Pavel Sidorenko

Phase matching of high harmonic generation in the soft and hard X-ray regions of the spectrum

We show how bright, tabletop, fully coherent hard X-ray beams can be generated through nonlinear upconversion of femtosecond laser light. By driving the high-order harmonic generation process using longer-wavelength midinfrared light, we show that, in theory, fully phase-matched frequency upconversion can extend into the hard X-ray region of the spectrum. We verify our scaling predictions experimentally by demonstrating phase matching in the soft X-ray region of the spectrum around 330 eV, using ultrafast driving laser pulses at 1.3-μm wavelength, in an extended, high-pressure, weakly ionized gas medium. We also show through calculations that scaling of the overall conversion efficiency is surprisingly favorable as the wavelength of the driving laser is increased, making tabletop, fully coherent, multi-keV X-ray sources feasible. The rapidly decreasing microscopic single-atom yield, predicted for harmonics driven by longer-wavelength lasers, is compensated macroscopically by an increased optimal pressure for phase matching and a rapidly decreasing reabsorption of the generated X-rays.

Sparse Phase Retrieval from Short-Time Fourier Measurements

We consider the classical 1D phase retrieval problem. In order to overcome the difficulties associated with phase retrieval from measurements of the Fourier magnitude, we treat recovery from the magnitude of the short-time Fourier transform (STFT). We first show that the redundancy offered by the STFT enables unique recovery for arbitrary nonvanishing inputs, under mild conditions. An efficient algorithm for recovery of a sparse input from the STFT magnitude is then suggested, based on an adaptation of the recently proposed GESPAR algorithm. We demonstrate through simulations that using the STFT leads to improved performance over recovery from the oversampled Fourier magnitude with the same number of measurements.

Sparsity-based super-resolved coherent diffraction imaging of one-dimensional objects

Phase-retrieval problems of one-dimensional (1D) signals are known to suffer from ambiguity that hampers their recovery from measurements of their Fourier magnitude, even when their support (a region that confines the signal) is known. Here we demonstrate sparsity-based coherent diffraction imaging of 1D objects using extreme-ultraviolet radiation produced from high harmonic generation. Using sparsity as prior information removes the ambiguity in many cases and enhances the resolution beyond the physical limit of the microscope. Our approach may be used in a variety of problems, such as diagnostics of defects in microelectronic chips. Importantly, this is the first demonstration of sparsity-based 1D phase retrieval from actual experiments, hence it paves the way for greatly improving the performance of Fourier-based measurement systems where 1D signals are inherent, such as diagnostics of ultrashort laser pulses, deciphering the complex time-dependent response functions (for example, time-dependent permittivity and permeability) from spectral measurements and vice versa.

Sawtooth grating-assisted phase-matching

A quasi-phase-matching method where the modulation has a sawtooth profile and the phase-mismatch is almost fully corrected is suggested. Schemes for implementing sawtooth grating-assisted-phase-matching in low-order as well as high-order harmonic generation are proposed.

On the Uniqueness of FROG Methods

The problem of recovering a signal from its power spectrum, called phase retrieval, arises in many scientific fields. One of many examples is ultrashort laser pulse characterization, in which the electromagnetic field is oscillating with

Ptychographic ultrahigh-speed imaging

\sim{\text{10}}^{15}

Sparsity-based super-resolution coherent diffractive imaging of (practically) 1D images using extreme UV radiation

Hz and phase information cannot be measured directly due to limitations of the electronic sensors. Phase retrieval is ill-posed in most of the cases, as there are many different signals with the same Fourier transform magnitude. To overcome this fundamental ill-posedness, several measurement techniques are used in practice. One of the most popular methods for complete characterization of ultrashort laser pulses is the frequency-resolved optical gating (FROG). In FROG, the acquired data are the power spectrum of the product of the unknown pulse with its delayed replica. Therefore, the measured signal is a quartic function of the unknown pulse. A generalized version of FROG, where the delayed replica is replaced by a second unknown pulse, is called blind FROG. In this case, the measured signal is quadratic with respect to both pulses. In this letter, we introduce and formulate FROG-type techniques. We then show that almost all band-limited signals are determined uniquely, up to trivial ambiguities, by blind FROG measurements (and thus also by FROG), if in addition we have access to the signals power spectrum.

Self-phase modulation spectral broadening in two-dimensional spatial solitons: toward three-dimensional spatiotemporal pulse-train solitons

We propose and demonstrate numerically a simple method for ultrahigh-speed imaging of complex (amplitude and phase) samples. Our method exploits redundancy in single-shot ptychography (SSP) for reconstruction of multiple frames from a single camera snapshot. We term the method Time-resolved Imaging by Multiplexed Ptychography (TIMP). We demonstrate TIMP numerically-reconstructing 15 frames of a complexed-valued dynamic object from a single noisy camera snapshot. Experimentally, we demonstrate SSP with single pulse illumination with pulse duration of 150 psec, where its spectral bandwidth can support 30 fsec pulses.

Super-resolution spectroscopy by compact representation

We demonstrate experimentally sparsity-based super-resolution of coherent diffraction imaging (CDI) with extreme UV radiation. We also present the first experimental CDI of a practically one-dimensional object, overcoming the well-known ambiguity problem in one-dimensional phase retrieval.

Several new directions for ultrafast fiber lasers [Invited]

We demonstrate self-phase modulation (SPM) spectral broadening in two-dimensional solitons in homogeneous media using two different schemes. In the active mode, a train of pulses are collectively trapped and form a spatial soliton through a photorefractive, slowly responding, and electronically controlled self-focusing nonlinearity, and each pulse experiences spectral broadening by the fast SPM nonlinearity. In the passive mode, the pulse-train beam is guided in a waveguide that is optically induced by a continuous-wave thermal spatial soliton. The soliton formation increased the normalized spectral broadening factor from 0.5% up to 197%. This experiment presents significant progress toward the experimental demonstration of three-dimensional spatiotemporal pulse-train solitons.