R. Maser

The Kleiner Feldberg Cloud Experiment 1990. An overview

An overview is given of the Kleiner Feldberg cloud experiment performed from 27 October until 13 November 1990. The experiment was carried out by numerous European research groups as a joint effort within the EUROTRAC-GCE project in order to study the interaction of cloud droplets with atmospheric trace constituents. After a description of the observational site and the measurements which were performed, the general cloud formation mechanisms encountered during the experiment are discussed. Special attention is given here to the process of moist adiabatic lifting. Furthermore, an overview is given regarding the pollutant levels in the gas phase, the particulate and the liquid phase, and some major findings are presented with respect to the experimental objectives. Finally, a first comparison attempts to put the results obtained during this campaign into perspective with the previous GCE field campaign in the Po Valley.

Probing Finescale Dynamics and Microphysics of Clouds with Helicopter-Borne Measurements

Abstract Helicopter-based measurements provide an opportunity for probing the finescale dynamics and microphysics of clouds simultaneously in space and time. Due to the low true air speed compared with research aircraft, a helicopter allows for measurements with much higher spatial resolution. To circumvent the influence of the helicopter downwash the autonomous measurement pay-load Airborne Cloud Turbulence Observation System (ACTOS) is carried as an external cargo 140 m below the helicopter. ACTOS allows for collocated measurements of the dynamical and cloud microphysical parameters with a spatial resolution of better than 10 cm. The interaction between turbulence and cloud microphysical processes is demonstrated using the following two cloud cases from recent helicopter measurements: i) a cumulus cloud with a low degree of turbulence and without strong vertical dynamics, and, in contrast, ii) an actively growing cloud with increased turbulence and stronger updrafts. The turbulence and microphysical mea...

Cloud processing of soluble gases

Abstract Experimental data from the Great Dun Fell Cloud Experiment 1993 were used to investigate interactions between soluble gases and cloud droplets. Concentrations of H 2 O 2 , SO 2 , CH 3 COOOH, HCOOH, and HCHO were monitored at different sites within and downwind of a hill cap cloud and their temporal and spatial evolution during several cloud events was investigated. Significant differences were found between in-cloud and out-of-cloud concentrations, most of which could not be explained by simple dissolution into cloud droplets. Concentration patterns were analysed in relation to the chemistry of cloud droplets and the gas/liquid equilibrium. Soluble gases do not undergo similar behaviour: CH 3 COOH simply dissolves in the aqueous phase and is outgassed upon cloud dissipation; instead, SO 2 is consumed by its reaction with H 2 O 2 . The behaviour of HCOOH is more complex because there is evidence for in-cloud chemical production. The formation of HCOOH interferes with the odd hydrogen cycle by enhancing the liquid-phase production of H 2 O 2 . The H 2 O 2 concentration in cloud therefore results from the balance of consumption by oxidation of SO 2 in-cloud production, and the rate by which it is supplied to the system by entrainment of new air into the clouds.

Phase partitioning of aerosol particles in clouds at Kleiner Feldberg

The partitioning of aerosol particles between cloud droplets and interstitial air by number and volume was determined both in terms of an integral value and as a function of size for clouds on Mt. Kleiner Feldberg (825 m asl), in the Taunus Mountains north-west of Frankfurt am Main, Germany. Differences in the integral values and the size dependent partitioning between two periods during the campaign were observed. Higher number and volume concentrations of aerosol particles in the accumulation mode were observed during Period II compared to Period I. In Period I on average 87±11% (±one standard deviation) and 73±7% of the accumulation mode volume and number were incorporated into cloud droplets. For Period II the corresponding fractions were 42±6% and 12±2% in one cloud event and 64±4% and 18±2% in another cloud event. The size dependent partitioning as a function of time was studied in Period II and found to have little variation. The major processes influencing the partitioning were found to be nucleation scavenging and entrainment.

The size-dependent chemical composition of cloud droplets

Abstract Size-dependent cloud droplet solute concentrations were measured using a two-stage fog water impactor at the summit station of Great Dun Fell (GDF) in the north of England. The measurements showed mostly higher concentrations in the small-droplet fraction. During one cloud event, however, higher solute concentrations were found in the larger-droplet fraction. In order to identify the factors governing the size dependence of cloud droplet solute concentrations, sensitivity studies by means of a diffusional growth model were performed. The time available for the droplets to grow was identified to be of great importance for the size dependence of solute concentrations. In cases when higher solute concentrations were found in the fraction containing the bigger droplets, the cloud droplets were relatively young having been formed by orographic lifting of the air at the GDF summit. For the other events the evidence indicates that the cloud was already formed far upwind from the summit site. Our experimental and model results imply that, after an initially strong decrease of solute concentrations with droplet size we would observe: • ⊎|increasing solute concentrations with increasing diameters during the initial stage of a cloud, e.g. near cloud base where the droplets have just been formed. The primary factors contributing to this behaviour are high peak supersaturations, large numbers of coarse aerosol particles, and high solubility of the aerosol particles. • ⊎|decreasing solute concentrations with increasing diameters in aged cloud parcels, such as those which can be observed high above the cloud base in cumuliform clouds or are advected to the observation point in the case of stratiform clouds. The primary factors contributing to this behaviour are low peak supersaturations, low numbers of coarse particles, and low solubility of the aerosol particles.

Microphysics of clouds at Kleiner Feldberg

During a field measuring campaign at Kleiner Feldberg (Taunus) in 1990, microphysical characteristics of clouds have been measured by Forward Scattering Spectrometer Probes (FSSP). The aim was to study the influence of aerosol and meteorological factors on droplet size and number. The results are: More mass in the accumulation size range of the aerosol leads to more droplets in stratocumulus clouds and to higher soluble masses in droplets of stratus clouds. However, the aerosol distribution was coarser in the stratus clouds compared to the stratocumulus clouds. Within the first 200 m from cloud base, the droplets grow while their number decreases. The growth results in a stable size of about 14 µm diameter over a large distance from cloud base in many stratocumulus clouds. Two types of mixing processes were observed: processes with reductions in the number of droplets (inhomogeneous mixing) and with reductions in the size of the droplets (homogeneous mixing).

A. TWO-STAGE IMPACTOR FOR FOG DROPLET COLLECTION: DESIGN AND PERFORMANCE

A two-stage fog water impactor was designed for the measurement of size-dependent cloud droplet solute concentrations. The instrument achieves isokinetic sampling conditions by using a variable inlet as well as by using a rotating stand in connection with a wind vane to keep the impactor aligned with the actual mean wind direction. These features are important for reliable results, especially at the high wind velocities which frequently occur at mountain stations. The instrument operated successfully during the Great Dun Fell Cloud Experiment in spring 1993. The results of field measurements, as well as of cloud chamber experiments to test the performance of the instrument are presented.

Deposition of trace substances via cloud interception on a coniferous forest at Kleiner Feldberg

A resistance model to calculate the deposition of cloud droplets on a coniferous forest and some improved parameterizations of the indispensable input parameters are described. The deposition model is adapted to the coniferous forest at the Kleiner Feldberg site and verified by the data of a drip water monitoring station below the forest canopy. The measurements of liqud water content, wind speed and trace substance compounds in cloud water of the Ground-based Cloud Experiment (GCE) at Kleiner Feldberg in 1990 are used to calculate the cloud water deposition fluxes and the deposition of trace substances via cloud water interception. The calculated deposition of trace substances via cloud water interceptions is three to six times higher than via rain during the experiment. On a long term data basis the yearly amount of cloud water deposition is 180 mm year−1 at Kleiner Feldberg site (840 m a.s.l.) while the precipitation amount is 1030 mm year−1. Due to higher trace substance concentrations in cloud water compared to rain the ionic deposition via cloud water interception and via precipitation were assessed to be of comparable magnitude.

Aircraft Particle Inlets: State-of-the-Art and Future Needs

Abstract Aircraft inlets connect airborne instruments for particle microphysical and chemical measurements with the ambient atmosphere. These inlets may bias the measurements due to their potential to enhance or remove certain particle size fractions in the sample. The aircraft body itself may disturb the ambient air streamlines and, hence, the particle sampling. Also, anisokinetic sampling and transmission losses within the sampling lines may cause the sampled aerosol to differ from the ambient aerosol. In addition, inlets may change the particle composition and size through the evaporation of water and other volatile materials due to compressibility effects or heat transfer. These problems have been discussed at an international workshop that was held at the Leibniz-Institute for Tropospheric Research (IfT) in Leipzig, Germany, on 12–13 April 2002. The discussions, conclusions, and recommendations from this workshop are summarized here.

Instrument Intercomparison Study on Cloud Droplet Size Distribution Measurements: Holography vs. Laser Optical Particle Counter

During the EUROTRAC Ground Based Cloud Experiment (GCE) 1990, a newly developed HODAR (Holographic Droplet and Acrosol Recording) was operated for the first time to measure cloud droplet size distributions by recording Fraunhofer in-line holograms of small cloud sample volumes in situ and analyzing the holographic images in the laboratory.This technical note compares the resulting size distributions with those obtained from two FSSP-100 laser optical particle counters. For all holograms analyzed during the GCE90 field experiment, the size distributions obtained from the two different methods agree well. Additionally, the liquid water contents (LWC) were measured directly by a Gerber particulate volume monitor PVM-100. The LWC calculated from the measured droplet size distributions deviate from the PVM-100 data.