high-dynamic-range measurement of sub-15 fs pulses by self-referenced spectral interferometry.

We explore theoretically and numerically the temporal contrast limitation of a self-referenced spectral interferometry measurement. An experimental confirmation is given by characterization and fine compression of hollow-core fiber generated sub-15 fs pulses, yielding an accurately measured coherent contrast of 50 dB on a ±400 fs time range.

Scalable Yb-MOPA-driven carrier-envelope phase-stable few-cycle parametric amplifier at 1.5 μm

Carrier-envelope phase-stable 4 microJ pulses at approximately 1.5 microm are obtained from a femtosecond Yb:KGW-MOPA-pumped two-stage optical parametric amplifier. This novel technology represents a highly attractive alternative to traditional Ti:sapphire front-ends for seeding multimillijoule-level optical parametric chirped-pulse amplifiers. For this task, we demonstrate stretching of the OPA output to approximately 40 ps and recompression to 33 fs pulse duration. As a stand-alone system, our tunable two-stage OPA might find numerous applications in time-resolved spectroscopy and micromachining.

Carrier-envelope phase stabilization and control using a transmission grating compressor and an AOPDF

Carrier-envelope phase (CEP) stabilization of a femtosecond chirped-pulse amplification system featuring a compact transmission grating compressor is demonstrated. The system includes two amplification stages and routinely generates phase-stable (approximately 250 mrad rms) 2 mJ, 25 fs pulses at 1 kHz. Minimizing the optical pathway in the compressor enables phase stabilization without feedback control of the grating separation or beam pointing. We also demonstrate for the first time to the best of our knowledge, out-of-loop control of the CEP using an acousto-optic programmable dispersive filter inside the laser chain.

Generation of high-contrast millijoule pulses by optical parametric chirped-pulse amplification in periodically poled KTiOPO4

A new high-contrast, high-gain optical parametric chirped-pulse amplifier (OPCPA) architecture is demonstrated in periodically poled KTiOPO4 (PPKTP). This architecture overcomes parametric fluorescence contrast limitations of the OPCPA in periodically poled materials. The scheme is based on two passes of a single relay-imaged pump pulse and a free-propagating signal pulse through a 1.5 mm x 5 mm x 7.5 mm PPKTP crystal. The output energy of 1.2 mJ is generated at a center wavelength of 1053 nm by 24 mJ of pump energy. A prepulse contrast level of > 3 x 10(7) was measured with > 10(6) saturated gain in the amplifier. Amplified pulses were compressed to 200 fs. This simple and versatile concept requires only a modest pump energy from a commercial pump laser and represents a possible high-contrast front end for high-energy Nd:glass-based petawatt-class lasers.

Self-referenced characterization of femtosecond laser pulses by chirp scan

We investigate a variant of the d-scan technique, an intuitive pulse characterization method for retrieving the spectral phase of ultrashort laser pulses. In this variant a ramp of quadratic spectral phases is applied to the input pulses and the second harmonic spectra of the resulting pulses are measured for each chirp value. We demonstrate that a given field envelope produces a unique and unequivocal chirp-scan map and that, under some asymptotic assumptions, both the spectral amplitude and phase of the measured pulse can be retrieved analytically from only two measurements. An iterative algorithm can exploit the redundancy of the information contained in the chirp-scan map to discard experimental noise, artifacts, calibration errors and improve the reconstruction of both the spectral intensity and phase. This technique is compared to two reference characterization techniques (FROG and SRSI). Finally, we perform d-scan measurements with a simple grating-pair compressor.

Actively mode-locked optical parametric oscillator.

We report on what we believe to be the first demonstration of active mode locking of an optical parametric oscillator. An acousto-optic modulator is inserted into a nearly degenerate (approximately 1064 nm) and doubly resonant optical parametric oscillator based on periodically poled LiNbO3 and pumped with the second harmonic of a quasi-continuous-wave single-frequency Nd:YAG laser. When the modulation frequency is matched to the free spectral range of the cavity (120 MHz), a pulsed regime is observed, with pulse durations as short as 700 ps.

Self-referenced spectral interferometry for ultrashort infrared pulse characterization

We demonstrate for the first time (to our knowledge) characterization of ultrashort IR pulses by self-referenced spectral interferometry. Both sub-55-fs pulses from 1.4 μm to 2 μm and broadband 2.5-cycle pulses at 1.65 μm (13 fs FWHM) are characterized.

Pulse-measurement techniques using a single amplitude and phase spectral shaper

We investigate, both theoretically and experimentally, the practical use of amplitude and phase pulse shapers to characterize ultrashort optical pulses. Pulse shapers greatly simplify the optical setup required for the SH-FROG and SPIDER measurement techniques, and both methods can even be implemented with a common optical layout. We also introduce, demonstrate, and compare several new interferometric variants of these techniques, which are compatible with a basic setup comprising no more than a pulse shaper, a type I second-harmonic stage, and a spectrometer.