Richard Hall-Wilton

B4C thin films for neutron detection

Due to the very limited availability of He-3, new kinds of neutron detectors, not based on 3He, are urgently needed. Here, we present a method to produce thin films of (B4C)-B-10, with maximized de ...

A very intense neutrino super beam experiment for leptonic CP violation discovery based on the European spallation source linac

Very intense neutrino beams and large neutrino detectors will be needed in order to enable the discovery of CP violation in the leptonic sector. We propose to use the proton linac of the European Spoliation Source currently under construction in Lund, Sweden, to deliver, in parallel with the spoliation neutron production, a very intense, cost effective and high performance neutrino beam. The baseline program for the European Spoliation Source linac is that it will be fully operational at 5 MW average power by 2022, producing 2 GeV 2.86 ms long proton pulses at a rate of 14 Hz. Our proposal is to upgrade the linac to 10 MW average power and 28 Hz, producing 14 pulses/s for neutron production and 14 pulses/s for neutrino production. Furthermore, because of the high current required in the pulsed neutrino horn, the length of the pulses used for neutrino production needs to be compressed to a few mu s with the aid of an accumulator ring. A long baseline experiment using this Super Beam and a megaton underground Water Cherenkov detector located in existing mines 300-600 km from Lund will make it possible to discover leptonic CP violation at 5 sigma significance level in up to 50% of the leptonic Dirac CP-violating phase range. This experiment could also determine the neutrino mass hierarchy at a significance level of more than 3 sigma if this issue will not already have been settled by other experiments by then. The mass hierarchy performance could be increased by combining the neutrino beam results with those obtained from atmospheric neutrinos detected by the same large volume detector. This detector will also be used to measure the proton lifetime, detect cosmological neutrinos and neutrinos from supernova explosions. Results on the sensitivity to leptonic CP violation and the neutrino mass hierarchy are presented

Neutron Position Sensitive Detectors for the ESS

The European Spallation Source (ESS) in Lund, Sweden will become the worlds leading neutron source for the study of materials. The instruments are being selected from conceptual proposals submitted by groups from around Europe. These instruments present numerous challenges for detector technology in the absence of the availability of Helium-3, which is the default choice for detectors for instruments built until today and due to the extreme rates expected across the ESS instrument suite. Additionally a new generation of source requires a new generation of detector technologies to fully exploit the opportunities that this source provides. The detectors will be sourced from partners across Europe through numerous in-kind arrangements; a process that is somewhat novel for the neutron scattering community. This contribution presents briefly the current status of detectors for the ESS, and outlines the timeline to completion. For a conjectured instrument suite based upon instruments recommended for construction, a recently updated snapshot of the current expected detector requirements is presented. A strategy outline as to how these requirements might be tackled by novel detector developments is shown. In terms of future developments for the neutron community, synergies should be sought with other disciples, as recognized by various recent initiatives in Europe, in the context of the fundamentally multi-disciplinary nature of detectors. This strategy has at its basis the in-kind and collaborative partnerships necessary to be able to produce optimally performant detectors that allow the ESS instruments to be world-leading. This foresees and encourages a high level of collaboration and interdependence at its core, and rather than each group being all-rounders in every technology, the further development of centres of excellence across Europe for particular technologies and niches.

Geant4 based simulations for novel neutron detector development

A Geant4-based Python/C++ simulation and coding framework, which has been developed and used in order to aid the R&D efforts for thermal neutron detectors at neutron scattering facilities, is described. Built upon configurable geometry and generator modules, it integrates a general purpose object oriented output file format with meta-data, developed to facilitate a faster turn-around time when setting up and analysing simulations. Also discussed are the extensions to Geant4 which have been implemented in order to include the effects of low-energy phenomena such as Bragg diffraction in the polycrystalline support materials of the neutron detectors. Finally, an example application of the framework is briefly shown.

Investigation of gamma-ray sensitivity of neutron detectors based on thin converter films

Currently, many detector technologies for thermal neutron detection are in development in order to lower the demand for the rare 3He gas. Gas detectors with solid thin film neutron converters readout by gas proportional counter method have been proposed as an appropriate choice for applications where large area coverage is necessary. In this paper, we investigate the probability for γ-rays to generate a false count in a neutron measurement. Simulated results are compared to measurement with 10B thin film prototypes and a 3He detector. It is demonstrated that equal γ-ray rejection to that of 3He tubes is achieved with the new technology. The arguments and results presented here are also applicable to gas detectors with converters other than solid 10B layers, such as 6Li layers and 10BF3 gas.

Boron carbide coatings for neutron detection probed by x-rays, ions, and neutrons to determine thin film quality

Due to the present shortage of 3He and the associated tremendous increase of its price, the supply of large neutron detection systems with 3He becomes unaffordable. Alternative neutron detection concepts, therefore, have been invented based on solid 10B converters. These concepts require development in thin film deposition technique regarding high adhesion, thickness uniformity and chemical purity of the converter coating on large area substrates. We report on the sputter deposition of highly uniform large-area 10B4C coatings of up to 2 μm thickness with a thickness deviation below 4% using the Helmholtz-Zentrum Geesthacht large area sputtering system. The 10B4C coatings are x-ray amorphous and highly adhesive to the substrate. Material analysis by means of X-ray-Photoelectron Spectroscopy, Secondary-Ion-Mass-Spectrometry, and Rutherford-Back-Scattering (RBS) revealed low impurities concentration in the coatings. The isotope composition determined by Secondary-Ion-Mass-Spectrometry, RBS, and inelastic nuclear reaction analysis of the converter coatings evidences almost identical 10B isotope contents in the sputter target and in the deposited coating. Neutron conversion and detection test measurements with variable irradiation geometry of the converter coating demonstrate an average relative quantum efficiency ranging from 65% to 90% for cold neutrons as compared to a black 3He-monitor. Thus, these converter coatings contribute to the development of 3He-free prototype detectors based on neutron grazing incidence. Transferring the developed coating process to an industrial scale sputtering system can make alternative 3He-free converter elements available for large area neutron detection systems.

A B-10-based neutron detector with stacked MultiWire Proportional Counters and macrostructured cathodes

We present the results of the measurements of the detection efficiency for a 4.7 angstrom neutron beam incident upon a detector incorporating a stack of up to five MultiWire Proportional Counters (MWPC) with Boron-coated cathodes. The cathodes were made of Aluminum and had a surface exhibiting millimeter-deep V-shaped grooves of 45 degrees, upon which the thin Boron film was deposited by DC magnetron sputtering. The incident neutrons interacting with the converter layer deposited on the sidewalls of the grooves have a higher capture probability, owing to the larger effective absorption film thickness. This leads to a higher overall detection efficiency for the grooved cathode when compared to a cathode with a flat surface. Both the experimental results and the predictions of the GEANT4 model suggests that a 5-counter detector stack with coated grooved cathodes has the same efficiency as a 7-counter stack with flat cathodes. The reduction in the number of counters in the stack without altering the detection efficiency will prove highly beneficial for large-area position-sensitive detectors for neutron scattering applications, for which the cost-effective manufacturing of the detector and associated readout electronics is an important objective. The proposed detector concept could be a technological option for one of the new chopper spectrometers and other instruments planned to be built at the future European Spallation Source in Sweden. These results with macrostructured cathodes generally apply not just to MWPCs but to other gaseous detectors as well.

10B multi-grid proportional gas counters for large area thermal neutron detectors

Introduction 10B fi lms have been studied as neutron convertors in semi-conductors [1], and in different types of gas proportional counters for neutron scattering applications: for example in [2] the detector is made of several layers of straw tubes coated on the inner side with B4C; in [3] several parallel GEM (Gas Electron Multipliers) operated with an amplifi cation gain of 1 are coated with B4C fi lms on both sides; and in [4], inclined substrates are proposed to reduce the self-absorption of fi ssion products in the convertor. These different solutions are well suited for small size detectors requiring high counting rate and high spatial resolution but not for large area detectors mounted in vacuum chambers. The multi-grid detector, introduced at the ILL in 2010 [5], is developed in collaboration with European Spallation Source (ESS) in the CRISP project (http://www.crisp-fp7.eu/) to replace 3He in large-Area Neutron detectors. We present its principle as well as some results obtained with a prototype of 8 cm × 200 cm. This contribution to the study of 10B-fi lms detectors has been done in the frame of the International Initiative to search for 3He alternative technologies (http://icnd. org/). Results obtained by other institutes are accessible via the web page of the last workshop dedicated to BF3 and 10B-fi lm detectors (http://www.ill.eu/10bbf3, see also NN 23.3, p. 6).

Mixing thermodynamics of TM1-xGdxN (TM=Ti, Zr, Hf) from first principles

The mixing thermodynamics of GdN with TiN, ZrN, and HfN is studied using first-principles methods. We find that while Ti(1-x)Gd(x)N has a strong preference for phase separation due to the large lat ...

Tagging fast neutrons from an (241)Am/(9)Be source.

Shielding, coincidence, and time-of-flight measurement techniques are employed to tag fast neutrons emitted from an (241)Am/(9)Be source resulting in a continuous polychromatic energy-tagged beam of neutrons with energies up to 7MeV. The measured energy structure of the beam agrees qualitatively with both previous measurements and theoretical calculations.