R. Nawrodt

Active Optical Metasurfaces Based on Defect-Engineered Phase-Transition Materials

Active, widely tunable optical materials have enabled rapid advances in photonics and optoelectronics, especially in the emerging field of meta-devices. Here, we demonstrate that spatially selective defect engineering on the nanometer scale can transform phase-transition materials into optical metasurfaces. Using ion irradiation through nanometer-scale masks, we selectively defect-engineered the insulator-metal transition of vanadium dioxide, a prototypical correlated phase-transition material whose optical properties change dramatically depending on its state. Using this robust technique, we demonstrated several optical metasurfaces, including tunable absorbers with artificially induced phase coexistence and tunable polarizers based on thermally triggered dichroism. Spatially selective nanoscale defect engineering represents a new paradigm for active photonic structures and devices.

Effect of heat treatment on mechanical dissipation in Ta2O5 coatings

Thermal noise arising from mechanical dissipation in dielectric reflective coatings is expected to critically limit the sensitivity of precision measurement systems such as high-resolution optical spectroscopy, optical frequency standards and future generations of interferometric gravitational wave detectors. We present measurements of the effect of post-deposition heat treatment on the temperature dependence of the mechanical dissipation in ion-beam sputtered tantalum pentoxide between 11 K and 300 K. We find that the temperature dependence of the dissipation is strongly dependent on the temperature at which the heat treatment was carried out, and we have identified three dissipation peaks occurring at different heat treatment temperatures. At temperatures below 200 K, the magnitude of the loss was found to increase with higher heat treatment temperatures, indicating that heat treatment is a significant factor in determining the level of coating thermal noise.

Measurements of a low-temperature mechanical dissipation peak in a single layer of Ta2O5 doped with TiO2

Thermal noise arising from mechanical dissipation in oxide coatings is a major limitation to many precision measurement systems, including optical frequency standards, high-resolution optical spectroscopy and interferometric gravity wave detectors. Presented here are measurements of dissipation as a function of temperature between 7 K and 290 K in ion-beam-sputtered Ta2O5 doped with TiO2, showing a loss peak at 20 K. Analysis of the peak provides the first evidence of the source of dissipation in doped Ta2O5 coatings, leading to possibilities for the reduction of thermal noise effects.

Comparison of the temperature dependence of the mechanical dissipation in thin films of Ta2O5 and Ta2O5 doped with TiO2

Here we report the first results comparing the temperature dependence of the mechanical dissipation in thin films of Ta_2O_5 and Ta_2O_5 doped with TiO_2, of a type suitable for use in the multilayer optical coatings for advanced gravitational wave detectors. The results indicate that doping Ta_2O_5 with TiO_2 can significantly alter the distribution of activation energies associated with the low-temperature dissipation peak.

Low temperature mechanical dissipation of an ion-beam sputtered silica film

Thermal noise arising from mechanical dissipation in oxide mirror coatings is an important limit to the sensitivity of future gravitational wave detectors, optical atomic clocks and other precision measurement systems. Here, we present measurements of the temperature dependence of the mechanical dissipation of an ion-beam sputtered silica film between 10 and 300 K. A dissipation peak was observed at 20 K and the low temperature dissipation was found to have significantly different characteristics than observed for bulk silica and silica films deposited by alternative techniques. These results are important for better understanding the underlying mechanisms of mechanical dissipation, and thus thermal noise, in the most commonly-used reflective coatings for precision measurements.

Cryogenic mechanical loss measurements of heat-treated hafnium dioxide

Low mechanical loss, high index-of-refraction thin-film coating materials are of particular interest to the gravitational wave detection community, where reduced mirror coating thermal noise in gravitational wave detectors is desirable. Current studies are focused on understanding the loss of amorphous metal oxides such as SiO2, Ta2O5 and HfO2. Here, we report recent measurements of the temperature dependence of the mechanical loss of ion-beam sputtered hafnium dioxide (HfO2) coatings that have undergone heat treatment. The results indicate that, even when partially crystallized, these coatings have lower loss than amorphous Ta2O5 films below ~100 K and that their loss exhibits some features which are heat-treatment dependent in the temperature range of ~100–200 K, with higher heat treatment yielding lower mechanical loss. The potential for using silica doping of hafnia coatings to prevent crystallization is discussed.

Calculation of thermal noise in grating reflectors

Grating reflectors have been repeatedly discussed to improve the noise performance of metrological applications due to the reduction or absence of any coating material. So far, however, no quantitative estimate on the thermal noise of these reflective structures exists. In this work we present a theoretical calculation of a grating reflector’s noise. We further apply it to a proposed third generation gravitational wave detector. Depending on the grating geometry, the grating material, and the temperature, we obtain a thermal noise decrease by up to a factor of 10 compared to conventional dielectric mirrors. Thus the use of grating reflectors can substantially improve the noise performance in metrological applications.

Silicon mirror suspensions for gravitational wave detectors

One of the most significant limits to the sensitivity of current, and future, long-baseline interferometric gravitational wave detectors is thermal displacement noise of the test masses and their suspensions. This paper reports results of analytical and experimental studies of the limits to thermal noise performance of cryogenic silicon test mass suspensions set by two constraints on suspension fibre dimensions: the minimum dimensions required to allow conductive cooling for extracting incident laser beam heat deposited in the mirrors; and the minimum dimensions of fibres (set by their tensile strength) which can support test masses of the size envisaged for use in future detectors. We report experimental studies of breaking strength of silicon ribbons, and resulting design implications for the feasibility of suspension designs for future gravitational wave detectors using silicon suspension fibres. We analyse the implication of this study for thermal noise performance of cryogenically cooled silicon suspensions.

Low-temperature strength tests and SEM imaging of hydroxide catalysis bonds in silicon

Silicon is under consideration as a substrate material for the test masses and suspension elements of gravitational wave detectors of improved sensitivity. Hydroxide catalysis bonding is a candidate technique for jointing silicon elements with the potential for both high strength and low mechanical loss. A future detector with quasi-monolithic silicon final stages may operate at cryogenic temperatures. Here we present the first studies of the strength of silicon–silicon bonds at 77 K (liquid nitrogen temperature) and show characteristic strengths of ~44 MPa. When comparing cryogenic to room temperature results, no significant difference is apparent in the strength. We also show that a minimum thickness of oxide layer of 50 nm is desirable to achieve reliably strong bonds. Bonds averaging 47 nm in thickness are achieved for oxide thicknesses greater than 50 nm.

Measurement of the mechanical loss of prototype GaP/AlGaP crystalline coatings for future gravitational wave detectors

Thermal noise associated with the dielectric optical coatings used to form the mirrors of interferometric gravitational wave detectors is expected to be an important limit to the sensitivity of future detectors. Improvements in detector performance are likely to require coating materials of lower mechanical dissipation. Typically, current coatings use multiple alternating layers of ion-beam-sputtered amorphous silica and tantalum pentoxide (doped with titania). We present here measurements of the mechanical dissipation of promising alternative crystalline coatings that use multi-layers of single crystal gallium phosphide (GaP) and aluminium gallium phosphide (AlGaP) that are epitaxially grown and lattice matched to a silicon substrate. Analysis shows that the dissipation of the crystalline coating materials appears to be significantly lower than that of the currently used amorphous coatings, potentially enabling a reduction of coating thermal noise in future gravitational wave detectors.