P. Pedri

Probing spin dynamics from the Mott insulating to the superfluid regime in a dipolar lattice gas

We analyze the spin dynamics of an out-of-equilibrium large spin dipolar atomic Bose gas in an optical lattice. We observe a smooth crossover from a complex oscillatory behavior to an exponential behavior throughout the Mott-to-superfluid transition. While both of these regimes are well described by our theoretical models, we provide data in the intermediate regime where dipolar interactions, contact interactions, and superexchange mechanisms compete. In this strongly correlated regime, spin dynamics and transport are coupled, which challenges theoretical models for quantum magnetism.

Nonequilibrium quantum magnetism in a dipolar lattice gas.

We report on the realization of quantum magnetism using a degenerate dipolar gas in an optical lattice. Our system implements a lattice model resembling the celebrated t-J model. It is characterized by a nonequilibrium spinor dynamics resulting from intersite Heisenberg-like spin-spin interactions provided by nonlocal dipole-dipole interactions. Moreover, due to its large spin, our chromium lattice gases constitute an excellent environment for the study of quantum magnetism of high-spin systems, as illustrated by the complex spin dynamics observed for doubly occupied sites.

Spontaneous Demagnetization of a Dipolar Spinor Bose Gas in an Ultralow Magnetic Field

We study the spinor properties of S = 3 (52)Cr condensates, in which dipole-dipole interactions allow changes in magnetization. We observe a demagnetization of the Bose-Einstein condensate (BEC) when the magnetic field is quenched below a critical value corresponding to a phase transition between a ferromagnetic and a nonpolarized ground state, which occurs when spin-dependent contact interactions overwhelm the linear Zeeman effect. The critical field is increased when the density is raised by loading the BEC in a deep 2D optical lattice. The magnetization dynamics is set by dipole-dipole interactions.

Phonon Instability with Respect to Soliton Formation in Two-Dimensional Dipolar Bose-Einstein Condensates

The partially attractive character of the dipole-dipole interaction leads to phonon instability in dipolar condensates, which is followed by collapse in three-dimensional geometries. We show that the nature of this instability is fundamentally different in two-dimensional condensates, due to the dipole-induced stabilization of two-dimensional bright solitons. As a consequence, a transient gas of attractive solitons is formed, and collapse may be avoided. In the presence of an harmonic confinement, the instability leads to transient pattern formation followed by the creation of stable two-dimensional solitons. This dynamics should be observable in on-going experiments, allowing for the creation of stable two-dimensional solitons for the first time ever in quantum gases.

Anisotropic excitation spectrum of a dipolar quantum Bose gas.

We measure the excitation spectrum of a dipolar chromium Bose-Einstein condensate with Raman-Bragg spectroscopy. The energy spectrum depends on the orientation of the dipoles with respect to the excitation momentum, demonstrating an anisotropy that originates from the dipole-dipole interactions between the atoms. We compare our results with the Bogoliubov theory based on the local density approximation and, at large excitation wavelengths, with the numerical simulations of the time-dependent Gross-Pitaevskii equation. Our results show an anisotropy of the speed of sound.

Collective excitations of a dipolar Bose-Einstein condensate.

We have measured the effect of dipole-dipole interactions on the frequency of a collective mode of a Bose-Einstein condensate. At relatively large numbers of atoms, the experimental measurements are in good agreement with zero temperature theoretical predictions based on the Thomas-Fermi approach. Experimental results obtained for the dipolar shift of a collective mode show a larger dependency to both the trap geometry and the atom number than the ones obtained when measuring the modification of the condensate aspect ratio due to dipolar forces. These findings are in good agreement with simulations based on a Gaussian ansatz.

Stability of Dark Solitons in Three Dimensional Dipolar Bose-Einstein Condensates

The dynamical stability of dark solitons in dipolar Bose-Einstein condensates is studied. For standard short-range interacting condensates, dark solitons are unstable against transverse excitations in two and three dimensions. On the contrary, due to its nonlocal character, the dipolar interaction allows for stable 3D stationary dark solitons, opening a qualitatively novel scenario in nonlinear atom optics. We discuss in detail the conditions to achieve this stability, which demand the use of an additional optical lattice, and the stability regimes.

Spin Relaxation and Band Excitation of a Dipolar Bose-Einstein Condensate in 2D Optical Lattices

We observe interband transitions mediated by dipole-dipole interactions for an array of 1D quantum gases of chromium atoms, trapped in a 2D optical lattice. Interband transitions occur when dipolar relaxation releases an energy larger than the lattice band gap. For symmetric lattice sites, and a magnetic field parallel to the lattice axis, we compare the measured dipolar relaxation rate with a Fermi golden rule calculation. Below a magnetic field threshold, we obtain an almost complete suppression of dipolar relaxation, leading to metastable 1D gases in the highest Zeeman state.

Resonant demagnetization of a dipolar Bose-Einstein condensate in a three-dimensional optical lattice

We study dipolar relaxation of a chromium BEC loaded into a 3D optical lattice. We observe dipolar relaxation resonances when the magnetic energy released during the inelastic collision matches an excitation towards higher energy bands. A spectroscopy of these resonances for two orientations of the magnetic field provides a 3D band spectroscopy of the lattice. The narrowest resonance is registered for the lowest excitation energy. Its line-shape is sensitive to the on-site interaction energy. We use such sensitivity to probe number squeezing in a Mott insulator, and we reveal the production of three-body states with entangled spin and orbital degrees of freedom.

Dipolar atomic spin ensembles in a double-well potential

We experimentally study the spin dynamics of mesoscopic ensembles of ultracold magnetic spin-3 atoms located in two separated wells of an optical dipole trap. We use a radio-frequency sweep to selectively flip the spin of the atoms in one of the wells, which produces two separated spin domains of opposite polarization. We observe that these engineered spin domains are metastable with respect to the long-range magnetic dipolar interactions between the two ensembles. The absence of inter-cloud dipolar spin-exchange processes reveals a classical behavior, in contrast to previous results with atoms loaded in an optical lattice. When we merge the two subsystems, we observe spin-exchange dynamics due to contact interactions which enable the first determination of the s-wave scattering length of 52Cr atoms in the S=0 molecular channel a_0=13.5^{+11}_{-10.5}a_B (where a_B is the Bohr radius).