Pierre Olivier Bejot

Higher-order Kerr terms allow ionization-free filamentation in gases

We show that higher-order nonlinear indices (n(4), n(6), n(8), n(10)) provide the main defocusing contribution to self-channeling of ultrashort laser pulses in air and argon at 800 nm, in contrast with the previously accepted mechanism of filamentation where plasma was considered as the dominant defocusing process. Their consideration allows us to reproduce experimentally observed intensities and plasma densities in self-guided filaments.

Compression of 1.8 μm laser pulses to sub two optical cycles with bulk material

We demonstrate a simple scheme to generate 0.4 mJ 11.5 fs laser pulses at 1.8 μm. Optical parametrically amplified pulses are spectrally broadened by nonlinear propagation in an argon-filled hollow-core fiber and subsequently compressed to 1.9 optical cycles by linear propagation through bulk material in the anomalous dispersion regime. This pulse compression scheme is confirmed through numerical simulations.

Transition from Plasma-Driven to Kerr-Driven Laser Filamentation

While filaments are generally interpreted as a dynamic balance between Kerr focusing and plasma defocusing, the role of the higher-order Kerr effect (HOKE) is actively debated as a potentially dominant defocusing contribution to filament stabilization. In a pump-probe experiment supported by numerical simulations, we demonstrate the transition between two distinct filamentation regimes at 800 nm. For long pulses (1.2 ps), the plasma substantially contributes to filamentation, while this contribution vanishes for short pulses (70 fs). These results confirm the occurrence, in adequate conditions, of filamentation driven by the HOKE rather than by plasma.

White light generation over three octaves by femtosecond filament at 3.9 µm in argon

We report the first (to our knowledge) experimental results and numerical simulations on mid-IR femtosecond pulse filamentation in argon using 0.1 TW peak-power, 80 fs, 3.9 μm pulses. A broadband supercontinuum spanning the spectral range from 350 nm to 5 μm is generated, whereby about 4% of the mid-IR pulse energy is converted into the 350-1700 nm spectral region. These mid-IR-visible coherent continua offer a new, unique tool for time-resolved spectroscopy based on a mid-IR filamentation laser source.

Optimal control of filamentation in air

The authors demonstrate optimal control of the propagation of ultrashort, ultraintense (multiterawatt) laser pulses in air over distances up to 36m in a closed-loop scheme. They optimized three spectral ranges within the white-light continuum as well as the ionization efficiency. Optimization results in signal enhancements by typical factors of 2 and 1.4 for the target parameters. The optimization results in shorter pulses by reducing their chirp in the case of white-light continuum generation, while they correct the pulse from its defects and set the filamentation onset near the detector as far as air ionization is concerned.

High-Field Quantum Calculation Reveals Time-Dependent Negative Kerr Contribution

The exact quantum time-dependent optical response of hydrogen under strong-field near-infrared excitation is investigated and compared to the perturbative model widely used for describing the effective atomic polarization induced by intense laser fields. By solving the full 3D time-dependent Schrödinger equation, we exhibit a supplementary, quasi-instantaneous defocusing contribution missing in the weak-field model of polarization. We show that this effect is far from being negligible, in particular when closures of ionization channels occur and stems from the interaction of electrons with their parent ions. It provides an interpretation of the higher-order Kerr effect recently observed in various gases.

Mid-infrared laser filamentation in molecular gases

We observed the filamentation of mid-infrared ultrashort laser pulses (3.9 μm, 80 fs) in molecular gases. It efficiently generates a broadband supercontinuum over two octaves in the 2.5-6 μm spectral range, with a red-shift up to 500 nm due to the Raman effect, which dominates over the blue shift induced by self-steepening and the gas ionization. As a result, the conversion efficiency into the Stokes region (4.3-6 μm) 65% is demonstrated.

On negative higher-order Kerr effect and filamentation

As a contribution to the ongoing controversy about the role of higher-order Kerr effect (HOKE) in laser filamentation, we first provide thorough details about the protocol that has been employed to infer the HOKE indices from the experiment. Next, we discuss potential sources of artifact in the experimental measurements of these terms and show that neither the value of the observed birefringence, nor its inversion, nor the intensity at which it is observed, appear to be flawed. Furthermore, we argue that, independently on our values, the principle of including HOKE is straightforward. Due to the different temporal and spectral dynamics, the respective efficiency of defocusing by the plasma and by the HOKE is expected to depend substantially on both incident wavelength and pulse duration. The discussion should therefore focus on defining the conditions where each filamentation regime dominates.

32TW atmospheric white-light laser

Ultrahigh power laser pulses delivered by the Alise beamline (26J, 32TW pulses) have been sent vertically into the atmosphere. The highly nonlinear propagation of the beam in the air gives rise to more than 400 self-guided filaments. This extremely powerful bundle of laser filaments generates a supercontinuum propagating up to the stratosphere, beyond 20km. This constitutes the highest power “atmospheric white-light laser” to date.

Spectral dependence of purely-Kerr-driven filamentation in air and argon

Based on numerical simulations, we show that higher-order nonlinear indices (up to n{sub 8} and n{sub 10}, respectively) of air and argon have a dominant contribution to both focusing and defocusing in the self-guiding of ultrashort laser pulses over most of the spectrum. Plasma generation and filamentation are therefore decoupled. As a consequence, ultraviolet wavelength may not be the optimal wavelength for applications requiring to maximize ionization.