Olivier Chalus

Mid-IR short-pulse OPCPA with micro-Joule energy at 100kHz

We present a novel mid-IR source based on optical parametric chirped pulse amplification (OPCPA) generating 96 fs pulses (9.0 cycles) at 3.2 mm with an energy of 1.2 microJ, at a repetition rate of 100 kHz. The amplified spectrum supports a minimum Fourier transform limited pulse duration of 45 fs, or 4.2 cycles. Our use of OPCPA allows the direct amplification of few-cycle pulses at this mid-IR wavelength, and is inherently scalable to higher energies. The seed source for the system is based on difference frequency generation (DFG) between two outputs of the same fibre laser: this source is expected to be intrinsically CEP stable.

Sub-250-mrad, passively carrier–envelope-phase-stable mid-infrared OPCPA source at high repetition rate

An all-optical and passively carrier-to-envelope-phase-stabilized (CEP-stabilized) optical parametric chirped pulse amplification (OPCPA) system is demonstrated with sub-250-mrad CEP stability over 11 min and better than 100 mrad over 11 s. This is achieved without any electronic CEP stabilization loop for 160 kHz pulse repetition rate in the few cycle regime.

Six-cycle mid-infrared source with 3.8 μJ at 100 kHz

We report on the shortest pulses to date from a mid-IR optical parametric chirped pulse amplification: 67 fs duration with 3.8 μJ energy operating at 3.2 μm. The system is all solid state and diode pumped and operates at 100 kHz with unprecedented power stability of 0.75%rms over 30 min.

Spatiotemporal amplitude and phase retrieval of space-time coupled ultrashort pulses using the Shackled-FROG technique

We demonstrate the validity of the Shackled-frequency-resolved-optical-gating technique for the complete characterization, both in space and in time, of ultrashort optical pulses that present strong angular dispersion. Combining a simple imaging grating with a Hartmann-Shack sensor and standard frequency-resolved-optical-gating detection at a single spatial position, we are able to retrieve the full spatiotemporal structure of a tilted pulse.

Optical amplification in the near-infrared in gas-filled hollow-core fibers

We demonstrate efficient optical parametric amplification and generation in a gas-filled hollow-core fiber of near-infrared pulses, peaked at 1.4 microm wavelength, with 5 microJ energy and 45 fs duration at the fiber output. Numerical simulations confirm that the OPA is phase matched through excitation of higher-order fiber modes.

Suppression of parasitic lasing in high energy, high repetition rate Ti:sapphire laser amplifiers

Transverse parasitic lasing is well known for limiting the signal gain and the pulse energy that can be extracted from Ti:sapphire petawatt amplifiers. We have developed a technique for suppressing these parasitic lasing modes based on perfect refractive index-matching liquid doped with a broad-bandwidth absorber to suppress the transverse lasing while ensuring proper heat removal from the Ti:sapphire crystal. The 800 nm laser output with a bandwidth of 41 nm (FWHM) and peak energy of 22.7 J at a repetition rate of 1 Hz is demonstrated.

Ultrashort pulse characterization in the mid-infrared

We describe a second-harmonic-generation frequency-resolved optical gating measurement device optimized for the characterization of few-cycle pulses in the mid-IR spectral range. The system has a temporal range of 100 ps with resolution of 0.12 fs, and it is capable of measuring pulses as short as 1.5 cycles (15 fs) at 3 microm. Through interchangeable beam splitters and detectors it covers a wavelength range from 800 nm to 5 microm with up to 0.5 cm(-1) resolution. We demonstrate measurement of a richly featured 3.2 microm pulse with 9.6 cycle duration, recovering the main pulse of 96 fs, as well as low-intensity post-pulses with picosecond offset. We also characterize a 100 fs pulse after dispersion through a 1 cm sapphire plate, comparing the measured phase difference with the calculated one.

Design and simulation of few-cycle optical parametric chirped pulse amplification at mid-IR wavelengths

We present a design for a novel carrier to envelope phase stable optical parametric chirped pulse amplification source in the mid-infrared. We calculate the amplification of a 3.1µm seed pulse, generated via DFG from a two-colour fibre laser, using a fully three dimensional OPCPA code. We combine this with a ray-tracing code to model pulse compression using a grating compressor and a deformable mirror for programmable phase compensation. The simulation models the complete system based on FROG measurements of the commercially available fibre laser, ensuring the simulation is realistic. The obtained results indicate energetic pulses of 56 fs duration, corresponding to 5.2 cycles, can be produced with calculated pulse energies of up to 9.6µJ at a central wavelength of 3.3µm.

Accuracy measurements and improvement for complete characterization of optical pulses from nonlinear processes via multiple spectral-shearing interferometry.

We demonstrate that multiple spectral-shearing interferometry increases the precision and accuracy of measurements of the spectral phase of a complex pulse (time-bandwidth product = 125) arising from self-phase modulation in a gas filled capillary. We verify that the measured interferometric phase is accurate to 0.1 rad across the full bandwidth by checking the consistency between the spectral phases of each individual shear measurement. The accuracy of extracting pulse parameters (group delay dispersion, pulse duration and peak intensity) for single shear measurements were verified to better than 10% by comparison with the multishear reconstruction. High order space-time coupling is quantified across a single transverse dimension, verifying the suitability of such pulses for use in strong field experiments.

Design and simulation of few-cycle optical parametric chirped pulse amplication at mid-IR wavelengths

We present a design for a novel carrier to envelope phase stable OPCPA source in the mid-infrared. The obtained results indicate pulses of 56 fs duration, with pulse energies of 9.6 µJ at a central wavelength of 3.3 µm.