Pierre-Ambroise Lacourt

High aspect ratio nanochannel machining using single shot femtosecond Bessel beams

We report high aspect ratio nanochannel fabrication in glass using single-shot femtosecond Bessel beams of sub-3u2002μJ pulse energies at 800 nm. We obtain near-parallel nanochannels with diameters in the range 200–800 nm, and aspect ratios that can exceed 100. An array of 230 nm diameter channels with 1.6u2002μm pitch illustrates the reproducibility of this approach and the potential for writing periodic structures. We also report proof-of-principle machining of a through-channel of 400 nm diameter in a 43u2002μm thick membrane. These results represent a significant advance of femtosecond laser ablation technology into the nanometric regime.

Real-time full bandwidth measurement of spectral noise in supercontinuum generation

The ability to measure real-time fluctuations of ultrashort pulses propagating in optical fiber has provided significant insights into fundamental dynamical effects such as modulation instability and the formation of frequency-shifting rogue wave solitons. We report here a detailed study of real-time fluctuations across the full bandwidth of a fiber supercontinuum which directly reveals the significant variation in measured noise statistics across the spectrum, and which allows us to study correlations between widely separated spectral components. For two different propagation distances corresponding to the onset phase of spectral broadening and the fully-developed supercontinuum, we measure real time noise across the supercontinuum bandwidth, and we quantify the supercontinuum noise using statistical higher-order moments and a frequency-dependent intensity correlation map. We identify correlated spectral regions within the supercontinuum associated with simultaneous sideband generation, as well as signatures of pump depletion and soliton-like pump dynamics. Experimental results are in excellent agreement with simulations.

High aspect ratio taper-free microchannel fabrication using femtosecond Bessel beams

We present a systematic study of femtosecond laser microchannel machining in glass using nondiffracting Bessel beams. In particular, our results identify a source and focusing parameter working window where high aspect ratio taper-free microchannels can be reproducibly produced without sample translation. With appropriate source parameters, we machine channels of 2 microm diameter and with aspect ratios up to 40. We propose the filamentation stability of the Bessel beam propagation as the critical factor underlying the controlled and reproducible results that have been obtained.

Arbitrary accelerating micron-scale caustic beams in two and three dimensions

We generate arbitrary convex accelerating beams by direct application of an appropriate spatial phase profile on an incident Gaussian beam. The spatial phase calculation exploits the geometrical properties of optical caustics and the Legendre transform. Using this technique, accelerating sheet caustic beams with parabolic profiles (i.e. Airy beams), as well as quartic and logarithmic profiles are experimentally synthesized from an incident Gaussian beam, and we show compatibility with material processing applications using an imaging system to reduce the main intensity lobe at the caustic to sub-10 micron transverse dimension. By applying additional and rotational spatial phase, we generate caustic-bounded sheet and volume beams, which both show evidence of the recently predicted effect of abrupt autofocussing. In addition, an engineered accelerating profile with femtosecond pulses is applied to generate a curved zone of refractive index modification in glass. These latter results provide proof of principle demonstration of how this technique may yield new degrees of freedom in both nonlinear optics and femtosecond micromachining.

Micromachining along a curve: Femtosecond laser micromachining of curved profiles in diamond and silicon using accelerating beams

We report femtosecond laser micromachining of micron-size curved structures using tailored accelerating beams. We report surface curvatures as small as 70u2009μm in both diamond and silicon, which demonstrates the wide applicability of the technique to materials that are optically transparent or opaque at the pump laser wavelength. We also report the machining of curved trenches in silicon. Our results are consistent with an ablation-threshold model based on calculated local beam intensity, and we also observe asymmetric debris deposition which is interpreted in terms of the optical properties of the incident accelerating beam.

Sending femtosecond pulses in circles: highly nonparaxial accelerating beams

We use caustic beam shaping on 100 fs pulses to experimentally generate nonparaxial accelerating beams along a 60° circular arc, moving laterally by 14 µm over a 28 µm propagation length. This is the highest degree of transverse acceleration reported to our knowledge. Using diffraction integral theory and numerical beam propagation simulations, we show that circular acceleration trajectories represent a unique class of nonparaxial diffraction-free beam profile which also preserves the femtosecond temporal structure in the vicinity of the caustic.

Surface nanoprocessing with nondiffracting femtosecond Bessel beams

We demonstrate the application of nondiffracting Bessel beams for reproducible nanometric-scale feature patterning in glass. A femtosecond pulse zero-order Bessel beam with a central spot radius of 360 nm was used to write 500 nm radius nanocraters over a longitudinal positioning range exceeding 20 microm, with a variation in radius of less than 10%. The use of Bessel beams significantly reduces constraints on critical sample positioning in the nanoscale writing regime, enabling the use of femtosecond pulses for fast inscription of nanometer-scale features over large sample areas.

Milliwatt-peak-power pulse characterization at 1.55 µm by wavelength-conversion frequency-resolved optical gating

A novel wavelength-conversion configuration based on four-wave mixing in an optical fiber has been used to generate a frequency-resolved optical gating (FROG) trace identical to that obtained from second-harmonic generation (SHG). The use of an optical fiber waveguide permits enhanced measurement sensitivity compared with that of conventional SHG-FROG and has been used for complete characterization of 1-mW peak-power picosecond pulses at 1.55 microm from an unamplified semiconductor laser diode gain switched at 10 GHz.

Generation of Ultralow Jitter Optical Pulses Using Optoelectronic Oscillators With Time-Lens Soliton-Assisted Compression

In this paper, we propose a new approach for the generation of ultralow jitter optical pulses using optoelectronic microwave oscillators. The short pulses are obtained through time-lens soliton-assisted compression of sinusoidally modulated prepulses, which are self-started from a conventional single-loop optoelectronic oscillator. The inherent ultralow phase noise of optoelectronic oscillators is converted into ultralow timing jitter for the generated pulses. We provide a time-domain model for the slowly varying amplitudes of the microwave and optical oscillations, and our analytical study is confirmed by numerical simulations and experimental measurements. We demonstrate the generation of 4.1 ps pulses along with a microwave whose phase noise is -140 dBc/Hz at 10 kHz from the 10 GHz carrier, with 2.7 fs jitter in the 1-10 kHz frequency band.

Femtosecond laser fabrication of micro and nano-disks in single layer graphene using vortex Bessel beams

We report the fabrication of micro and nano-disks in single layer chemical vapor deposition graphene on glass substrate using femtosecond laser ablation with vortex Bessel beams. The fabricated graphene disks with diameters ranging from 650u2009nm to 4u2009μm were characterized by spatially resolved micro-Raman spectroscopy. The variation of ablation threshold was investigated as a function of the number of pulses showing an incubation effect. A very high degree of size control of the fabricated graphene disks is enabled using a sequence of femtosecond pulses with different vortex orders.