Nora Tischler

Electromagnetic Duality Symmetry and Helicity Conservation for the Macroscopic Maxwell’s Equations

In this Letter, we show that the electromagnetic duality symmetry, broken in the microscopic Maxwells equations by the presence of charges, can be restored for the macroscopic Maxwells equations. The restoration of this symmetry is shown to be independent of the geometry of the problem. These results provide a tool for the study of light-matter interactions within the framework of symmetries and conservation laws. We illustrate its use by determining the helicity content of the natural modes of structures possessing spatial inversion symmetries and by elucidating the root causes for some surprising effects in the scattering off magnetic spheres.

Necessary symmetry conditions for the rotation of light

Two conditions on symmetries are identified as necessary for a linear scattering system to be able to rotate the linear polarization of light: Lack of at least one mirror plane of symmetry and electromagnetic duality symmetry. Duality symmetry is equivalent to the conservation of the helicity of light in the same way that rotational symmetry is equivalent to the conservation of angular momentum. When the system is a solution of a single species of particles, the lack of at least one mirror plane of symmetry leads to the familiar requirement of chirality of the individual particle. With respect to helicity preservation, according to the analytical and numerical evidence presented in this paper, the solution preserves helicity if and only if the individual particle itself preserves helicity. However, only in the particular case of forward scattering the helicity preservation condition on the particle is relaxed: We show that the random orientation of the molecules endows the solution with an effective rotational symmetry; at its turn, this leads to helicity preservation in the forward scattering direction independently of any property of the particle. This is not the case for a general scattering direction. These results advance the current understanding of the phenomena of molecular optical activity and provide insight for the design of polarization control devices at the nanoscale.

On small beams with large topological charge

Light beams can carry a discrete, in principle unbounded amount of angular momentum. Examples of such beams, the Laguerre-Gauss modes, are frequently expressed as solutions of the paraxial wave equation. There, they are eigenstates of the orbital angular momentum (OAM) operator. The paraxial solutions predict that beams with large OAM could be used to resolve arbitrarily small distances - a dubious situation. Here we show how to solve that situation by calculating the properties of beams free from the paraxial approximation. We find the surprising result that indeed one can resolve smaller distances with larger OAM, although with decreased visibility. If the visibility is kept constant (for instance at the Rayleigh criterion, the limit where two points are reasonably distinguishable), larger OAM does not provide an advantage. The drop in visibility is due to a field in the direction of propagation, which is neglected within the paraxial limit.

Scattering in multilayered structures : diffraction from a nanohole

The spectral expansion of the Greens tensor for a planar multilayered structure allows us to semianalytically obtain the angular spectrum representation of the field scattered by an arbitrary dielectric perturbation present in the structure. In this paper we present a method to find the expansion coefficients of the scattered field, given that the electric field inside the perturbation is available. The method uses a complete set of orthogonal vector wave functions to solve the structures vector wave equation. In the two semi-infinite bottom and top media, those vector wave functions coincide with the plane-wave basis vectors, including both propagating and evanescent components. The technique is used to obtain the complete angular spectrum of the field scattered by a nanohole in a metallic film under Gaussian illumination. We also show how the obtained formalism can easily be extended to spherically and cylindrically multilayered media. In those cases, the expansion coefficients would multiply the spherical and cylindrical vector wave functions.

Simulations of the effect of waveguide cross-section on quantum dot-plasmon coupling

Quantum dot–plasmon waveguide systems are of interest for the active control of plasmon propagation, and consequently, the development of active nanophotonic devices such as nano-sized optical transistors. This paper is concerned with how varying aspect ratio of the waveguide cross-section affects the quantum dot–plasmon coupling. We compare a stripe waveguide with an equivalent nanowire, illustrating that both waveguides have a similar coupling strength to a nearby quantum dot for small waveguide cross-section, thereby indicating that stripe lithographic waveguides have strong potential use in quantum dot–plasmon waveguide systems. We also demonstrate that changing the aspect ratio of both stripe and wire waveguides can increase the spontaneous emission rate of the quantum dot into the plasmon mode, by up to a factor of five. The results of this paper will contribute to the optimisation of quantum dot–plasmon waveguide systems and help pave the way for the development of active nanophotonics devices.

Measurement and Shaping of Biphoton Spectral Wave Functions

In this work we present a simple method to reconstruct the complex spectral wave function of a biphoton, and hence gain complete information about the spectral and temporal properties of a photon pair. The technique, which relies on quantum interference, is applicable to biphoton states produced with a monochromatic pump when a shift of the pump frequency produces a shift in the relative frequencies contributing to the biphoton. We demonstrate an example of such a situation in type-II parametric down conversion allowing arbitrary paraxial spatial pump and detection modes. Moreover, our test cases demonstrate the possibility to shape the spectral wave function. This is achieved by choosing the spatial mode of the pump and of the detection modes, and takes advantage of spatiotemporal correlations.

The role of angular momentum in the construction of electromagnetic multipolar fields

Multipolar solutions of Maxwells equations are used in many practical applications and are essential for the understanding of light–matter interactions at the fundamental level. Unlike the set of plane wave solutions of electromagnetic fields, the multipolar solutions do not share a standard derivation or notation. As a result, expressions originating from different derivations can be difficult to compare. Some of the derivations of the multipolar solutions do not explicitly show their relation to the angular momentum operators, thus hiding important properties of these solutions. In this paper, the relation between two of the most common derivations of this set of solutions is explicitly shown and their relation to the angular momentum operators is exposed.

Quantum optical rotatory dispersion

A technique for multiwavelength phase measurements with quantum light is proposed and applied to the study of optical activity. The phenomenon of molecular optical activity manifests itself as the rotation of the plane of linear polarization when light passes through chiral media. Measurements of optical activity and its wavelength dependence, that is, optical rotatory dispersion, can reveal information about intricate properties of molecules, such as the three-dimensional arrangement of atoms comprising a molecule. Given a limited probe power, quantum metrology offers the possibility of outperforming classical measurements. This has particular appeal when samples may be damaged by high power, which is a potential concern for chiroptical studies. We present the first experiment in which multiwavelength polarization-entangled photon pairs are used to measure the optical activity and optical rotatory dispersion exhibited by a solution of chiral molecules. Our work paves the way for quantum-enhanced measurements of chirality, with potential applications in chemistry, biology, materials science, and the pharmaceutical industry. The scheme that we use for probing wavelength dependence not only allows one to surpass the information extracted per photon in a classical measurement but also can be used for more general differential measurements.

Strong Unitary and Overlap Uncertainty Relations: Theory and Experiment

We derive and experimentally investigate a strong uncertainty relation valid for any n unitary operators, which implies the standard uncertainty relation and others as special cases, and which can be written in terms of geometric phases. It is saturated by every pure state of any n-dimensional quantum system, generates a tight overlap uncertainty relation for the transition probabilities of any n+1 pure states, and gives an upper bound for the out-of-time-order correlation function. We test these uncertainty relations experimentally for photonic polarization qubits, including the minimum uncertainty states of the overlap uncertainty relation, via interferometric measurements of generalized geometric phases.

Photonic entanglement processing with a single sub-wavelength structure

The progress in quantum information theory and the advances in the manipulation and control of quantum systems promise the advent of an era where quantum technologies will significantly change the fields of communication, computation and sensors. Even though some of these new technologies have already been successfully implemented, such as quantum key distribution [1] and quantum clocks [2], to fully develop the potential of these technologies we need to find new compact, reliable and robust quantum systems. In particular, we need to be able to control and process the elusive and delicate features of quantum entangled states, which are at the core of quantum technologies. In this sense, quantum photonics arises as one mature technology where most of the quantum information building blocks have been demonstrated. Most of the achievements in quantum photonics are hindered by the same limitations as the classical processing of light: weak interactions with matter, which impede efficient nonlinear processes, and large devices with dimensions many times the wavelength of light. Plasmonic devices may hold the key to overcome these hurdles due to strong interaction with light, small volumes of interaction, and the possibility to engineer and fabricate suitable nanostructures to address particular tasks [3].