Nitzan Akerman

Single-ion quantum lock-in amplifier

Quantum metrology uses tools from quantum information science to improve measurement signal-to-noise ratios. The challenge is to increase sensitivity while reducing susceptibility to noise, tasks that are often in conflict. Lock-in measurement is a detection scheme designed to overcome this difficulty by spectrally separating signal from noise. Here we report on the implementation of a quantum analogue to the classical lock-in amplifier. All the lock-in operations—modulation, detection and mixing—are performed through the application of non-commuting quantum operators to the electronic spin state of a single, trapped Sr+ ion. We significantly increase its sensitivity to external fields while extending phase coherence by three orders of magnitude, to more than one second. Using this technique, we measure frequency shifts with a sensitivity of 0.42 Hz Hz−1/2 (corresponding to a magnetic field measurement sensitivity of 15 pT Hz−1/2), obtaining an uncertainty of less than 10 mHz (350 fT) after 3,720 seconds of averaging. These sensitivities are limited by quantum projection noise and improve on other single-spin probe technologies by two orders of magnitude. Our reported sensitivity is sufficient for the measurement of parity non-conservation, as well as the detection of the magnetic field of a single electronic spin one micrometre from an ion detector with nanometre resolution. As a first application, we perform light shift spectroscopy of a narrow optical quadrupole transition. Finally, we emphasize that the quantum lock-in technique is generic and can potentially enhance the sensitivity of any quantum sensor.

Measurement of the magnetic interaction between two bound electrons of two separate ions

Electrons have an intrinsic, indivisible, magnetic dipole aligned with their internal angular momentum (spin)1. The magnetic interaction between two electrons can therefore impose a change in their spin orientation. Similar dipolar magnetic interactions exists between other spin systems and were studied experimentally. Examples include the interaction between an electron and its nucleus or between several multi-electron spin complexes2–8. The process for two electrons, however, was never observed in experiment. The challenge is two-fold. At the atomic scale, where the coupling is relatively large, the magnetic interaction is often overshadowed by the much larger coulomb exchange counterpart2. In typical situations where exchange is negligible, magnetic interactions are also very weak and well below ambient magnetic noise. Here we report on the first measurement of the magnetic interaction between two electronic spins. To this end, we used the ground state valence electrons of two Sr ions, co-trapped in an electric Paul trap and separated by more than two micrometers. We measured the weak, millihertz scale (alternatively 10−18 eV or 10−14 K), magnetic interaction between their electronic spins. This, in the presence of magnetic noise that was six ∗Current address: Physical Measurement Laboratory, National Institute of Science and Technology, Boulder CO, 80305, USA. †Current address: Cavendish Laboratory, University of Cambridge, J.J. Thomson Avenue, Cambridge CB30HE, United Kingdom.

Dynamics of a Ground-State Cooled Ion Colliding with Ultracold Atoms

Ultracold atom-ion mixtures are gaining increasing interest due to their potential applications in ultracold and state-controlled chemistry, quantum computing, and many-body physics. Here, we studied the dynamics of a single ground-state cooled ion during few, to many, Langevin (spiraling) collisions with ultracold atoms. We measured the ions energy distribution and observed a clear deviation from the Maxwell-Boltzmann distribution, characterized by an exponential tail, to a power-law distribution best described by a Tsallis function. Unlike previous experiments, the energy scale of atom-ion interactions is not determined by either the atomic cloud temperature or the ions trap residual excess-micromotion energy. Instead, it is determined by the force the atom exerts on the ion during a collision which is then amplified by the trap dynamics. This effect is intrinsic to ion Paul traps and sets the lower bound of atom-ion steady-state interaction energy in these systems. Despite the fact that our system is eventually driven out of the ultracold regime, we are capable of studying quantum effects by limiting the interaction to the first collision when the ion is initialized in the ground state of the trap.

Nonlinear single-spin spectrum analyzer.

A qubit can be used as a sensitive spectrum analyzer of its environment. Here we show how the problem of spectral analysis of noise induced by a strongly coupled environment can be solved for discrete spectra. Our analytical model shows non-linear signal dependence on noise power, as well as possible frequency mixing, both are inherent to quantum evolution. This model enabled us to use a single trapped ion as a sensitive probe for strong, non-Gaussian, discrete magnetic field noise. To overcome ambiguities arising from the non-linear character of strong noise, we develop a three step noise characterization scheme: peak identification, magnitude identification and fine-tuning. Finally, we compare experimentally equidistant versus Uhrig pulse schemes for spectral analysis. The method is readily available to any quantum probe which can be coherently manipulated.

Single-ion nonlinear mechanical oscillator

We study the steady-state motion of a single trapped ion oscillator driven to the nonlinear regime. Damping is achieved via Doppler laser cooling. The ion motion is found to be well described by the Duffing oscillator model with an additional nonlinear damping term. We demonstrate here the unique ability of tuning both the linear as well as the nonlinear damping coefficients by controlling the laser-cooling parameters. Our observations pave the way for the investigation of nonlinear dynamics on the quantum-to-classical interface as well as mechanical noise squeezing in laser-cooling dynamics.

Universal gate-set for trapped-ion qubits using a narrow linewidth diode laser

We report on the implementation of a high fidelity universal gate-set on optical qubits based on trapped 88Sr+ ions for the purpose of quantum information processing. All coherent operations were performed using a narrow linewidth diode laser. We employed a master-slave configuration for the laser, where an ultra low expansion glass Fabry–Perot cavity is used as a stable reference as well as a spectral filter. We characterized the laser spectrum using the ions with a modified Ramsey sequence which eliminated the affect of the magnetic field noise. We demonstrated high fidelity single qubit gates with individual addressing, based on inhomogeneous micromotion, on a two-ion chain as well as the Molmer–Sorensen two-qubit entangling gate.

High-fidelity state detection and tomography of a single-ion Zeeman qubit

We demonstrate high-fidelity Zeeman qubit state detection in a single trapped 88Sr+ ion. Qubit readout is performed by shelving one of the qubit states to a metastable level using a narrow linewidth diode laser at 674 nm, followed by state-selective fluorescence detection. The average fidelity reached for the readout of the qubit state is 0.9989(1). We then measure the fidelity of state tomography, averaged over all possible single-qubit states, which is 0.9979(2). We also fully characterize the detection process using quantum process tomography. This readout fidelity is compatible with recent estimates of the detection error threshold required for fault-tolerant computation, whereas high-fidelity state tomography opens the way for high-precision quantum process tomography.

Addressing two-level systems variably coupled to an oscillating field.

We propose a simple method to spectrally resolve an array of identical two-level systems coupled to an inhomogeneous oscillating field. The addressing protocol uses a dressing field with a spatially dependent coupling to the atoms. We validate this scheme experimentally by realizing single-spin addressing of a linear chain of trapped ions that are separated by ~3 μm, dressed by a laser field that is resonant with the micromotion sideband of a narrow optical transition.

Spin-controlled atom–ion chemistry

Quantum control of chemical reactions is an important goal in chemistry and physics. Ultracold chemical reactions are often controlled by preparing the reactants in specific quantum states. Here we demonstrate spin-controlled atom–ion inelastic (spin-exchange) processes and chemical (charge-exchange) reactions in an ultracold Rb-Sr+ mixture. The ion’s spin state is controlled by the atomic hyperfine spin state via spin-exchange collisions, which polarize the ion’s spin parallel to the atomic spin. We achieve ~ 90% spin polarization due to the absence of strong spin-relaxation channel. Charge-exchange collisions involving electron transfer are only allowed for (RbSr)+ colliding in the singlet manifold. Initializing the atoms in various spin states affects the overlap of the collision wave function with the singlet molecular manifold and therefore also the reaction rate. Our observations agree with theoretical predictions.Chemical reactions with ultracold atoms and ions are explored so far with the atom–ion interactions. Here the authors discuss spin-exchange process and show that the spin state of an ensemble of neutral Rb atoms can be used to control the final spin of an imbedded Sr+ ion in the collisions.

Doppler cooling thermometry of a multilevel ion in the presence of micromotion

We study the time-dependent fluorescence of an initially hot, multi-level, single atomic ion trapped in a radio-frequency Paul trap during Doppler cooling. We have developed an analytical model that describes the fluorescence dynamics during Doppler cooling which is used to extract the initial energy of the ion. While previous models of Doppler cooling thermometry were limited to atoms with a two-level energy structure and neglected the effect of the trap oscillating electric fields, our model applies to atoms with multi-level energy structure and takes into account the influence of micromotion on the cooling dynamics. This thermometry applies to any initial energy distribution. We experimentally test our model with an ion prepared in a coherent, thermal and Tsallis energy distributions.