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Featured researches published by Qiming Liu.


Optics Letters | 2012

Three-dimensional photoprecipitation of oriented LiNbO 3 -like crystals in silica-based glass with femtosecond laser irradiation

Chaxing Fan; Bertrand Poumellec; Matthieu Lancry; Xuan He; Huidan Zeng; Abdel Erraji-Chahid; Qiming Liu; Guorong Chen

We demonstrate crystals (LiNbO(3)-like) that were space-selectively nucleated and grown in the bulk of silica-based glass by femtosecond laser irradiation at a high repetition rate (typ. 300 kHz). Oriented crystals with their polar axis mostly aligned with or perpendicular to the laser scanning direction have been fabricated by manipulation of the temperature gradient in adjusting the laser parameters. The mechanism for the orientation of femtosecond laser-induced crystallization is briefly discussed.


Journal of The Optical Society of America B-optical Physics | 2014

Size-controlled oriented crystallization in SiO 2 -based glasses by femtosecond laser irradiation

Xuan He; Chaxing Fan; Bertrand Poumellec; Qiming Liu; Huidan Zeng; François Brisset; Guorong Chen; Xiujian Zhao; Matthieu Lancry

3D nano-crystallization has been investigated with a femtosecond laser beam in 33Li2O-33Nb2O5-34SiO2 glass by changing the pulse energy and polarization direction. Electron backscattered diffraction was used to characterize the size and the orientation of crystals in cross sections of laser tracks, while second harmonic generation was employed to investigate the nonlinear optical properties of laser lines macroscopically. We are the first, to the best of our knowledge, to reveal that crystals of nano-size were precipitated both at low pulse energy with laser polarization parallel to the laser motion direction and at high pulse energy in the perpendicular case, but they preferred to orientate perpendicularly to the written lines in the former case.


Applied Physics Letters | 2006

Stability of electron-beam poling in N or Ge-doped H:SiO2 films

Qiming Liu; Bertrand Poumellec; R. Blum; G. Girard; J.E. Bourée; Alexandre Kudlinski; Gilbert Martinelli

We study the thermal stability of the second-harmonic signal in electron-beam poled silica based thin films developed for this application. Effects of N or Ge concentration as dopant, on one hand, and hydroxyl species, on the other hand, are tested. We conclude that water molecules inducing an ionic conductivity are detrimental to the e-beam poling efficiency and have to be avoided. Nevertheless, despite such precaution, the stability of the second-harmonic signal in an e-beam poled sample is worse than in a thermally poled sample.


Optics Letters | 2014

One-step photoinscription of asymmetrically oriented fresnoite-type crystals in glass by ultrafast laser.

Xuan He; Bertrand Poumellec; Qiming Liu; François Brisset; Matthieu Lancry

Oriented fresnoite-type crystals (Sr(2)TiSi(2)O(8)) were photoinduced directly in bulk silica-based glass by femtosecond laser irradiation at high repetition rate (typ. 300 kHz). Unlike related results obtained from other researchers, asymmetrical polar-axis orientation of those nonlinear crystals in transverse direction of the cross section has been demonstrated by electron backscattered diffraction and micro-second-harmonic generation (SHG). The nonlinear optical property of laser lines has been further characterized by SHG measurement. We found that the preferential directions of the polar axis were in the laser motion direction with a small dispersion in part of the heated volume. The other part of the crystallized volume shows an axis perpendicular to the writing direction. The mechanism of asymmetric orientation of femtosecond-laser-induced crystallization also is discussed.


Optics Letters | 2012

Origin of thermally induced second harmonic generation in PbO–B 2 O 3 glasses

Qiming Liu; Jincheng Du

Optical second harmonic generation (SHG) with second-order nonlinearity χ((2)) as high as 2.1 pm/V has been achieved in water quenched PbO-B(2)O(3) glasses. No nonlinear depletion layer or microcrystals were observed in these glasses and the mechanism for nonlinearity has been explored in this Letter. Our results show that the possible mechanism for SHG in these glasses can be attributed to their low thermal conductivity that led to a large surface stress gradient, which broke the inversion symmetry of the glasses and subsequently induced the nonlinear effect. These findings suggest that low thermal conductivity induced high stress gradients to lead to large SHG.


Journal of Non-crystalline Solids | 2013

Optical non-linearity in nano- and micro-crystallized glasses

Haizheng Tao; Xiujian Zhao; Qiming Liu


Journal of Non-crystalline Solids | 2011

Third-order nonlinearity in Ag-nanoparticles embedded 56GeS2–24Ga2S3–20KBr chalcohalide glasses

Qiming Liu; Xuan He; Xiong Zhou; Feng Ren; Xiangheng Xiao; Changzhong Jiang; Hui Zhou; Xiujian Zhao; Liping Lu; Shixiong Qian


Journal of Nanoparticle Research | 2011

Enhancement of third-order nonlinearity in Ag-nanoparticles-contained chalcohalide glasses

Qiming Liu; Xuan He; Xiujian Zhao; Feng Ren; Xiangheng Xiao; Changzhong Jiang; Xiong Zhou; Liping Lu; Hui Zhou; Shixiong Qian; Bertrand Poumellec; Matthieu Lancry


Chemical Physics Letters | 2009

Synthesis and second-order optical nonlinearity of DAMS/Mn2P2S6 intercalated materials by ion exchange method

Qiming Liu; Wei Zhou; Chang Gao; Ting Hu; Xiujian Zhao


Optical Materials | 2009

Ultrafast third-order optical non-linearity of 0.56GeS2―0.24Ga2S3―0.2KX(X = Cl, Br, I) chalcohalide glasses by femtosecond Optical Kerr Effect

Qiming Liu; Chang Gao; Hui Zhou; Benqiang Lu; Xuan He; Qian Shi-Xiong; Xiujian Zhao

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Xiujian Zhao

Wuhan University of Technology

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Chang Gao

Wuhan University of Technology

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Xuan He

Wuhan University of Technology

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Xuan He

Wuhan University of Technology

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Ting Hu

Wuhan University of Technology

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