Reimar Waitz

Subharmonic Resonant Optical Excitation of Confined Acoustic Modes in a Free-Standing Semiconductor Membrane at GHz Frequencies with a High-Repetition-Rate Femtosecond Laser

We propose subharmonic resonant optical excitation with femtosecond lasers as a new method for the characterization of phononic and nanomechanical systems in the gigahertz to terahertz frequency range. This method is applied for the investigation of confined acoustic modes in a free-standing semiconductor membrane. By tuning the repetition rate of a femtosecond laser through a subharmonic of a mechanical resonance we amplify the mechanical amplitude, directly measure the linewidth with megahertz resolution, infer the lifetime of the coherently excited vibrational states, accurately determine the systems quality factor, and determine the amplitude of the mechanical motion with femtometer resolution.

Optical transmission and laser structuring of silicon membranes

The optical linear and nonlinear properties of ~ 340-nm thick Si membranes were investigated. The investigation included both experiments in which the reflection and transmission from the membranes were measured, and finite differences time domain simulations. The linear optical transmission of the Si membranes can be controlled by changing the thickness of a thermally grown oxide on the membrane. Illumination of the membranes with high levels of irradiation leads to optical modifications that are consistent with the formation of amorphous silicon and dielectric breakdown. When irradiated under conditions where dielectric breakdown occurs, the membranes can be ablated in a well-controlled manner. Laser micro-structuring of the membranes by ablation was carried out to make micrometer-sized holes by focused fs-pulses. Ns-pulses were also used to fabricate arrays of holes by proximity-ablation of a closely-packed pattern of colloidal particles.

Lateral and temporal dependence of the transport through an atomic gold contact under light irradiation: signature of propagating surface plasmon polaritons.

Metallic point contacts (MPCs) with dimensions comparable to the Fermi wavelength of conduction electrons act as electronic waveguides and might operate as plasmon transmitters. Here we present a correlated study of optical and conductance response of MPCs under irradiation with laser light. For elucidating the role of surface plasmon polaritons (SPPs), we integrate line gratings into the leads that increase the SPP excitation efficiency. By analyzing spatial, polarization, and time dependence, we identify two SPP contributions that we attribute to transmitted and decaying SPPs, respectively. The results demonstrate the role of SPPs for optically controlling the transport in metallic nanostructures and are important for designing opto-nanoelectronic devices.

Nanofabricated adjustable multicontact devices on membranes

Adjustable atomic size contacts realized by break junctions have become a standard tool during the last decade. Although nanofabricated break junctions may in principle be incorporated onto complex electronic circuits, a fundamental drawback of the standard break junction technique is its limitation to a single adjustable junction per device. We have fabricated single break junctions as well as devices containing two break junctions on a silicon membrane. The junctions are adjusted by positioning a fine tip via piezocontrol on the rear side of the membrane. We describe the fabrication process of the membranes and the devices and present results obtained on circuits made of gold and platinum. We show that the junctions can be addressed independently by a suitable choice of the tip position. Single-atom contacts, vacuum tunneling contacts as well as larger contacts can be stabilized.

Vibrational modes of ultrathin carbon nanomembrane mechanical resonators

We report measurements of vibrational mode shapes of mechanical resonators made from ultrathin carbon nanomembranes (CNMs) with a thickness of approximately 1 nm. CNMs are prepared from electron irradiation induced cross-linking of aromatic self-assembled monolayers and the variation of membrane thickness and/or density can be achieved by varying the precursor molecule. Single- and triple-layer freestanding CNMs were made by transferring them onto Si substrates with square/rectangular orifices. The vibration of the membrane was actuated by applying a sinusoidal voltage to a piezoelectric disk on which the sample was glued. The vibrational mode shapes were visualized with an imaging Mirau interferometer using a stroboscopic light source. Several mode shapes of a square membrane can be readily identified and their dynamic behavior can be well described by linear response theory of a membrane with negligible bending rigidity. By applying Fourier transformations to the time-dependent surface profiles, the dispersion relation of the transverse membrane waves can be obtained and its linear behavior verifies the membrane model. By comparing the dispersion relation to an analytical model, the static stress of the membranes was determined and found to be caused by the fabrication process.

Time-resolved detection of propagating Lamb waves in thin silicon membranes with frequencies up to 197 GHz

Guided acoustic waves are generated in nanopatterned silicon membranes with aluminum gratings by optical excitation with a femtosecond laser. The spatial modulation of the photoacoustic excitation leads to Lamb waves with wavelengths determined by the grating period. The excited Lamb waves are optically detected for different grating periods and at distances up to several μm between pump and probe spot. The measured frequencies are compared to the theoretical dispersion relation for Lamb waves in thin silicon membranes. Compared to surface acoustic waves in bulk silicon twice higher frequencies for Lamb waves (197 GHz with a 100 nm grating) are generated in a membrane at equal grating periods.

Time-resolved optical measurement of thermal transport by surface plasmon polaritons in thin metal stripes

We investigate the thermal transport originating from the propagation of surface plasmon polaritons (SPPs) in a thin gold stripe. The SPPs are excited by a grating coupler on the Au stripe which was patterned onto a silicon membrane. The transmissivity changes of the Si membrane due to temperature-induced changes of the interference conditions enable measuring the temperature distribution with temporal and spatial resolution better than 1 μs and 1 μm. With this setup, we demonstrate that SPP excitation, propagation, and decay are accompanied by considerable heating and heat transport.

Characterization and applications of plasmon fields in metal nanostructures

The excitation of plasmons in metallic nanostructures by light can give rise to pronounced local optical field enhancement with respect to the incident electromagnetic field. The details of these optical near fields depend sensitively on the properties of the nanostructures (material, size and shape), on the light wavelength and polarization, and also on the substrate. In this article we discuss several of these aspects influencing the near-field distribution for a given object and the resulting surface ablation by optical near fields. To this end we use both experimental and simulation techniques. Additionally we will present first results of experiments investigating the light emitted during nanoscale ablation. Finally, we will present an example how plasmon-mediated near-field effects act on the conductance of atomic-size contacts.

Fast quantitative optical detection of heat dissipation by surface plasmon polaritons

Heat management at the nanoscale is an issue of increasing importance. In optoelectronic devices the transport and decay of plasmons contribute to the dissipation of heat. By comparison of experimental data and simulations we demonstrate that it is possible to gain quantitative information about excitation, propagation and decay of surface plasmon polaritons (SPPs) in a thin gold stripe supported by a silicon membrane. The temperature-dependent optical transmissivity of the membrane is used to determine the temperature distribution around the metal stripe with high spatial and temporal resolution. This method is complementary to techniques where the propagation of SPPs is monitored optically, and provides additional information which is not readily accessible by other means. In particular, we demonstrate that the thermal conductivity of the membrane can also be derived from our analysis. The results presented here show the high potential of this tool for heat management studies in nanoscale devices.

Optical generation of a broadband acoustic frequency comb in the 100 GHz-regime

Acoustic properties in the GHz frequency range are not very well understood for most semiconductors although intrinsic attenuation and scattering at interfaces of acoustic waves is of great interest for both fundamental and applied science. Additionally adhesion properties of very thin films are both hard to control and to evaluate. A thin silicon membrane with an aluminum transducer on top is used to gain knowledge of these crucial properties. The two-layer system is investigated by asynchronous optical sampling, a pump-probe technique employing 2 fs lasers [1]. The pump pulse generates strain fronts in the membrane, which are propagating and thereby defining a pulse. The Si/air-interface and the Al/air interface act as mirros and reflect the acoustic pulse. As a result an acoustic cavity is formed.