O. Cyr-Choinière

Broken rotational symmetry in the pseudogap phase of a high-Tc superconductor

The nature of the pseudogap phase is a central problem in the effort to understand the high-transition-temperature (high-Tc) copper oxide superconductors. A fundamental question is what symmetries are broken when the pseudogap phase sets in, which occurs when the temperature decreases below a value T*. There is evidence from measurements of both polarized neutron diffraction and the polar Kerr effect that time-reversal symmetry is broken, but at temperatures that differ significantly from one another. Broken rotational symmetry was detected from both resistivity measurements and inelastic neutron scattering at low doping, and from scanning tunnelling spectroscopy at low temperature, but showed no clear relation to T*. Here we report the observation of a large in-plane anisotropy of the Nernst effect in YBa2Cu3Oy that sets in precisely at T* throughout the doping phase diagram. We show that the CuO chains of the orthorhombic lattice are not responsible for this anisotropy, which is therefore an intrinsic property of the CuO2 planes. We conclude that the pseudogap phase is an electronic state that strongly breaks four-fold rotational symmetry. This narrows the range of possible states considerably, pointing to stripe or nematic order.

Lifshitz critical point in the cuprate superconductor YBa2Cu3Oy from high-field Hall effect measurements

The Hall coefficient RH of the cuprate superconductor YBa 2Cu3Oy was measured in magnetic fields up to 60 T for a hole concentration p from 0.078 to 0.152 in the underdoped regime. In fields large enough to suppress superconductivity, RH(T) is seen to go from positive at high temperature to negative at low temperature, for p0.08. This change of sign is attributed to the emergence of an electron pocket in the Fermi surface at low temperature. At p<0.08, the normal-state R H(T) remains positive at all temperatures, increasing monotonically as T→0. We attribute the change of behavior across p=0.08 to a Lifshitz transition, namely a change in Fermi-surface topology occurring at a critical concentration pL=0.08, where the electron pocket vanishes. The loss of the high-mobility electron pocket across pL coincides with a tenfold drop in the conductivity at low temperature, revealed in measurements of the electrical resistivity ρ at high fields, showing that the so-called metal-insulator crossover of cuprates is in fact driven by a Lifshitz transition. It also coincides with a jump in the in-plane anisotropy of ρ, showing that without its electron pocket, the Fermi surface must have strong twofold in-plane anisotropy. These findings are consistent with a Fermi-surface reconstruction caused by a unidirectional spin-density wave or stripe order.

Linear temperature dependence of resistivity and change in the Fermi surface at the pseudogap critical point of|[nbsp]|a|[nbsp]|high-Tc superconductor

Transport measurements in a high-temperature superconductor provide evidence that the so-called pseudogap phase ends at a quantum critical point located inside the superconducting dome in the phase diagram of cuprates.

Direct measurement of the upper critical field in cuprate superconductors

In the quest to increase the critical temperature Tc of cuprate superconductors, it is essential to identify the factors that limit the strength of superconductivity. The upper critical field Hc2 is a fundamental measure of that strength, yet there is no agreement on its magnitude and doping dependence in cuprate superconductors. Here we show that the thermal conductivity can be used to directly detect Hc2 in the cuprates YBa2Cu3Oy, YBa2Cu4O8 and Tl2Ba2CuO6+δ, allowing us to map out Hc2 across the doping phase diagram. It exhibits two peaks, each located at a critical point where the Fermi surface of YBa2Cu3Oy is known to undergo a transformation. Below the higher critical point, the condensation energy, obtained directly from Hc2, suffers a sudden 20-fold collapse. This reveals that phase competition—associated with Fermi-surface reconstruction and charge-density-wave order—is a key limiting factor in the superconductivity of cuprates.

Enhancement of the Nernst effect by stripe order in a high-Tc superconductor

The Nernst effect in metals is highly sensitive to two kinds of phase transition: superconductivity and density-wave order. The large, positive Nernst signal observed in hole-doped high-Tc superconductors above their transition temperature (Tc) has so far been attributed to fluctuating superconductivity. Here we report that in some of these materials the large Nernst signal is in fact the result of stripe order, a form of spin/charge modulation that causes a reconstruction of the Fermi surface. In La2-xSrxCuO4 (LSCO) doped with Nd or Eu, the onset of stripe order causes the Nernst signal to change from being small and negative to being large and positive, as revealed either by lowering the hole concentration across the quantum critical point in Nd-doped LSCO (refs 6–8) or by lowering the temperature across the ordering temperature in Eu-doped LSCO (refs 9, 10). In the second case, two separate peaks are resolved, respectively associated with the onset of stripe order at high temperature and superconductivity near Tc.

Decrease of upper critical field with underdoping in cuprate superconductors

Decreasing the doping of a cuprate superconductor below a certain critical value causes its critical temperature to fall, however the reason for this has been unclear. Sensitive measurements of the Nernst effect in yttrium barium copper oxide suggest it is the result of competition with an emerging stripe phase.

Hall, Seebeck, and Nernst Coefficients of Underdoped HgBa_{2}CuO_{4+δ}: Fermi-Surface Reconstruction in an Archetypal Cuprate Superconductor

A key to understanding high-temperature superconductivity in cuprates lies in the identification of competing electronic phases in these materials. In YBa

Two types of nematicity in the phase diagram of the cuprate superconductor YBa 2 Cu 3 O y

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Fermi-surface transformation across the pseudogap critical point of the cuprate superconductor La1.6-xNd0.4SrxCuO4

Cu

Pseudogap phase of cuprate superconductors confined by Fermi surface topology

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