Paul H. Kaye

The mean physical and optical properties of regional haze dominated by biomass burning aerosol measured from the C‐130 aircraft during SAFARI 2000

Original article can be found at: http://www.agu.org/journals/jd/ Copyright American Geophysical Union DOI: 10.1029/2002JD002226 [Full text of this article is not available in the UHRA]

Ice Particle Interarrival Times Measured with a Fast FSSP

Abstract Ice particle interarrival times have been measured with a fast forward scattering spectrometer probe (FSSP). The distribution of interarrival times is bimodal instead of the exponential distribution expected for a Poisson process. The interarrival time modes are located at ∼10−2 and ∼10−4 s. This equates to horizontal spacings on both the centimeter and meter scales. The characteristics of the interarrival times are well modeled by a Markov chain process that couples together two independent Poisson processes operating at different scales. The possibility that ice crystals shattering on the probe tip causes the bimodal interarrival times is explored and cannot be ruled out. If the observations are indicating real spacings of particles in clouds, then the observations show very localized (centimeter scale) concentrations of ∼100 s cm−3 embedded within an average concentration of typically ∼1 cm−3. If the localized high concentrations are produced by the ice crystals shattering, then the concentrat...

Single particle multichannel bio-aerosol fluorescence sensor

We describe a prototype low-cost multi-channel aerosol fluorescence sensor designed for unattended deployment in medium to large area bio-aerosol detection networks. Individual airborne particles down to ~1mum in size are detected and sized by measurement of light scattered from a continuous-wave diode laser (660nm). This scatter signal is then used to trigger the sequential firing of two xenon sources which irradiate the particle with UV pulses at ~280 nm and ~370 nm, optimal for excitation of bio-fluorophores tryptophan and NADH (nicotinamide adenine dinucleotide) respectively. For each excitation wavelength, fluorescence is detected across two bands embracing the peak emissions of the same bio-fluorophores. Current measurement rates are up to ~125 particles/s, corresponding to all particles for concentrations up to 1.3 x 104 particles/l. Developments to increase this to ~500 particles/s are in hand. Device sensitivity is illustrated in preliminary data recorded from aerosols of E.coli, BG spores, and a variety of non-biological materials.

Spatial light-scattering analysis as a means of characterizing and classifying non-spherical particles

The manner in which a particle scatters incident light is a function of the particles shape, its size, its structure and its orientation with respect to the illumination direction, as well as to the wavelength and polarization state of the light. The spatial intensity distribution of scattered light thus contains information by which the particle may often be classified or even identified. This paper briefly reviews the development of spatial light scattering analysis as an analytical and monitoring tool now finding application in areas as diverse as environmental monitoring, aerosol and hydrosol research, microbiology and fine-powder characterization. The paper concludes with a practical example of the use of spatial scattering analysis to achieve real-time discrimination of a specific particle type, namely airborne asbestos fibres.

The Ability of the Small Ice Detector (SID-2) to Characterize Cloud Particle and Aerosol Morphologies Obtained during Flights of the FAAM BAe-146 Research Aircraft

Abstract The Small Ice Detector mark 2 (SID-2), which was built by the University of Hertfordshire, has been operated by the Met Office on the Facility for Atmospheric Airborne Research (FAAM) BAe-146 aircraft during a large number of flights. The flights covered a wide range of atmospheric conditions, including stratocumulus, altocumulus lenticularis, cirrus, and mixed-phase cumulus clouds, as well as clear-sky flights over the sea and over desert surfaces. SID-2 is a laser scattering device that provides in situ data on cloud particle concentration and size. SID-2 also provides the spatial light scattering data from individual particles to give some information on the particle shape. The advantage of SID-2 is that it can characterize the cloud particle shape for particle sizes less than the resolutions of the more usual commercially available ice crystal imaging probes. The particle shape characteristics enable, for example, small just-nucleated ice particles to be discriminated from supercooled water d...

Discrimination of micrometre-sized ice and super-cooled droplets in mixed-phase cloud

Original article can be found at: http://www.sciencedirect.com/science/journal/13522310 Copyright Elsevier Ltd. DOI: 10.1016/S1352-2310(00)00377-0 [Full text of this article is not available in the UHRA]

A silicon micromachined device for use in blood cell deformability studies

An application of silicon micromachining to the analysis of blood cell rheology is described. The system, based upon a micromachined flow cell, provides a specific measurement of each cell in a statistically significant population in terms of both flow velocity profile and an index of cell volume while the cells flow through an array of microchannels. The rationale, design, and fabrication of the silicon micromachined flow cell is discussed. Interrelated considerations determining the design of the associated fluidic, mechanical, imaging, and real-time image analysis subsystems are examined. Sample data comparing normal and iron deficiency anaemic blood are presented to illustrate the potential of this technique.<<ETX>>

Classifying atmospheric ice crystals by spatial light scattering

We describe preliminary results from an optical scattering instrument designed to assess the shapes and sizes of microscopic atmospheric cloud particles, especially the smallest ice crystals, that can profoundly affect cloud processes and radiative properties. The new instrument captures high-resolution spatial light scattering patterns from individual particles down to approximately 1 microm in size passing through a focused laser beam. Its significance lies in the ability of these patterns to provide morphological data for particle sizes well below the optical resolution limits of current cloud particle probes.

Light scattering from deformed droplets and droplets with inclusions. I. Experimental results

We provide experimental results from the scattering of light by deformed liquid droplets and droplets with inclusions. The characterization of droplet deformation could lead to improved measurement of droplet size as measured by commercial aerodynamic particle-sizing instruments. The characterization of droplets with inclusions can be of importance in some industrial, occupational, and military aerosol monitoring situations. The nozzle assembly from a TSI Aerodynamic Particle Sizer was used to provide the accelerating flow conditions in which experimental data were recorded. A helium-neon laser was employed to generate the light-scattering data, and an externally triggered, pulsed copper vapor laser provided illumination for a droplet imaging system arranged orthogonal to the He-Ne scattering axis. The observed droplet deformation correlates well over a limited acceleration range with theoretical predictions derived from an analytical solution of the Navier-Stokes equation.

Incidence of rough and irregular atmospheric ice particles from Small Ice Detector 3 measurements

The knowledge of properties of ice crystals such as size, shape, concavity and roughness is critical in the context of radiative properties of ice and mixed-phase clouds. Limitations of current cloud probes to measure these properties can be circumvented by acquiring two-dimensional lightscattering patterns instead of particle images. Such patterns were obtained in situ for the first time using the Small Ice Detector 3 (SID-3) probe during several flights in a variety of mid-latitude mixed-phase and cirrus clouds. The patterns are analysed using several measures of pattern texture, selected to reveal the magnitude of particle roughness or complexity. The retrieved roughness is compared to values obtained from a range of well-characterized test particles in the laboratory. It is found that typical in situ roughness corresponds to that found in the rougher subset of the test particles, and sometimes even extends beyond the most extreme values found in the laboratory. In this study we do not differentiate between small-scale, fine surface roughness and large-scale crystal complexity. Instead, we argue that both can have similar manifestations in terms of light-scattering properties and also similar causes. Overall, the in situ data are consistent, with ice particles with highly irregular or rough surfaces being dominant. Similar magnitudes of roughness were found in growth and sublimation zones of cirrus. The roughness was found to be negatively correlated with the halo ratio, but not with other thermodynamic or microphysical properties found in situ. Slightly higher roughness was observed in cirrus forming in clean oceanic air masses than in a continental, polluted one. Overall, the roughness and complexity are expected to lead to increased shortwave cloud reflectivity, in comparison with cirrus composed of more regular, smooth ice crystal shapes. These findings put into question suggestions that climate could be modified through aerosol seeding to reduce cirrus cover and optical depth, as the seeding may result in decreased shortwave reflectivity.