R.-D. Herzberg

The GREAT spectrometer

Abstract The GREAT spectrometer is designed to measure the decay properties of reaction products transported to the focal plane of a recoil separator. GREAT comprises a system of silicon, germanium and gas detectors optimised for detecting the arrival of the reaction products and correlating with any subsequent radioactive decay involving the emission of protons, α particles, β particles, γ rays, X-rays or conversion electrons. GREAT can either be employed as a sensitive stand-alone device for decay measurements at the focal plane, or used to provide a selective tag for prompt conversion electrons or γ rays measured with arrays of detectors deployed at the target position. A new concept of triggerless data acquisition (total data readout) has also been developed as part of the GREAT project, which circumvents the problems and limitations of common dead time in conventional data acquisition systems.

Nuclear isomers in superheavy elements as stepping stones towards the island of stability

A long-standing prediction of nuclear models is the emergence of a region of long-lived, or even stable, superheavy elements beyond the actinides. These nuclei owe their enhanced stability to closed shells in the structure of both protons and neutrons. However, theoretical approaches to date do not yield consistent predictions of the precise limits of the ‘island of stability’; experimental studies are therefore crucial. The bulk of experimental effort so far has been focused on the direct creation of superheavy elements in heavy ion fusion reactions, leading to the production of elements up to proton number Z = 118 (refs 4, 5). Recently, it has become possible to make detailed spectroscopic studies of nuclei beyond fermium (Z = 100), with the aim of understanding the underlying single-particle structure of superheavy elements. Here we report such a study of the nobelium isotope 254No, with 102 protons and 152 neutrons—the heaviest nucleus studied in this manner to date. We find three excited structures, two of which are isomeric (metastable). One of these structures is firmly assigned to a two-proton excitation. These states are highly significant as their location is sensitive to single-particle levels above the gap in shell energies predicted at Z = 114, and thus provide a microscopic benchmark for nuclear models of the superheavy elements.

Superheavy Element Flerovium (Element 114) Is a Volatile Metal

The electron shell structure of superheavy elements, i.e., elements with atomic number Z ≥ 104, is influenced by strong relativistic effects caused by the high Z. Early atomic calculations on element 112 (copernicium, Cn) and element 114 (flerovium, Fl) having closed and quasi-closed electron shell configurations of 6d(10)7s(2) and 6d(10)7s(2)7p1/2(2), respectively, predicted them to be noble-gas-like due to very strong relativistic effects on the 7s and 7p1/2 valence orbitals. Recent fully relativistic calculations studying Cn and Fl in different environments suggest them to be less reactive compared to their lighter homologues in the groups, but still exhibiting a metallic character. Experimental gas-solid chromatography studies on Cn have, indeed, revealed a metal-metal bond formation with Au. In contrast to this, for Fl, the formation of a weak bond upon physisorption on a Au surface was inferred from first experiments. Here, we report on a gas-solid chromatography study of the adsorption of Fl on a Au surface. Fl was produced in the nuclear fusion reaction (244)Pu((48)Ca, 3-4n)(288,289)Fl and was isolated in-flight from the primary (48)Ca beam in a physical recoil separator. The adsorption behavior of Fl, its nuclear α-decay product Cn, their lighter homologues in groups 14 and 12, i.e., Pb and Hg, and the noble gas Rn were studied simultaneously by isothermal gas chromatography and thermochromatography. Two Fl atoms were detected. They adsorbed on a Au surface at room temperature in the first, isothermal part, but not as readily as Pb and Hg. The observed adsorption behavior of Fl points to a higher inertness compared to its nearest homologue in the group, Pb. However, the measured lower limit for the adsorption enthalpy of Fl on a Au surface points to the formation of a metal-metal bond of Fl with Au. Fl is the least reactive element in the group, but still a metal.

Spectroscopy of actinide and transactinide nuclei

Abstract The role of isomers for nuclei with Z ≥ 100 is discussed. Recent advances in experimental instrumentation leading to combined in-beam gamma ray and conversion electron spectroscopy are discussed. The rotational spectra of nuclei with Z ≥ 94 and their moments of inertia are discussed. Examples for in-beam spectroscopy leading to the discovery and identification of isomers are given in 248,250Fm. Here some attention is given to the assignment of nuclear configurations from g-factors measured via the branching ratios of coupled bands built on the isomers. A full list of the longest lived isomers in nuclei with Z ≥ 82 is given.

In-beam spectroscopy using the JYFL gas-filled magnetic recoil separator RITU

The techniques of recoil-gating and recoil-decay tagging have been employed at Jyvaskyla to perform in-beam γ-ray and electron spectroscopy studies of heavy nuclei. The JUROSPHERE γ-ray array and the SACRED electron spectrometer have been placed at the target position of the JYFL gas-filled recoil separator recoil ion transport unit (RITU). The RITU separator has been used to collect the recoils of interest and separate them from beam particles and fission products. At the focal plane a detector system consisting of time-of-flight and implantation detectors has been used for further event identification. The method and some highlights from the results in the lead region close to the proton drip line and in the transuranium region will be presented and discussed.

Search for a 2-quasiparticle high-K isomer in 256Rf

The energies of 2-quasiparticle (2-qp) states in heavy shell-stabilized nuclei provide information on the single-particle states that are responsible for the stability of superheavy nuclei. We have calculated the energies of 2-qp states in {sup 256}Rf, which suggest that a long-lived, low-energy 8{sup -} isomer should exist. A search was conducted for this isomer through a calorimetric conversion electron signal, sandwiched in time between implantation of a {sup 256}Rf nucleus and its fission decay, all within the same pixel of a double-sided Si strip detector. A 17(5)-{mu}s isomer was identified. However, its low population, {approx}5(2)% that of the ground state instead of the expected {approx}30%, suggests that it is more likely a 4-qp isomer. Possible reasons for the absence of an electromagnetic signature of a 2-qp isomer decay are discussed. These include the favored possibility that the isomer decays by fission, with a half-life indistinguishably close to that of the ground state. Another possibility, that there is no 2-qp isomer at all, would imply an abrupt termination of axially symmetric deformed shapes at Z=104, which describes nuclei with Z=92-103 very well.

The SPEDE spectrometer: combined in-beam

The SPEDE spectrometer [1] aims to combine a silicon detector, for the detection of electrons, with the MINIBALL γ-ray detection array for in-beam studies employing radioactive ion beams at the HIE-ISOLDE facility at CERN. The setup will be primarily used for octupole collectivity [2] and shape coexistence studies [3, 4] in Coulomb excitation experiments. In the shape coexistence cases the transitions between states of the same spin and parity have enhanced E0 strength [5]. Additionally the 0→0 transitions, typically present in nuclei exhibiting shape coexistence [6], can only occur via E0 transitions, i.e. via internal conversion electron emission.

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This chapter is dedicated to the nuclear structure of superheavy elements. It brings together all aspects of nuclear structure that have an influence on the stability of the nucleus on the one hand and that form the basis of experiments performed on superheavy elements to elucidate their nuclear structure on the other hand. The liquid drop model (LDM) is introduced and used to explain the limits of stability against fission, before the shell model is used to explain magic numbers and shell stabilization. Rotational properties of deformed nuclei are introduced and their sensitivity to the underlying nuclear structure is explored. The single particle structure and the influence of pairing on nuclei is discussed before experimental techniques for in-beam gamma and conversion electron spectroscopy are introduced. Finally spectroscopy following alpha decay is discussed.

-ray and conversion electron spectroscopy with radioactive ion beams

A comprehensive Geant4 simulation was built for the SAGE spectrometer. The simulation package includes the silicon and germanium detectors, the mechanical structure and the electromagnetic fields present in SAGE. This simulation can be used for making predictions through simulating experiments and for comparing simulated and experimental data to better understand the underlying physics.

Nuclear Structure of Superheavy Elements

Abstract.The electron spectrometer, SPEDE, has been developed and will be employed in conjunction with the Miniball spectrometer at the HIE-ISOLDE facility, CERN. SPEDE allows for direct measurement of internal conversion electrons emitted in-flight, without employing magnetic fields to transport or momentum filter the electrons. Together with the Miniball spectrometer, it enables simultaneous observation of